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The Science of Nature - 相似文献
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Investigation of the Aerobic Biodegradability of Several Types of Cyclodextrins in a Laboratory-Controlled Composting Test 总被引:1,自引:0,他引:1
Steven Verstichel Bruno De Wilde Eva Fenyvesi József Szejtli 《Journal of Polymers and the Environment》2004,12(2):47-55
The biodegradation of several types of cyclodextrins (CDs) under laboratory-controlled composting conditions was investigated. CDs are used in a broad range of applications in food, pharmaceutical, medical, chemical, and textile industries because of their specific chemical characteristics related to their hydrophobic interior and hydrophilic exterior. The three naturally occurring cyclodextrins -CD, -CD, and -CD proved to be completely and readily biodegradable. Chemical modification of these basic compounds can have a major impact on the biodegradation rate and final biodegradation percentage. Fully acetylated -CD and -CD were found to be nonbiodegradable during 45 days of composting. Reducing the degree of acetylation had a positive effect on the biodegradation. Complete biodegradation was obtained for partially acetylated -CD with a degree of substitution (DS) of 7. The methylation (DS = 13) of -CD resulted in an undegradable compound during the 47 days composting, while (2-hydroxy)propyl--CD reached a plateau in biodegradation at a percentage of 20%. The incorporation of the antimicrobial agents imazalil and allyl-isothiocyanate into -CD had no negative impact on biodegradation, which makes these antimicrobial agents/CD complexes suitable for incorporation into biodegradable active packaging. 相似文献
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Smith KJ León Vintró L Mitchell PI Bally de Bois P Boust D 《Journal of environmental radioactivity》2004,74(1-3):199-210
In this paper we report and compare the concentrations of 234Th and 238U measured in surface and subsurface waters collected in the course of a sampling campaign in the north east Atlantic in June-July 1998. Dissolved 234Th concentrations in surface waters ranged from 5 to 20 Bq m(-3), showing a large deficiency relative to 238U concentrations (typically 42 Bq m-3). This disequilibrium is indicative of active 234Th scavenging from surface waters. Observed 234Th/238U activity ratios, together with corresponding 234Th particulate concentrations, were used to calculate mean residence times for 234Th with respect to scavenging onto particles (tau(diss)) and subsequent removal from surface waters (tau(part)). Residence times in the range 5-30 days were determined for tau(diss) and 4-18 days for tau(part) (n=14). In addition, ultrafiltration experiments at six stations in the course of the same expedition revealed that in north-east Atlantic surface waters a significant fraction (46+/-17%; n=6) of the thorium in the (operationally-defined) dissolved phase (<0.45 microm) is in colloidal form. These observations are consistent with the 'colloidal pumping' model in which it is assumed that 234Th is rapidly absorbed by colloidal particles, which then aggregate, albeit at a slower rate, into larger filterable particles. In essence, colloids act as intermediaries in the transition from the fully dissolved to the filter-retained (>0.45 microm) phase. Thus, the time (tau(c)) for fully dissolved 234Th to appear in the filter-retained fraction is dependent on the rate of colloidal aggregation. Here, we determined tau(c) values in the range 3-17 days. 相似文献
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The results of an assessment study of both industrial and non-industrial dioxin and furan (PCDD/Fs) emissions in the Lombardy Region (Italy) are outlined below. The main data source refer to 1997, and are compiled from the Lombardy Emissions Inventory (developed under the framework of the Regional Air Quality Plan) together with documented emissions factors available. Due to the uncertain nature of the emissions assessment, results are provided as a most probable value within a given range. Total PCDD/Fs emissions in Lombardy average 33 g I-TEQ y(-1), ranging from minimum 13 g I-TEQ y(-1) to maximum 88 g I-TEQ y(-1). The main PCDD/Fs sources are waste incineration, electric arc furnace for steel production, vehicle diesel combustion and residential wood combustion. Incineration emission factors are expected to decrease over the period 2005-2010, in compliance with legal requirements. This will prioritize control over the remaining main PCDD/Fs contributors. Due to limited information available concerning this data, the accuracy of which is uncertain, further research is needed to evaluate the future role of these sources. 相似文献