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411.
将太原东山新沟垃圾填埋场矿化垃圾筛分为900~300μm、300~150μm、150~105μm、105~90μm和90~0μm共5个不同粒径范围,制备浸出液。在分析不同粒径矿化垃圾浸出液的理化指标基础上,研究了矿化垃圾浸出液对大麦和斑马鱼胚胎生长发育的影响。结果显示,矿化垃圾浸出液p H值随粒径的减小而减小,电导率、CODCr、全盐量和总氮则随粒径的减小而增大。矿化垃圾浸出液对大麦的萌发、根长和芽长均表现出抑制作用,且抑制作用随粒径的减小而显著增加,90~0μm抑制作用最强,具体表现为染毒1 d、2 d和3 d后,大麦种子处理组萌发率为对照组的39.74%、56.38%和59.81%;染毒3 d、5 d和7 d后,根长分别为对照组的57.08%、48.33%和41.66%;芽长分别为对照组的66.60%、64.79%和61.65%。斑马鱼胚胎暴露于不同粒径的矿化垃圾浸出液中,胚胎生长发育的毒害作用与粒径大小呈现明显负相关关系,即在最小粒径90~0μm处理后,卵凝结、血循环异常、孵化率、心包水肿及脊柱畸形影响作用达到最大,这5个指标值分别为40.28%、50.00%、51.39%、31.94%和29.17%。以上研究表明,矿化垃圾浸出液对大麦和斑马鱼胚胎生长发育的毒性效应与矿化垃圾粒径分布显著相关,小粒径矿化垃圾(90~0μm)的生态毒性效应最大。 相似文献
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We investigated the efficiency and kinetics of the degradation of soluble dyes over the p H range 5.0–9.0 using a method employing microwave radiation in combination with nanoscale zero-valent iron(MW–n ZVI). The n ZVI particles(40–70 nm in diameter) were prepared by a liquid-phase chemical reduction method employing starch as a dispersant.Compared to the removal of Solvent Blue 36 and Reactive Yellow K-RN using only n ZVI,more rapid and efficient dye removal and total organic carbon removal were achieved using MW–n ZVI. The dye removal efficiency increased significantly with decreasing p H, but was negligibly affected by variation in the microwave power. The kinetics of dye removal by MW–n ZVI followed both an empirical equation and the pseudo first-order model, while the kinetics of dye removal using n ZVI could only be described by an empirical equation. It was also concluded that microwave heating of the dye solutions as well as acceleration of corrosion of n ZVI and consumption of Fe(II) were possible reasons behind the enhanced dye degradation. 相似文献
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Xue Fei Xi Lei Wang Jia Jun Hu Yu Shu Tang Yu Hu Xiao Hua Fu Ying Sun Yiu Fai Tsang Yan Nan Zhang Jin Hai Chen 《环境科学学报(英文版)》2014,26(12):2562-2570
Estuarine wetland, where freshwater mixes with salt water, comprises different regions(rivers and marine ecosystems) with significantly varying tidal salinities. Two sampling areas, ZXS and JS, were selected to investigate the effect of tidal salinity on soil respiration(SR). ZXS and JS were located in Zhongxia Shoal and Jiangyanan Shoal of Jiuduansha Wetland respectively, with similar elevation and plant species, but significantly different in salinity. The results showed that with almost identical plant biomass, the SR and soil microbial respiration(SMR) of the tidal wetland with lower salinity(JS) were significantly higher than those of the tidal wetland with higher salinity(ZXS)(p 〈 0.05). However, unlike SMR and SR, the difference in the soil microbial biomass(SMB) was not significant(p 〉 0.05)with the SMB of ZXS a little higher than that of JS. The higher SMR and SR of JS may be closely connected to the soil microbial community structures and amount of dominant bacteria. Abundant β- and γ-Proteobacteria and Actinobacteria in JS soil, which have strong heterotrophic metabolic capabilities, could be the main reason for higher SMR and SR,whereas a high number of ε-Proteobacteria in ZXS, some of which have carbon fixation ability, could be responsible for relatively lower carbon output. Path analysis indicated that soil salinity had the maximum negative total influencing coefficient with SMR among the various soil physical and chemical factors, suggesting that higher soil salinity, restricting highly heterotrophic bacteria, is the principle reason for lower SMR and SR in the ZXS. 相似文献
416.
本文以贵州省普定县陈旗喀斯特泉流量为研究对象,采用相关分析和谱分析方法,分析降雨-出口泉流量的响应特征,统计结果表明,该喀斯特流域出口处泉流量对降雨表现出三种响应滞时,分别为短时段、中等时段和长时段响应。对应的响应滞时长度分别为2~4 h、47~49 h和176~290 h。对比流域山坡上部和坡脚两处降雨-泉流量响应特征,结合野外水文地质调查与实验,分析了表层岩溶带发育厚度、多重裂隙渗透性等水文地质条件对降雨-泉流量响应特征的影响机制。山坡上部表层岩溶带厚度较薄,且表层裂隙更为发育,导致山坡上部泉对降雨的响应更迅速,各时段滞时均小于全流域对应时段滞时。 相似文献
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Bo Yao Lingxi Zhou Lingjun Xi Gen Zhang Lifeng Guo Zhao Liu Shuangxi Fang 《环境科学学报(英文版)》2014,26(12):2451-2458
We present in-situ measurements of atmospheric sulfur hexafluoride(SF6) conducted by an automated gas chromatograph–electron capture detector system and a gas chromatography/mass spectrometry system at a regional background site, Shangdianzi,in China, from June 2009 to May 2011, using the System for Observation of Greenhouse gases in Europe and Asia and Advanced Global Atmospheric Gases Experiment(AGAGE)techniques. The mean background and polluted mixing ratios for SF6 during the study period were 7.22 × 10-12(mol/mol, hereinafter) and 8.66 × 10-12, respectively. The averaged SF6 background mixing ratios at Shangdianzi were consistent with those obtained at other AGAGE stations located at similar latitudes(Trinidad Head and Mace Head), but larger than AGAGE stations in the Southern Hemisphere(Cape Grim and Cape Matatula). SF6 background mixing ratios increased rapidly during our study period, with a positive growth rate at 0.30 × 10-12year-1. The peak to peak amplitude of the seasonal cycle for SF6 background conditions was 0.07 × 10-12, while the seasonal fluctuation of polluted conditions was 2.16 × 10-12. During the study period, peak values of SF6 mixing ratios occurred in autumn when local surface horizontal winds originated from W/WSW/SW/SWS/S sectors, while lower levels of SF6 mixing ratios appeared as winds originated from N/NNE/NE/ENE/E sectors. 相似文献