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21.
Modified Fenton's processes for effective in‐situ chemical oxidation—Laboratory and field evaluation
Prasad K. Kakarla Thomas Andrews Richard S. Greenberg David S. Zervas 《补救:环境净化治理成本、技术与工艺杂志》2002,12(4):23-36
Fenton's reagent in its conventional form, although effective for contaminant treatment, is impractical from an in‐situ field application perspective due to low pH requirements (i.e., pH 3‐4), and limited reagent mobility when introduced into the subsurface. Modified Fenton's processes that use chelated‐iron catalysts and stabilized hydrogen peroxide have been developed with the goal of promoting effective in‐situ field application under native pH conditions (i.e., pH 5‐7), while extending the longevity of hydrogen peroxide. Laboratory experiments conducted in soil columns packed with organic soil to compare modified Fenton's catalysts with conventional catalysts (acidified iron [II]) indicated superior mobility and sorption characteristics for modified Fenton's catalysts. Furthermore, the acidic pH of a conventional catalyst was buffered to the native soil range, leading to increased iron precipitation/adsorption following permeation through the soil column. The chelates present within the modified Fenton's catalyst showed greater affinity toward iron compared with the native soil and, hence, minimized iron loss through adsorption during the permeation process even at pH 5‐7. Field effectiveness of the modified Fenton's process was demonstrated at a former dry‐cleaning facility located in northeast Florida. Preliminary laboratory‐scale experiments were conducted on soil‐slurry and groundwater samples to test the process efficacy for remediation of chlorinated solvents. Based on successful experimental results that indicated a 94 percent (soil slurry) to 99 percent (groundwater) reduction of cis‐1,2‐DCE, PCE, and TCE, a field‐scale treatment program was initiated utilizing a plurality of dual‐zone direct push injection points installed in a grid fashion throughout the site. Results of treatment indicated a 72 percent reduction in total chlorinated contamination detected in the site groundwater following the first injection event; the reduction increased to 90 percent following the second injection event. © 2002 Wiley Periodicals Inc. 相似文献
22.
E. Andrews P. Saxena S. Musarra L.M. Hildemann P. Koutrakis P.H. McMurry 《Journal of the Air & Waste Management Association (1995)》2013,63(5):648-664
ABSTRACT We summarize the results from the various measurements and the inter-sampler comparisons from Southeastern Aerosol and Visibility Study (SEAVS), a study with one of its objectives to test for closure among chemical, gravimetric and optical measurements of atmospheric aerosol particles. Sulfate and organics are the dominant components of the SEAVS fine particles (nominally, particles with aerodynamic diameter <2.5 u,m) but between 28 and 42% (range over various samplers) of the gravimetrically measured total fine particle concentration is unidentified by the chemical measurements. Estimates of water associated with inorganic components and measurement imprecision do not totally explain the observed difference between gravimetric and chemical measurements. We examine the theoretical and empirical basis for assumptions commonly made in the published literature to extrapolate total fine particle concentration on the basis of chemical measurements of ions, carbon and elements. 相似文献
23.
A 30-year series (1978–2007) of photographic records were analysed to determine changes in lake ice cover, local (low elevation)
and montane (high elevation) snow cover and phenological stages of mountain birch (Betula pubescens ssp. czerepanovii) at the Abisko Scientific Research Station, Sweden. In most cases, the photographic-derived data showed no significant difference
in phenophase score from manually observed field records from the same period, demonstrating the accuracy and potential of
using weekly repeat photography as a quicker, cheaper and more adaptable tool to remotely study phenology in both biological
and physical systems. Overall, increases in ambient temperatures coupled with decreases in winter ice and snow cover, and
earlier occurrence of birch foliage, signal a reduction in the length of winter, a shift towards earlier springs and an increase
in the length of available growing season in the Swedish sub-arctic. 相似文献
24.
Callaghan TV Tweedie CE Akerman J Andrews C Bergstedt J Butler MG Christensen TR Cooley D Dahlberg U Danby RK Daniëls FJ de Molenaar JG Dick J Mortensen CE Ebert-May D Emanuelsson U Eriksson H Hedenås H Henry H R G Hik DS Hobbie JE Jantze EJ Jaspers C Johansson C Johansson M Johnson DR Johnstone JF Jonasson C Kennedy C Kenney AJ Keuper F Koh S Krebs CJ Lantuit H Lara MJ Lin D Lougheed VL Madsen J Matveyeva N Mcewen DC Myers-Smith IH Narozhniy YK Olsson H Pohjola VA Price LW Rigét F Rundqvist S 《Ambio》2011,40(6):705-716
Understanding the responses of tundra systems to global change has global implications. Most tundra regions lack sustained environmental monitoring and one of the only ways to document multi-decadal change is to resample historic research sites. The International Polar Year (IPY) provided a unique opportunity for such research through the Back to the Future (BTF) project (IPY project #512). This article synthesizes the results from 13 papers within this Ambio Special Issue. Abiotic changes include glacial recession in the Altai Mountains, Russia; increased snow depth and hardness, permafrost warming, and increased growing season length in sub-arctic Sweden; drying of ponds in Greenland; increased nutrient availability in Alaskan tundra ponds, and warming at most locations studied. Biotic changes ranged from relatively minor plant community change at two sites in Greenland to moderate change in the Yukon, and to dramatic increases in shrub and tree density on Herschel Island, and in subarctic Sweden. The population of geese tripled at one site in northeast Greenland where biomass in non-grazed plots doubled. A model parameterized using results from a BTF study forecasts substantial declines in all snowbeds and increases in shrub tundra on Niwot Ridge, Colorado over the next century. In general, results support and provide improved capacities for validating experimental manipulation, remote sensing, and modeling studies. 相似文献
25.
Anne H. Beaudreau Kelly S. Andrews Donald A. Larsen Graham Young Brian R. Beckman 《Marine Biology》2011,158(2):439-450
The physiological response of a fish to its environment is mediated through the endocrine axis controlling growth. Therefore,
growth-regulating hormone levels can serve as ecologically relevant indicators of fish growth rate. We quantified variation
in plasma insulin-like growth factor-I (IGF-I) to evaluate its potential as an indicator of growth in lingcod, an economically
and ecologically important bottomfish species in the northeast Pacific. An information-theoretic model selection approach
was used to test the hypothesis that variation in lingcod IGF-I is related to season, body size, and gonadal steroid concentration.
Season and a length × season interaction were the most important predictors of plasma IGF-I among the variables we evaluated,
suggesting that season and body size should be explicitly accounted for when interpreting endocrine patterns in wild fish
populations. This is among the few studies that have measured and interpreted patterns of IGF-I in wild fish and the first
to describe seasonal endocrine profiles in lingcod. 相似文献
26.
Comparison of fine-scale acoustic monitoring systems using home range size of a demersal fish 总被引:1,自引:0,他引:1
Kelly S. Andrews Nick Tolimieri Greg D. Williams Jameal F. Samhouri Chris J. Harvey Phillip S. Levin 《Marine Biology》2011,158(10):2377-2387
We compared the results from fixed acoustic transmitters and transmitters implanted in lingcod Ophiodon elongatus provided by two fine-scale passive acoustic monitoring systems: the older Vemco? Radio Acoustic Positioning (VRAP) system and the newer VR2W Positioning System (VPS) with either three or four receivers.
The four-receiver VPS method calculated five times more positions of lingcod than VRAP and more than twice as many as the
three-receiver VPS. Calculated positions of fixed transmitters were less precise with VRAP than either VPS approach. Measurements
of home range for lingcod were similar between the four-receiver VPS and VRAP, which were both greater than the three-receiver
VPS. Comparisons varied when lingcod were in/near complex habitats. As new technology develops, it is important to understand
how new methods compare to previous methods. This may be important when describing patterns of movement or habitat use in
the context of changes in habitat or management efforts. 相似文献
27.
Abdulmajid M. Na'inna Herodotos N. Phylaktou Gordon E. Andrews 《Journal of Loss Prevention in the Process Industries》2013,26(6):1597-1603
The separation distance (or pitch) between two successive obstacles or rows of obstacles is an important parameter in the acceleration of flame propagation and increase in explosion severity. Whilst this is generally recognised, it has received little specific attention by investigators. In this work a vented cylindrical vessel 162 mm in diameter 4.5 m long was used to study the effect of separation distance of two low blockage (30%) obstacles. The set up was demonstrated to produce overpressure through the fast flame speeds generated (i.e. in a similar mechanism to vapour cloud explosions). A worst case separation distance was found to be 1.75 m which produced close to 3 bar overpressure and a flame speed of about 500 m/s. These values were of the order of twice the overpressure and flame speed with a double obstacle separated 2.75 m (83 characteristic obstacle length scales) apart. The profile of effects with separation distance was shown to agree with the cold flow turbulence profile determined in cold flows by other researchers. However, the present results showed that the maximum effect in explosions is experienced further downstream than the position of maximum turbulence determined in the cold flow studies. It is suggested that this may be due to the convection of the turbulence profile by the propagating flame. The present results would suggest that in many previous studies of repeated obstacles the separation distance investigated might not have included the worst case set up, and therefore existing explosion protection guidelines may not be derived from worst case scenarios. 相似文献
28.
R.M. Kasmani G.E. Andrews H.N. Phylaktou 《Process Safety and Environmental Protection》2013,91(4):245-252
A study of vented explosions in a length over diameter (L/D) of 2 in cylindrical vessel connecting with a vent duct (L/D = 7) is reported. The influence of vent burst pressure and ignition locations on the maximum overpressure and flame speeds at constant vent coefficient, K of 16.4 were investigated to elucidate how these parameters affect the severity of a vented explosion. Propane and methane/air mixtures were studied with equivalence ratio, Φ ranges from 0.8 to 1.6. It is demonstrated that end ignition exhibited higher maximum overpressures and flame speeds in comparison to central ignition, contrary to what is reported in literature. There was a large acceleration of the flame toward the duct due to the development of cellular flames and end ignition demonstrated to have higher flame speeds prior to entry into the vent due to the larger flame distance. The higher vent flow velocities and subsequent flame speeds were responsible for the higher overpressures obtained. Rich mixtures for propane/air mixtures at Φ = 1.35 had the greatest flame acceleration and the highest overpressures. In addition, the results showed that Bartknecht's gas explosion venting correlation is grossly overestimated the overpressure for K = 16.4 and thus, misleading the impact of the vent burst pressure. 相似文献
29.
We characterise US materials exchanges by means of an exploratory survey, with 63 respondents classified by materials handled, organisation type and implementation strategy. Few respondents handle hazardous materials; instead, most focus on pre-consumer items such as building materials or post-consumer durable goods such as furniture. Non-profit organisations and state/local government agencies predominate in this niche, which fills a gap between ubiquitous for-profit scrap recyclers and used-merchandise stores. There are three distinct implementation strategies: passive listers of materials; active brokers, who become involved in each transaction; and those who take possession of materials for storage and display in a warehouse. Warehouse operations typically have a local focus and a loyal customer base, whereas passive listing services serve larger areas and are undergoing consolidation. Passive listing services appear to be relatively marginal enterprises, although the adoption of Internet technology is improving their viability. 相似文献
30.
Olivia Lee Russel D. Andrews Vladimir N. Burkanov Randall W. Davis 《Marine Biology》2014,161(5):1165-1178
The ontogeny of diving and foraging behavior of northern fur seal pups from a stable population on Bering Island, Russia, was recorded with animal-borne instruments during their first few months at sea, a critical period during their first year at sea. Thirty-five pups were instrumented with satellite-linked time-depth recorders and stomach temperature pills. Diving occurred predominantly at night with deeper and longer dives as the pups matured. Mean dive depths were correlated with lunar illumination, whereas mean dive durations were also correlated with time of day and sex. Foraging success did not differ between sexes, and there was no relationship between meal size (as indicated by feeding event duration and minimum stomach temperature) and lunar illumination fraction or maximum foraging depth. Although most pups were able to successfully forage within 3 days of starting their migration, the number of feeding events recorded each day remained low (mean 1.6 events day?1). There was no indication of an appreciable increase in meal size after the first 2 weeks of the migration despite an increase in dive frequency and depth. The results are consistent with observations that pups do not gain mass during their first year and emphasize the risk of starvation from infrequent foraging in cold water. 相似文献