全文获取类型
收费全文 | 6828篇 |
免费 | 150篇 |
国内免费 | 76篇 |
专业分类
安全科学 | 313篇 |
废物处理 | 228篇 |
环保管理 | 1407篇 |
综合类 | 843篇 |
基础理论 | 1799篇 |
环境理论 | 11篇 |
污染及防治 | 1629篇 |
评价与监测 | 462篇 |
社会与环境 | 303篇 |
灾害及防治 | 59篇 |
出版年
2023年 | 72篇 |
2022年 | 101篇 |
2021年 | 100篇 |
2020年 | 85篇 |
2019年 | 96篇 |
2018年 | 226篇 |
2017年 | 214篇 |
2016年 | 311篇 |
2015年 | 188篇 |
2014年 | 262篇 |
2013年 | 549篇 |
2012年 | 350篇 |
2011年 | 459篇 |
2010年 | 288篇 |
2009年 | 319篇 |
2008年 | 377篇 |
2007年 | 362篇 |
2006年 | 317篇 |
2005年 | 254篇 |
2004年 | 250篇 |
2003年 | 193篇 |
2002年 | 178篇 |
2001年 | 114篇 |
2000年 | 112篇 |
1999年 | 80篇 |
1998年 | 79篇 |
1997年 | 68篇 |
1996年 | 72篇 |
1995年 | 87篇 |
1994年 | 82篇 |
1993年 | 76篇 |
1992年 | 63篇 |
1991年 | 46篇 |
1990年 | 40篇 |
1989年 | 39篇 |
1988年 | 36篇 |
1987年 | 41篇 |
1986年 | 42篇 |
1985年 | 42篇 |
1984年 | 47篇 |
1983年 | 47篇 |
1982年 | 55篇 |
1981年 | 46篇 |
1980年 | 37篇 |
1979年 | 15篇 |
1978年 | 29篇 |
1977年 | 19篇 |
1976年 | 15篇 |
1972年 | 8篇 |
1971年 | 9篇 |
排序方式: 共有7054条查询结果,搜索用时 31 毫秒
191.
Thomassen Y Koch W Dunkhorst W Ellingsen DG Skaugset NP Jordbekken L Arne Drabløs P Weinbruch S 《Journal of environmental monitoring : JEM》2006,8(1):127-133
The number concentration and size distribution of ultrafine particles in a S?derberg and a prebake potroom of an aluminium primary smelter have been measured using a scanning mobility particle spectrometer. The particle morphology was studied by transmission electron microscopy (TEM). The study shows the existence of elevated number concentrations of ultrafine particles in both potrooms. The main source of these particles is likely to be the process of anode changing. The ultrafine particles were measured directly at the source but could also be identified as episodes of high number concentrations in the general background air. Unlike the larger particles belonging to the 50-100 nm mode, the nanoparticle mode could not be detected in the TEM indicating that they may not be stable under the applied sampling conditions and/or the high vacuum in the instrument. 相似文献
192.
Bioaerosol sampling by a personal rotating cup sampler CIP 10-M 总被引:1,自引:0,他引:1
Görner P Fabriès JF Duquenne P Witschger O Wrobel R 《Journal of environmental monitoring : JEM》2006,8(1):43-48
High concentrations of bioaerosols containing bacterial, fungal and biotoxinic matter are encountered in many workplaces, e.g. solid waste treatment plants, waste water treatment plants and sewage networks. A personal bioaerosol sampler, the CIP 10-M (M-microbiologic), has been developed to measure worker exposure to airborne biological agents. This sampler is battery operated; it is light and easy to wear and offers full work shift autonomy. It can sample much higher concentrations than biological impactors and limits the mechanical stress on the microorganisms. Biological particles are collected in 2 ml of liquid medium inside a rotating cup fitted with radial vanes to maintain an air flow rate of 10 l min(-1) at a rotational speed of approximately 7,000 rpm. The rotating cup is made of sterilisable material. The sampled particles follow a helicoidal trajectory as they are pushed to the surface of the liquid by centrifugal force, which creates a thin vertical liquid layer. Sterile water or another collecting liquid can be used. Three particle size selectors allow health-related aerosol fractions to be sampled according to international conventions. The sampled microbiological particles can be easily recovered for counting, incubation or further biochemical analysis, e.g., for airborne endotoxins. Its physical sampling efficiency was laboratory tested and field trials were carried out in industrial waste management conditions. The results indicate satisfactory collection efficiency, whilst experimental application has demonstrated the usefulness of the CIP 10-M personal sampler for individual bioaerosol exposure monitoring. 相似文献
193.
Trace Element Concentrations and Bioindicator Responses in Tree Swallows from Northwestern Minnesota 总被引:5,自引:0,他引:5
Custer CM Custer TW Warburton D Hoffman DJ Bickham JW Matson CW 《Environmental monitoring and assessment》2006,118(1-3):247-266
Extremely high concentrations of cadmium (3.5 μg/g dry wgt.) and elevated concentrations of chromium (>10 μg/g dry wgt.) and mercury (1.6 μg/g dry wgt.) were reported in waterbird tissues at Agassiz National Wildlife Refuge in northwestern Minnesota in 1994. Tree
swallows (Tachycineta bicolor) were studied during 1998–2001 at three drainages into the Refuge, two pools on the Refuge, and at a nearby reference location
to document whether high levels of contaminants were still present, and if so to quantify the source and severity of the contamination.
Trace elements were measured in tree swallow eggs, livers, and diet. Reproductive success and bioindicator responses were
monitored. In 2000, water was drawn down on Agassiz Pool, one of the main pools on the Refuge. This presented an opportunity
to evaluate the response of trace element concentrations in the diet and tissues of tree swallows after reflooding. High concentrations
of trace elements were not detected in swallow tissues, nor were there differences among locations. Less than 20% of swallow
samples had detectable concentrations of cadmium or chromium. Mercury concentrations were low and averaged <0.25 μg/g dry wgt. in swallow tissues. Trace elements, including mercury, did not increase in tree swallows following the 2000 drawdown
at Agassiz Pool. Hatching success and survival of nestlings to 12 days-of-age for tree swallows on the Refuge were similar
to the national average and consistent with background trace element concentrations. Bioindicator measurements were within
the normal ranges as well. 相似文献
194.
Weyer PJ Smith BJ Feng ZF Kantamneni JR Riley DG 《Environmental monitoring and assessment》2006,116(1-3):81-90
Nitrate contamination of water sources is a concern where large amounts of nitrogen fertilizers are regularly applied to soils.
Ingested nitrate from dietary sources and drinking water can be converted to nitrite and ultimately to N-nitroso compounds,
many of which are known carcinogens. Epidemiologic studies of drinking water nitrate and cancer report mixed findings; a criticism
is the use of nitrate concentrations from retrospective drinking water data to assign exposure levels. Residential point-of-use
nitrate data are scarce; gaps in historical data for municipal supply finished water hamper exposure classification efforts.
We used generalized linear regression models to estimate and compare historical raw water and finished water nitrate levels
(1960s--1990s) in single source Iowa municipal supplies to determine whether raw water monitoring data could supplement finished
water data to improve exposure assessment. Comparison of raw water and finished water samples (same sampling date) showed
a significant difference in nitrate levels in municipalities using rivers; municipalities using other surface water or alluvial
groundwater had no difference in nitrate levels. A regional aggregation of alluvial groundwater municipalities was constructed
based on results from a previous study showing regional differences in nitrate contamination of private wells; results from
this analysis were mixed, dependent upon region and decade. These analyses demonstrate using historical raw water nitrate
monitoring data to supplement finished water data for exposure assessment is appropriate for individual Iowa municipal supplies
using alluvial groundwater, lakes or reservoirs. Using alluvial raw water data on a regional basis is dependent on region
and decade. 相似文献
195.
Rhea DT Harper DD Farag AM Brumbaugh WG 《Environmental monitoring and assessment》2006,115(1-3):381-393
Portions of the Boulder River watershed contain elevated concentrations of arsenic, cadmium, copper, lead, and zinc in water, sediment, and biota. We measured concentrations of As, Cd, Cu, Pb, and Zn in biofilm and macroinvertebrates, and assessed macroinvertebrate assemblage and aquatic habitat with the objective of monitoring planned remediation efforts. Concentrations of metals were generally higher in downstream sites compared with upstream or reference sites, and two sites contained metal concentrations in macroinvertebrates greater than values reported to reduce health and survival of resident trout. Macroinvertebrate assemblage was correlated with metal concentrations in biofilm and macroinvertebrates. However, macroinvertebrate metrics were significantly correlated with a greater number of biofilm metals (8) than metals in invertebrates (4). Lead concentrations in biofilm appeared to have the most significant impact on macroinvertebrate assemblage. Metal concentrations in macroinvertebrates were directly proportional to concentrations in biofilm, indicating biofilm as a potential surrogate for monitoring metal impacts in aquatic systems. 相似文献
196.
Christian Mrz Felipe S. Freitas Johan C. Faust Jasmin A. Godbold Sian F. Henley Allyson C. Tessin Geoffrey D. Abbott Ruth Airs Sandra Arndt David K. A. Barnes Laura J. Grange Neil D. Gray Ian M. Head Katharine R. Hendry Robert G. Hilton Adam J. Reed Saskia Rühl Martin Solan Terri A. Souster Mark A. Stevenson Karen Tait James Ward Stephen Widdicombe 《Ambio》2022,51(2):370
Unprecedented and dramatic transformations are occurring in the Arctic in response to climate change, but academic, public, and political discourse has disproportionately focussed on the most visible and direct aspects of change, including sea ice melt, permafrost thaw, the fate of charismatic megafauna, and the expansion of fisheries. Such narratives disregard the importance of less visible and indirect processes and, in particular, miss the substantive contribution of the shelf seafloor in regulating nutrients and sequestering carbon. Here, we summarise the biogeochemical functioning of the Arctic shelf seafloor before considering how climate change and regional adjustments to human activities may alter its biogeochemical and ecological dynamics, including ecosystem function, carbon burial, or nutrient recycling. We highlight the importance of the Arctic benthic system in mitigating climatic and anthropogenic change and, with a focus on the Barents Sea, offer some observations and our perspectives on future management and policy. 相似文献
197.
Chile ratified the Montreal Protocol in 1990 which sets out an agenda for the reduction and then elimination of ozone depleting substances (ODS); however, by 1998 the country had not yet defined a strategy to encourage greater compliance, so that in the same year the National Environmental Commission decided to examine the policy options available. This paper examines the process followed to develop this strategy. As a first step it was necessary to look at how far the implicit policy of "business as usual" could be stretched without jeopardizing Chile's compliance obligations. A second step included quantifying compliance costs and their impact on different policy instruments and so policy choice. Finally, the attitudes of decision-makers or participants were identified, by interviews with officials of the different public agents involved, in order to weigh their views about policy. A strategy was proposed, based on this information, which the Chilean regulator has used, although not in its entirety. The methodology developed could well be useful for developing-country Protocol signatories building their own appropriate compliance strategy. 相似文献
198.
A Regional Classification Scheme for Estimating Reference Water Quality in Streams Using Land-Use-Adjusted Spatial Regression-Tree Analysis 总被引:1,自引:0,他引:1
Various approaches are used to subdivide large areas into regions containing streams that have similar reference or background
water quality and that respond similarly to different factors. For many applications, such as establishing reference conditions,
it is preferable to use physical characteristics that are not affected by human activities to delineate these regions. However,
most approaches, such as ecoregion classifications, rely on land use to delineate regions or have difficulties compensating
for the effects of land use. Land use not only directly affects water quality, but it is often correlated with the factors
used to define the regions. In this article, we describe modifications to SPARTA (spatial regression-tree analysis), a relatively
new approach applied to water-quality and environmental characteristic data to delineate zones with similar factors affecting
water quality. In this modified approach, land-use-adjusted (residualized) water quality and environmental characteristics
are computed for each site. Regression-tree analysis is applied to the residualized data to determine the most statistically
important environmental characteristics describing the distribution of a specific water-quality constituent. Geographic information
for small basins throughout the study area is then used to subdivide the area into relatively homogeneous environmental water-quality
zones. For each zone, commonly used approaches are subsequently used to define its reference water quality and how its water
quality responds to changes in land use. SPARTA is used to delineate zones of similar reference concentrations of total phosphorus
and suspended sediment throughout the upper Midwestern part of the United States. 相似文献
199.
Long-term water quality records for assessing natural variability, impact of management, and that guide regulatory processes to safeguard water resources are rare for California oak woodland rangelands. This study presents a 20-yr record (1981-2000) of nitrate-nitrogen (NO(3)-N) and suspended sediment export from a typical, grazed oak woodland watershed (103 ha) in the northern Sierra Nevada foothills of California. Mean annual precipitation over the 20-yr period was 734 mm yr(-1) (range 366-1205 mm yr(-1)). Mean annual stream flow was 353 mm y(-1) (range 87-848 mm yr(-1)). Average annual stream flow was 48.1 +/- 16% of precipitation. Mean annual NO(3)-N export was 1.6 kg ha(-1) yr(-1) (range 0.18-3.6 kg ha(-1) yr(-1)). Annual NO(3)-N export significantly (P < 0.05) increased with increasing annual stream flow and precipitation. Mean daily NO(3)-N export was 0.004 kg ha(-1) d(-1) (range 10(-5) to 0.55 kg ha(-1) d(-1)). Mean annual suspended sediment export was 198 kg ha(-1) yr(-1) (range 23-479 kg ha(-1) yr(-1)). There was a positive relationship (P < 0.05) between annual suspended sediment export, annual stream flow and precipitation. Mean daily suspended sediment export was 0.54 kg ha(-1) d(-1) (range 10(-4) to 155 kg ha(-1) d(-1)). Virtually no sediment was exported during the dry season. The large variation in daily and annual fluxes highlights the necessity of using long-term records to establish quantitative water quality targets for rangelands and demonstrates the difficulty of designing a water quality monitoring program for these ecosystems. 相似文献
200.
Wu Y Lerner DN Banwart SA Thornton SF Pickup RW 《Journal of environmental quality》2006,35(6):2021-2025
The fermentation process is an important component in the biodegradation of organic compounds in natural and contaminated systems. Comparing with terminal electron-accepting processes (TEAPs), however, research on fermentation processes has to some extent been ignored in the past decades, particularly on the persistence of fermentation process in the presence of toxic organic pollutants. Both field and laboratory studies, presented here, showed that microbial processes in a groundwater-based system exhibited a differential inhibitory response to toxicity of phenolic compounds from coal tar distillation, thus resulting in the accumulation of volatile fatty acids (VFAs) and hydrogen. This indicated that fermentation processes could be more resistant to phenol toxicity than the subsequent TEAPs such as methanogenesis and sulfate reduction, thus providing us with more options for enhancing bioremediation processes. 相似文献