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Humic acid (HA) and fulvic acid (FA) extracted from landfills at different landfill ages were characterized by elemental composition, (13)C CP/MAS NMR, and TMAH-Py-GC/MS. The elemental composition analysis revealed high O/C and low H/C ratios in the FA, indicating a high proportion of O-alkyl and carboxylic acids in the FA. The analytical results of (13)C CP/MAS NMR suggested that there were more oxygenated aliphatic carbons and fewer aromatic carbons in FA than in HA. The Py-GC/MS products showed that the HA and FA extracted from the refuse in the landfill were mainly composed of various lignin-derived compounds. Oxidized aromatic acid derivatives originated from the oxidation of side-chains of lignin-like compounds, and this process played a significant role in the process of HA and FA formation in the landfill. All of the results demonstrated that the degree of humification increased with landfill age. 相似文献
144.
Boran WU Dongyang WANG Xiaoli CHAI Fumitake TAKAHASHI Takayuki SHIMAOKA 《Frontiers of Environmental Science & Engineering》2016,10(4):8
Bottom ash is an inevitable by-product from municipal solid waste (MSW) incineration plants. Recycling it as additives for cement production is a promising disposal method. However, the heavy metals and chlorine are the main limiting factors because of the potential environmental risks and corrosion of cement kilns. Therefore, investigating heavy metal and chlorine characteristics of bottom ash is the significant prerequisite of its reuse in cement industries. In this study, a correlative analysis was conducted to evaluate the effect of the MSW components and collection mode on the heavy metal and chlorine characteristics in bottom ash. The chemical speciation of insoluble chlorine was also investigated by synchrotron X-ray diffraction analysis. The results showed that industrial waste was the main source of heavy metals, especially Cr and Pb, in bottom ash. The higher contents of plastics and kitchen waste lead to the higher chlorine level (0.6 wt.%–0.7 wt.%) of the bottom ash. The insoluble chlorine in the MSW incineration bottom ash existed primarily as AlOCl, which was produced under the high temperature (1250°C) in incinerators.
相似文献
145.
Chai Minwei Li Ruili Tam Nora Fung Yee Zan Qijie 《Environmental geochemistry and health》2019,41(1):175-189
Environmental Geochemistry and Health - The present study compared accumulation of heavy metals in a mangrove swamp dominated by Kandelia obovata with that by Sonneratia apetala in Pearl River... 相似文献
146.
Zhang Min Shan Shengdao Chen Yonggen Wang Fang Yang Deyi Ren Jikai Lu Haoyu Ping Lifeng Chai Yanjun 《Environmental geochemistry and health》2019,41(1):43-52
Environmental Geochemistry and Health - Cadmium (Cd)-contaminated rice (Oryza sativa) in Southern China is a great threat to food security, and the paddy soil remediation is urgently needed to... 相似文献
147.
柴豫申 《安全.健康和环境》2010,10(6):32-33
近年来,随着高含硫原油加工量的增多,石油化工企业硫化氢中毒事故频发,引起了整个行业的高度重视。针对硫化氢的应急防范,各企业不断加大投入,配置报警仪、防护器具,细化应急预案和管理规定。但在实施过程中也产生了许多误区,本文对几个带有普遍性的问题逐一分析,并提出整改建议。 相似文献
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利用一株新分离Cr(Ⅵ)还原菌Leucobacter spp. Ch1进行高浓度Cr(Ⅵ)还原的研究.发现生长于Luria Broth培养基中的Leucobacter spp. Ch1最大能还原1800mg/LCr(Ⅵ),而休眠Leucobacter spp. Ch1细胞悬液可以完全还原2100mg/L Cr(Ⅵ).扫描电镜观察到还原cr(Ⅵ)后的细菌末端黏附大团反应产物,电子顺磁共振分析确定产物的成分为Cr(Ⅲ).在分批加Cr(Ⅵ)还原实验中,休眠Leucobacter spp. Ch1细胞悬液在1060min内还原了2368mg/L Cr(Ⅵ),重新加入的乳酸钠可以再次启动Cr(Ⅵ)的生物还原.结果表明,乳酸钠的存在是Leucobacter spp. Ch1还原Cr(Ⅵ)的必要条件,推测该物质在反应中起电子供体的作用. 相似文献
150.
氧化镁湿法烟气脱硫回收工艺的技术经济可行性初步分析 总被引:5,自引:0,他引:5
介绍了回收结晶硫酸镁的氧化镁湿法烟气脱硫工艺的基本工艺流程,在抛弃法脱硫系统上所作的工业试验证明了吸收液循环提浓MgSO4的可行性。参照工业硫酸镁生产工艺对130t/h燃煤锅炉烟气脱硫作了回收工艺的投资效益分析和整体工艺的经济性评价,结果表明回收工业硫酸镁具有良好的经济效益。 相似文献