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61.
Effect of the carbon coating in Fe-C-TiO(2) photocatalyst on phenol decomposition under UV irradiation via photo-Fenton process 总被引:1,自引:0,他引:1
Fe-C-TiO(2) photocatalysts which contained the residue carbon (0.2-3.3 mass%) were prepared from a mixture of TiO(2) and FeC(2)O(4) through the heating at 673-1173 K in Ar. These photocatalysts did not show a high adsorption of phenol, but they were active in photo-Fenton reactions during decomposition of phenol under UV irradiation with addition of H(2)O(2). It was proved that Fe(2+) governed the photoactivity of Fe-C-TiO(2) photocatalysts, it decreased with heat-treatment temperature above 773 K. For comparison, Fe-TiO(2) photocatalyst was prepared by heating TiO(2) and FeC(2)O(4) at 823 K in air for 3h. Phenol decomposition was going much slower on Fe-TiO(2) photocatalyst in comparison with Fe-C-TiO(2), of which mechanism was different, on the former phenol was decomposed by the radical reaction, on the latter through a complex reaction with iron and intermediates of phenol decomposition. Therefore carbon-coating TiO(2) was found to be advantageous for mounting iron and its application for the phenol decomposition via photo-Fenton process. 相似文献
62.
Stef Bokhorst Stine Højlund Pedersen Ludovic Brucker Oleg Anisimov Jarle W. Bjerke Ross D. Brown Dorothee Ehrich Richard L. H. Essery Achim Heilig Susanne Ingvander Cecilia Johansson Margareta Johansson Ingibjörg Svala Jónsdóttir Niila Inga Kari Luojus Giovanni Macelloni Heather Mariash Donald McLennan Gunhild Ninis Rosqvist Atsushi Sato Hannele Savela Martin Schneebeli Aleksandr Sokolov Sergey A. Sokratov Silvia Terzago Dagrun Vikhamar-Schuler Scott Williamson Yubao Qiu Terry V. Callaghan 《Ambio》2016,45(5):516-537
63.
Sonoko Dorothea Bellingrath-Kimura Ayaka Wenhong Kishimoto-Mo Noriko Oura Seiko Sekikawa Seichiro Yonemura Shigeto Sudo Atsushi Hayakawa Kazunori Minamikawa Yusuke Takata Hiroshi Hara 《Ambio》2015,44(1):55-66
The spatial variability of carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O) fluxes from forest soil with high nitrogen (N) deposition was investigated at a rolling hill region in Japan. Gas fluxes were measured on July 25th and December 5th, 2008 at 100 points within a 100 × 100 m grid. Slope direction and position influenced soil characteristics and site-specific emissions were found. The CO2 flux showed no topological difference in July, but was significantly lower in December for north-slope with coniferous trees. Spatial dependency of CH4 fluxes was stronger than that of CO2 or N2O and showed a significantly higher uptake in hill top, and emissions in the valley indicating strong influence of water status. N2O fluxes showed no spatial dependency and exhibited high hot spots at different topology in July and December. The high N deposition led to high N2O fluxes and emphasized the spatial variability. 相似文献
64.
Yoshiaki Mitsui Noriyuki Imada Hirofumi Kikkawa Atsushi Katagawa 《International Journal of Greenhouse Gas Control》2011
Oxy-fuel combustion systems have been under development to reduce CO2 emissions from coal-fired power plants. In oxy-fuel combustion system, Hg in the flue gas causes corrosion in CO2 purification and compression units. Also, SO3 in the flue gas corrodes the equipment and ducts of oxy-fuel combustion system. Therefore, Hg and SO3 need to be removed.Babcock-Hitachi conducted tests using a 1.5 MWth Combustion & Air Quality Control System (AQCS) test facility which consists of oxygen supply unit, furnace, Selective Catalytic Reduction (SCR) catalyst, Clean Energy Recuperator (CER), Dry Electrostatic Precipitator (DESP), flue gas recirculation system, Wet Flue Gas Desulfurization (WFGD), and CO2 Compression and Purification Unit (CPU). In both cases of air and oxy-fuel combustion, the Hg removal across the DESP could be improved, and SO3 concentration at the DESP outlet could be reduced to less than 1 ppm by installing a CER upstream of the DESP and reducing the gas temperature at the DESP inlet. Hg was not dissolved in the drain recovered from CO2 compressor, and may be adsorbed at an inner part of CO2 compressor. This indicated that Hg needs to be removed at a location upstream of the CO2 compressor to prevent corrosion of the compressor. 相似文献
65.
Masahito Ueyama Atsushi KaiKazuhito Ichii Ken HamotaniYoshiko Kosugi Nobutaka Monji 《Ecological modelling》2011,222(17):3216-3225
The role of disturbance and climate factors in determining the forest carbon balance was investigated at a Japanese cypress forest in central Japan with eddy flux measurements, tree-ring analyses, and a terrestrial biosphere model. The forest was established as a plantation after intermittent harvesting and replanting between 1959 and 1977, and acted as a strong carbon sink of approximately 500 g C m−2 year−1 for the measurement years between 2001 and 2007. A terrestrial biosphere model, BIOME-BGC, was validated using the eddy flux data at daily to interannual timescales, and the tree-ring width data at interannual to decadal timescales. According to the model simulation, during the observation period 270 ± 55 g C m−2 year−1 was additionally sequestered due to the indirect effects of the harvesting and planting, whereas the increase of CO2 concentration and the change in climate increased the sink of 110 ± 40 and 30 ± 80 g C m−2 year−1, respectively. The model simulation shows that the forest is now recovering from harvesting, and that harvesting is a more important determinant of the current carbon sink than either interannual climate anomalies or increased atmospheric CO2 concentration. We found that harvesting with long rotation length could be effective management activity in order to increase carbon sequestration, if the harvested timber is converted into products with long lifecycles. 相似文献
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68.
Aya Yoshida Tomohiro Tasaki Atsushi Terazono 《Waste management (New York, N.Y.)》2009,29(5):1602-1614
Most personal computers (PCs) are discarded by consumers after the data files have been moved to a new PC. Therefore, a used PC collection scheme should be created that does not depend on the distribution route of new PCs. In Japan, manufacturers’ voluntary take-back recycling schemes were established in 2001 (for business PCs) and 2003 (for household PCs). At the same time, the export of used PCs from Japan increased, affecting the domestic PC reuse market. These regulatory and economic conditions would have changed the flow of used PCs.In this paper, we developed a method of minimizing the errors in estimating the material flow of used PCs. The method’s features include utilization of both input and output flow data and elimination of subjective estimation as much as possible. Flow rate data from existing surveys were used for estimating the flow of used PCs in Japan for fiscal years (FY) 2000, 2001, and 2004. The results show that 3.92 million and 4.88 million used PCs were discarded in FY 2000 and 2001, respectively. Approximately two-thirds of the discarded PCs were disposed of or recycled within the country, one-fourth was reused within the country, and 8% were exported. In FY 2004, 7.47 million used PCs were discarded. The ratio of domestic disposal and recycling decreased to 37% in FY 2004, whereas the domestic reuse and export ratios increased to 37% and 26%, respectively. Flows from businesses to retailers in FY 2004 increased dramatically, which led to increased domestic reuse. An increase in the flow of used PCs from lease and rental companies to secondhand shops has led to increased exports. Results of interviews with members of PC reuse companies were and trade statistics were used to verify the results of our estimation of domestic reuse and export of used PCs. 相似文献
69.
Masahiro Miura Atsushi Shimahata Toshio Nishikawa Masakazu Aoyama Kiyoshi Tada Junichi Horiuchi Masahiro Nakahara Chikara Sakai 《Journal of Material Cycles and Waste Management》2011,13(1):80-83
To prepare a substrate for microbial conversion of xylose into xylitol, the culm of Sasa senanensis was hydrolyzed with dilute sulfuric acid. When the reaction temperature was fixed at 121°C, an optimum yield of xylose was
obtained by treatment with 2% sulfuric acid for 1 h. An increase in the sulfuric acid concentration or a prolonged reaction
time resulted in a decrease in the xylose yield. A fermentable substrate with a relatively high xylose concentration (36.7
g l−1) was obtained by hydrolysis with 2% sulfuric acid with a liquid-to-solid ratio of 5 g g−1. During hydrolysis at elevated temperatures, certain undesired byproducts were also generated, such as degradation products
of solubilized sugars and lignin, which are potential inhibitors of microbial metabolism. These compounds were, however, successfully
removed from the hydrolysate by treatment with activated char. 相似文献
70.