全文获取类型
收费全文 | 843篇 |
免费 | 18篇 |
国内免费 | 16篇 |
专业分类
安全科学 | 14篇 |
废物处理 | 62篇 |
环保管理 | 75篇 |
综合类 | 101篇 |
基础理论 | 177篇 |
环境理论 | 1篇 |
污染及防治 | 322篇 |
评价与监测 | 76篇 |
社会与环境 | 45篇 |
灾害及防治 | 4篇 |
出版年
2023年 | 9篇 |
2022年 | 55篇 |
2021年 | 51篇 |
2020年 | 17篇 |
2019年 | 21篇 |
2018年 | 45篇 |
2017年 | 45篇 |
2016年 | 60篇 |
2015年 | 41篇 |
2014年 | 61篇 |
2013年 | 83篇 |
2012年 | 63篇 |
2011年 | 55篇 |
2010年 | 36篇 |
2009年 | 37篇 |
2008年 | 50篇 |
2007年 | 33篇 |
2006年 | 30篇 |
2005年 | 14篇 |
2004年 | 16篇 |
2003年 | 14篇 |
2002年 | 13篇 |
2001年 | 7篇 |
2000年 | 1篇 |
1999年 | 4篇 |
1998年 | 3篇 |
1997年 | 1篇 |
1996年 | 3篇 |
1995年 | 3篇 |
1994年 | 2篇 |
1991年 | 1篇 |
1984年 | 1篇 |
1957年 | 1篇 |
1956年 | 1篇 |
排序方式: 共有877条查询结果,搜索用时 46 毫秒
41.
Carolina Fernández-Ramos Oscar Ballesteros Alberto Zafra-Gómez Francisco Javier Camino-Sánchez Rosario Blanc Alberto Navalón José Luís Vílchez 《Environmental science and pollution research international》2014,21(6):4286-4296
The study describes the environmental monitoring of anionic surfactants―alcohol sulfates (AS) and alcohol ethoxysulfates (AES)—in marine sediments. Concentration values were obtained after pressurised liquid extraction (PLE) and liquid chromatography–tandem mass spectrometry analysis (LC–MS/MS). Samples were collected from a range of wastewater discharge points along the coast of the provinces of Huelva, Málaga, Granada and Almería. Urban, agricultural and industrial wastewaters are discharged at the selected 38 sampling sites. Principal component analysis was carried out in order to evaluate the distribution and behaviour of these compounds in these coastal environments. Evaluation of the data revealed that the behaviour and sources of AS and AES in marine sediments are different, and that the distribution of AES depends on the length of the alkyl chain, while the number of ethoxylated units is not relevant. Additionally, the 38 sampling sites can be grouped into only two types of outfalls according to their AS distribution. The concentration of compounds in sediment samples ranged from 7.52 to 13.50 mg kg?1 for AS, from 3.04 to 10.68 mg kg?1 for AES–C12Ex and from 3.83 to 11.56 mg kg?1 for AES–C14Ex. 相似文献
42.
Patterns of land-use and land-cover change are usually grouped into one of two categories defined by the dominant trend: (1) deforestation resulting from expanding agriculture and (2) forest expansion, usually related to the abandonment of marginal lands. At regional scale, however, both processes can occur simultaneously even in the absence of net change. Given the focus on net change, such redistribution of agricultural and natural and seminatural lands has been generally overlooked. The interaction between agriculture modernization, human demography and complex topographic gradients of northwestern Argentina has resulted in processes of both forest recovery and deforestation, thus providing the opportunity to analyze patterns and driving forces of land-cover redistribution. We analyzed 20 years (1986–2006) of land-cover change in a subtropical watershed in relation to topographic and demographic variables. Although net forest change represented <1 %, forests redistribution affected 7 % of forest lands. There was a consistent geographic segregation of deforestation and forest recovery, with forests expanding over steep highlands and agriculture expanding over lowland irrigated areas. Population trends were not associated to forest expansion in lowlands but they explained 32 % of forest recovery in highlands. Highland forest expansion and lowland deforestation, respectively, imply conservation opportunities for humid montane forests and the environmental services they provide (e.g., watershed conservation) and threats for the conservation of dry forests and its biodiversity. Our study exemplifies the importance of land-use redistribution (rather than net change) with relevant environmental consequences at regional scale. 相似文献
43.
Tatiana Simonetto Colla Robson Andreazza Francielle Bücker Marcela Moreira de Souza Letícia Tramontini Gerônimo Rodrigues Prado Ana Paula Guedes Frazzon Flávio Anastácio de Oliveira Camargo Fátima Menezes Bento 《Environmental science and pollution research international》2014,21(4):2592-2602
This study investigated the effectiveness of successive bioaugmentation, conventional bioaugmentation, and biostimulation of biodegradation of B10 in soil. In addition, the structure of the soil microbial community was assessed by polymerase chain reaction-denaturing gradient gel electrophoresis. The consortium was inoculated on the initial and the 11th day of incubation for successive bioaugmentation and only on the initial day for bioaugmentation and conventional bioaugmentation. The experiment was conducted for 32 days. The microbial consortium was identified based on sequencing of 16S rRNA gene and consisted as Pseudomonas aeruginosa, Achromobacter xylosoxidans, and Ochrobactrum intermedium. Nutrient introduction (biostimulation) promoted a positive effect on microbial populations. The results indicate that the edaphic community structure and dynamics were different according to the treatments employed. CO2 evolution demonstrated no significant difference in soil microbial activity between biostimulation and bioaugmentation treatments. The total petroleum hydrocarbon (TPH) analysis indicated a biodegradation level of 35.7 and 32.2 % for the biostimulation and successive bioaugmentation treatments, respectively. Successive bioaugmentation displayed positive effects on biodegradation, with a substantial reduction in TPH levels. 相似文献
44.
Distribution of PCDD/Fs and dioxin-like PCBs in sediment and plants from a contaminated salt marsh (Tejo estuary,Portugal) 总被引:1,自引:0,他引:1
Margarida Nunes Anaïs Vernisseau Philippe Marchand Bruno Le Bizec Fernando Ramos Miguel A. Pardal 《Environmental science and pollution research international》2014,21(4):2540-2549
Concentrations and profiles of 2,3,7,8-substituted polychlorinated dibenzo-p-dioxins, polychlorinated dibenzofurans (PCDD/Fs) and dioxin-like polychlorinated biphenyls (dl-PCBs) were investigated in sediment and plants collected from a salt marsh in the Tejo estuary, Portugal. The highest PCDD/F and dl-PCB concentrations were detected in uncolonized sediments, averaging 325.25?±?57.55 pg g?1 dry weight (dw) and 8,146.33?±?2,142.14 pg g?1 dw, respectively. The plants Sarcocornia perennis and Halimione portulacoides growing in PCDD/F and dl-PCB contaminated sediments accumulated contaminants in roots, stems, and leaves. It was observed that PCDD/F and dl-PCB concentrations in roots were significantly lower in comparison with stems and leaves. In general, concentration of ΣPCDD/Fs and Σdl-PCBs in H. portulacoides tissues were found to be twofold higher than those in S. perennis, indicating a difference in the accumulation capability of both species. Furthermore, congener profiles changed between sediments and plant tissues, reflecting a selective accumulation of low chlorinated PCDD/Fs and non-ortho dl-PCBs in plants. 相似文献
45.
Silvestre García de Jalón Ana Iglesias Ruth Cunningham Juan I. Pérez Díaz 《Regional Environmental Change》2014,14(3):1229-1242
Agricultural water management needs to evolve in view of increased water scarcity, especially when farming and natural protected areas are closely linked. In the study site of Doñana (southern Spain), water is shared by rice producers and a world heritage biodiversity ecosystem. Our aim is to contribute to defining adaptation strategies that may build resilience to increasing water scarcity and minimize water conflicts among agricultural and natural systems. The analytical framework links a participatory process with quantitative methods to prioritize the adaptation options. Bottom-up proposed adaptation measures are evaluated by a multi-criteria analysis (MCA) that includes both socioeconomic criteria and criteria of the ecosystem services affected by the adaptation options. Criteria weights are estimated by three different methods—analytic hierarchy process, Likert scale and equal weights—that are then compared. Finally, scores from an MCA are input into an optimization model used to determine the optimal land-use distribution in order to maximize utility and land-use diversification according to different scenarios of funds and water availability. While our results show a spectrum of perceptions of priorities among stakeholders, there is one overriding theme that is to define a way to restore part of the rice fields to natural wetlands. These results hold true under the current climate scenario and even more so under an increased water scarcity scenario. 相似文献
46.
Brondi SH De Macedo AN de Souza GB Nogueira AR 《Journal of environmental science and health. Part. B》2011,46(8):671-677
Analytical methods for the isolation and determination of cypermethrin in milk, based on the solid-phase microextraction (SPME) and QuEChERS methods (Quick, Easy, Cheap, Effective, Rugged, and Safe) are presented. The SPME technique was not appropriate to analyse cypermethrin in milk, even establishing the best extraction conditions, polydimethylsiloxane fiber, 60 min time extraction, 60 °C temperature extraction, addition of salt (NaCl) and stirring rate. The extraction efficiency was low probably because of the matrix constituents. The QuEChERS method involves the extraction of the analyte with acetonitrile and simultaneous liquid-liquid partitioning formed by adding anhydrous MgSO(4) plus NaCl, followed by the removal of residual water and cleanup using a procedure called dispersive solid-phase extraction, in which anhydrous MgSO(4) plus PSA and C18 are mixed with 1 mL of acetonitrile extract. The detection and quantification limits were 0.01 and 0.04 mg kg(-1), respectively, and the percentage recovery obtained ranged from 92 to 105% with relative standard deviations below 7%. 相似文献
47.
Nogueira L Sanches AL da Silva DG Ferrizi VC Moreira AB de Almeida EA 《Chemosphere》2011,85(1):97-105
Fossil fuels such as diesel are being gradually replaced by biodiesel, a renewable energy source, cheaper and less polluting. However, little is known about the toxic effects of this new energy source on aquatic organisms. Thus, we evaluated biochemical biomarkers related to oxidative stress in Nile tilapia (Oreochromis niloticus) after two and seven exposure days to diesel and pure biodiesel (B100) and blends B5 and B20 at concentrations of 0.01 and 0.1 mL L−1. The hepatic ethoxyresorufin-O-deethylase activity was highly induced in all groups, except for those animals exposed to B100. There was an increase in lipid peroxidation in liver and gills in the group exposed to the higher concentration of B5. All treatments caused a significant increase in the levels of 1-hydroxypyrene excreted in the bile after 2 and 7 d, except for those fish exposed to B100. The hepatic glutathione-S-transferase increased after 7 d in animals exposed to the higher concentration of diesel and in the gill of fish exposed to the higher concentration of pure diesel and B5, but decreased for the two tested concentrations of B100. Superoxide dismutase, catalase and glutathione peroxidase also presented significant changes according to the treatments for all groups, including B100. Biodiesel B20 in the conditions tested had fewer adverse effects than diesel and B5 for the Nile tilapia, and can be suggested as a less harmful fuel in substitution to diesel. However, even B100 could activate biochemical responses in fish, at the experimental conditions tested, indicating that this fuel can also represent a risk to the aquatic biota. 相似文献
48.
Filgueiras Ana Virginia Gago Jesús Campillo Juan Antonio León Víctor Manuel 《Environmental science and pollution research international》2019,26(21):21264-21273
Environmental Science and Pollution Research - Microplastics (MPs) are widely recognised as a contaminant of emerging concern in the marine environment. This work provides original data of the... 相似文献
49.
Agata Szygua Eric Guibal María Ario Palacín Montserrat Ruiz Ana Maria Sastre 《Journal of environmental management》2009,90(10):2979-2986
Chitosan (a biopolymer) is an aminopolysaccharide that can be used for the treatment of colored solutions by coagulation–flocculation (as an alternative to more conventional processes such as sorption). Acid Blue 92 (a sulfonic dye) was selected as a model dye for verifying chitosan's ability to treat textile wastewater. A preliminary experiment demonstrated that chitosan was more efficient at color removal in tap water than in demineralized water, and that a substantially lower concentration of chitosan could be used with tap water. Dye removal reached up to 99% under optimum concentration; i.e., in terms of the acidic solutions and the stoichiometric ratio between the amine groups of the biopolymer and the sulfonic groups in the dye. The flocs were recovered and the dye was efficiently removed using alkaline solutions (0.001–1 M NaOH solutions) and the biopolymer, re-dissolved in acetic acid solution, was reused in a further treatment cycle. 相似文献
50.
Miguel Delibes-Mateos Miguel ángel Farfán Jesús Olivero Ana Luz Márquez Juan Mario Vargas 《Environmental management》2009,43(6):1256-1268
Agricultural change has transformed large areas of traditional farming landscapes, leading to important changes in the species
community assemblages in most European countries. We suspect that the drastic changes in land-use that have occurred in Andalusia
(southern Spain) over recent decades, may have affected the distribution and abundance of game species in this region. This
article compares the distribution of the main game species in Andalusia during the 1960s and 1990s, using data from maps available
from the Mainland Spanish Fish, Game and National Parks Service and from recent datasets on hunting yield distributions, respectively.
Big-game and small-game species were significantly segregated in southern Spain during the 1990s, as two clearly independent
chorotypes (groups of species whose abundances are similarly distributed) were obtained from the classification analysis.
In contrast, big-game and small-game species were not significantly segregated several decades ago, when there was only one
chorotype consisting of small-game species and wild boar. The other three ungulates did not constitute a significant chorotype,
as they showed positive correlations with some species in the group mentioned above. These changes seem to be a consequence
of the transformations that have occurred in the Iberian Mediterranean landscape over the last few decades. The abandoning
of traditional activities, and the consequent formation of dense scrubland and woodland, has led to an expansion of big-game
species, and a decrease of small-game species in mountain areas. Moreover, agricultural intensification has apparently depleted
small-game species populations in some agricultural areas. On the other hand, the increasingly intensive hunting management
could be artificially boosting this segregation between small-game and big-game species. Our results suggest that the conservation
and regeneration of traditional agricultural landscapes (like those predominating in the 1960s) should be a priority for the
conservation of small-game species. 相似文献