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81.
Evaluation of mercury speciation and removal through air pollution control
devices of a 190 MW boiler 总被引:1,自引:0,他引:1
Chengli Wu Yan Cao Zhongbing Dong Chinmin Cheng Hanxu Li Weiping Pan 《环境科学学报(英文版)》2010,22(2):277-282
Air pollution control devices (APCDs) are installed at coal-fired power plants for air pollutant regulation. Selective catalytic reduction
(SCR) and wet flue gas desulfurization (FGD) systems have the co-benefits of air pollutant and mercury removal. Configuration
and operational conditions of APCDs and mercury speciation a ect mercury removal e ciently at coal-fired utilities. The Ontario
Hydro Method (OHM) recommended by the U.S. Environmental Protection Agency (EPA) was used to determine mercury speciation
simultaneously at five sampling locations through SCR-ESP-FGD at a 190 MW unit. Chlorine in coal had been suggested as a factor
a ecting the mercury speciation in flue gas; and low-chlorine coal was purported to produce less oxidized mercury (Hg2+) and more
elemental mercury (Hg0) at the SCR inlet compared to higher chlorine coal. SCR could oxidize elemental mercury into oxidized
mercury when SCR was in service, and oxidation e ciency reached 71.0%. Therefore, oxidized mercury removal e ciency was
enhanced through a wet FGD system. In the non-ozone season, about 89.5%–96.8% of oxidized mercury was controlled, but only
54.9%–68.8% of the total mercury was captured through wet FGD. Oxidized mercury removal e ciency was 95.9%–98.0%, and there
was a big di erence in the total mercury removal e ciencies from 78.0% to 90.2% in the ozone season. Mercury mass balance was
evaluated to validate reliability of OHM testing data, and the ratio of mercury input in the coal to mercury output at the stack was from
0.84 to 1.08. 相似文献
82.
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84.
通过参观学习提高自身认识,拓思路,产生构想,为做好本职工作奠定了基础,增强了信心。 相似文献
85.
Fengzu Zhang Sufang Fan Shaowen Liu Xuesheng Li Canping Pan 《Environmental monitoring and assessment》2013,185(11):9101-9109
A modified LC-MS method for the analysis of mepiquat residue in wheat, potato, and soil was developed and validated. A hydrophilic interaction liquid chromatographic column has been successfully used to retain and separate the mepiquat. Mepiquat residue dynamics and final residues in supervised field trials at Good Agricultural Practice (GAP) conditions in wheat, potato, and soil were studied. The limits of quantification for mepiquat in all samples were all 0.007 mg kg?1, which were lower than their maximum residue limits. At fortification levels of 0.04, 0.2, and 2 mg kg?1 in all samples, recoveries ranged from 77.5 to 116.4 % with relative standard deviations of 0.4–7.9 % (n?=?5). The dissipation half-lives (T 1/2) of mepiquat in soil (wheat), wheat plants, soil (potato), and potato plants were 4.5–6.3, 3.0–5.6, 2.2–4.6, and 2.4–3.2 days, respectively. The final residues of mepiquat were below 0.153 mg kg?1 in soil (wheat), 0.052–1.900 mg kg?1 in wheat, below 0.072 mg kg?1 in soil (potato), and below 1.173 mg kg?1 in potato at harvest time. Moreover, pesticide risk assessment for all the detected residues was conducted. A maximum 0.0012 % of acceptable daily intake (150 mg kg?1) for national estimated daily intake indicated low dietary risk of these products. 相似文献
86.
用于船舶防污漆和农作物杀菌剂的三苯基锡(TPT)对淡水生态环境具有潜在的危害.用1 ~6 μgSn/L的TPT对热带爪蟾(Xenopus tropicalis)胚胎从NF11/12阶段开始进行72h暴露.结果表明,6μgSn/L暴露组胚胎的存活率比对照组降低了83%,3.5 μgSn/L及以上质量浓度的TPT暴露使胚胎的体长减少16%~35%,2.25μgSn/L及以上质量浓度暴露组胚胎的总畸形率均达100%.畸形现象主要包括眼睛异常,躯干拉长,泄殖腔突出,鳍变窄或消失,尾巴弯曲和皮肤色素减少等.在所有畸形表型中,TPT对鳍的影响最突出.暴露组胚胎的尾鳍宽度比对照组减少了17% ~ 100%,并呈现明显的剂量效应关系.因此,TPT能抑制热带爪蟾胚胎的生长,并具有极强的致畸性,能特异性地阻碍爪蟾鳍的形成. 相似文献
87.
Chen B Pan Y Wang J Fu Z Zhang Y Zhou Y 《Environmental monitoring and assessment》2012,184(6):3545-3556
Evenly distributed sampling design is generally considered as an efficient sampling design. It is widely used in sampling
for the environmental survey. In this paper, we present a novel method for generating N evenly distributed samples within a given irregular polygon via simulating the movements of some ideal homogeneous point
charges. Initially, charges are randomly put into the sampling region; then, they are freed and held orderly; and after enough
runs, the charges will finally reach a stable state with all of them having a zero resultant force and velocity; and so they
distribute evenly within the region. Their layout can thus be considered as an evenly distributed sampling design. The main
advantages of this method are: (1) it is easy to understand and implement; (2) it is efficient in both running and generating
better designs. Analysis and experimental results indicate that this method is an efficient and robust method for generating
even sampling designs for 2D polygonal sampling region. 相似文献
88.
89.
酸性洗涤塔-生物滤塔-生物曝气池组合工艺处理恶臭气体NH3和H2S 总被引:1,自引:0,他引:1
采用酸性洗涤塔、生物滤塔和生物曝气池的组合工艺处理NH3、H2S恶臭混合气体,研究表明,该组合工艺对NH3和H2S有很好的去除效果,在进气流量为35 L/min,喷淋量45 L/h时,NH3进气浓度50.15~525.4 mg/m3,H2S进气浓度10.23~110.36 mg/m3时,NH3单一进气去除率稳定在99%以上,H2S单一进气去除率90%以上。混合进气后,NH3去除率几乎为100%,H2S的去除率提高至98%以上。在一定的浓度范围内,NH3和H2S之间的相互作用对两者的去除效果没有明显的影响,而且起到了相互促进降解的作用。同时,进气流量和填料层高度都会影响NH3、H2S的去除率。系统对进气容积负荷变化的缓冲能力强,在偶尔超负荷条件下运行并不能使系统崩溃,并且微生物对高负荷逐渐表现出适应性。大部分溶于水的氨由生物曝气池去除,去除率达到96.9%。 相似文献
90.
通过静态动力学和热力学吸附实验,研究了温度、共存离子以及溶质的初始浓度对As(V)在金红石TiO2颗粒表面吸附的影响,探讨了As(V)在金红石TiO2颗粒表面吸附特性及机理。结果表明,在As(V)初始浓度为10mg/L,pH为7的条件下,25℃时的吸附量0.41mg/g高于30℃时的吸附量0.31mg/g,As(V)在金红石TiO,上的吸附为放热过程。CaCl2和MgCl2的添加对As(V)在金红石TiO2表面吸附起到明显的促进作用。T=25℃,Ca2+或Mg2+浓度为10mmol/L时,As(V)吸附量分别为0.64和0.56mg/g,Ca2+比Mg2+对As(V)吸附促进作用强。As(V)在金红石TiO2的吸附等温线符合Frendlich方程,Lagergren二级动力学方程能较好地描述As(V)在金红石TiO2颗粒表面吸附的动力学过程。 相似文献