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941.
生物炭因具有较大的孔隙度、比表面积以及较强的吸附能力等优点,在环境污染修复、土壤改良和固碳方面应用广泛.由于大多数生物炭表面带有负电荷,而土壤中的无机砷主要以砷酸盐和亚砷酸盐等阴离子形式存在.因此,生物炭对砷的吸附效率通常较低,需要对生物炭进行改性以提升其对砷的吸附效果.零价铁和氧化铁等铁基材料对砷吸附能力强且来源广泛,通过沉淀法、热解法、球磨法和微生物法等方法将铁基材料与生物炭负载形成铁修饰生物炭,可将二者的优良特性相结合,拓展生物炭材料在环境修复中的应用.在对近年来有关铁修饰生物炭的文献进行系统分析的基础上,综述了常见的铁修饰生物炭的制备方法,比较分析了生物炭基底、铁修饰材料以及两者对砷的协同作用机制,并简要阐述了铁修饰生物炭在土壤污染修复中的应用现状,最后对铁修饰生物炭的未来研究方向提出了展望. 相似文献
942.
近年来,许多学者利用现场地震监测或数值试验来研究斜坡的地震响应,然而不同斜坡往往存在不同类型的地貌单元,其动力响应机制往往也存在很大差异。本文依托海原大地震区域,基于室内试验、现场波速测试等方法,运用有限元数值模拟技术对海原大地震影响范围内不同地貌单元的斜坡的动力响应进行了研究。结果表明:黄土塬具有高程放大效应,在同一高程水平面上,且距坡面一定范围内时越趋近坡面斜坡动力放大系数(peak ground acceleration amplification coefficient,PGA放大系数)越大;对比不同类型的地貌单元,地层结构相同的斜坡其响应规律一致,但在古土壤层其PGA放大效应会减弱。模型分析较好地揭示了人工合成地震波作用下黄土高原斜坡的动力放大效应,可为不同地貌单元地震诱发的地质灾害的风险评价和防灾减灾提供有益的借鉴与参考。 相似文献
943.
Jianfeng Zhang Shichang Wei Zhenxing Liu Huang Tang Xiaoguang Meng Weihuang Zhu 《环境科学学报(英文版)》2022,34(8):67-75
In this study, Pb(II) was used as a target heavy metal pollutant, and the metabolism of Shewanella putrefaciens (S. putrefaciens) was applied to achieve reducing conditions to study the effect of microbial reduction on lead that was preadsorbed on graphene oxide (GO) surfaces. The results showed that GO was transformed to its reduced form (r-GO) by bacteria, and this process induced the release of Pb(II) adsorbed on the GO surfaces. After 72 hr of exposure in an S. putrefaciens system, 5.76% of the total adsorbed Pb(II) was stably dispersed in solution in the form of a Pb(II)-extracellular polymer substance (EPS) complex, while another portion of Pb(II) released from GO-Pb(II) was observed as lead phosphate hydroxide (Pb10(PO4)6(OH)2) precipitates or adsorbed species on the surface of the cell. Additionally, increasing pH induced the stripping of oxidative debris (OD) and elevated the content of dispersible Pb(II) in aqueous solution under the conditions of S. putrefaciens metabolism. These research results provide valuable information regarding the migration of heavy metals adsorbed on GO under reducing conditions due to microbial metabolism. 相似文献
944.
Sulfur deposition simulations over China, Japan, and Korea: a model intercomparison study for abating sulfur emission 总被引:1,自引:1,他引:0
Cheol-Hee Kim Lim-Seok Chang Fan Meng Mizuo Kajino Hiromasa Ueda Yuanhang Zhang Hye-Young Son Jong-Jae Lee Youjiang He Jun Xu Keiichi Sato Tatsuya Sakurai Zhiwei Han Lei Duan Jeong-Soo Kim Suk-Jo Lee Chang-Keun Song Soo-Jin Ban Shang-Gyoo Shim Young Sunwoo Tae-Young Lee 《Environmental science and pollution research international》2012,19(9):4073-4089
In response to increasing trends in sulfur deposition in Northeast Asia, three countries in the region (China, Japan, and Korea) agreed to devise abatement strategies. The concepts of critical loads and source?Creceptor (S?CR) relationships provide guidance for formulating such strategies. Based on the Long-range Transboundary Air Pollutants in Northeast Asia (LTP) project, this study analyzes sulfur deposition data in order to optimize acidic loads over the three countries. The three groups involved in this study carried out a full year (2002) of sulfur deposition modeling over the geographic region spanning the three countries, using three air quality models: MM5-CMAQ, MM5-RAQM, and RAMS-CADM, employed by Chinese, Japanese, and Korean modeling groups, respectively. Each model employed its own meteorological numerical model and model parameters. Only the emission rates for SO2 and NOx obtained from the LTP project were the common parameter used in the three models. Three models revealed some bias from dry to wet deposition, particularly the latter because of the bias in annual precipitation. This finding points to the need for further sensitivity tests of the wet removal rates in association with underlying cloud?Cprecipitation physics and parameterizations. Despite this bias, the annual total (dry plus wet) sulfur deposition predicted by the models were surprisingly very similar. The ensemble average annual total deposition was 7,203.6?±?370 kt S with a minimal mean fractional error (MFE) of 8.95?±?5.24?% and a pattern correlation (PC) of 0.89?C0.93 between the models. This exercise revealed that despite rather poor error scores in comparison with observations, these consistent total deposition values across the three models, based on LTP group's input data assumptions, suggest a plausible S?CR relationship that can be applied to the next task of designing cost-effective emission abatement strategies. 相似文献
945.
Wang Jiajun Meng Xiaoqing Chen Yu Zheng Guanyu Zhou Lixiang 《Environmental science and pollution research international》2021,28(11):13300-13311
Environmental Science and Pollution Research - Fenton conditioning processes have been recently employed to improve the dewaterability of sewage sludge. However, it remains unclear whether the... 相似文献
946.
Shanshan Zhao Zhu Tao Liwei Chen Muqiao Han Bin Zhao Xuelin Tian Liang Wang Fangang Meng 《Frontiers of Environmental Science & Engineering》2021,15(4):63
947.
Mu Yunsong Shao Meichen Zhong Buqing Zhao Yiqun Leung Kenneth M. Y. Giesy John P. Ma Jin Wu Fengchang Zeng Fangang 《Environmental science and pollution research international》2021,28(28):37051-37059
Environmental Science and Pollution Research - The coronavirus disease 2019 (COVID-19) pandemic has brought unprecedented public health, and social and economic challenges. It remains unclear... 相似文献
948.
排污许可制度改革是我国"十三五"期间一项重大内容。宁夏自2017年开始全面推行排污许可制改革,积极推进排污许可证的核发。本文对宁夏排污许可证制度落实情况进行梳理,并从工作机制、证后监管、信息化平台、培育第三方服务等方面提出对策建议。 相似文献
949.
Zhang Bo Yuan Qingbin Wang Meng meng Sun Ruonan Liu Huiling Wang Peng 《Environmental science and pollution research international》2021,28(12):14423-14433
Environmental Science and Pollution Research - Though heavy metals are widely reported to induce antibiotic resistance propagation, how antibiotic resistance changes in response to heavy metal... 相似文献
950.
Meng Qingxin Liu Shuang Guo Yue Hu Yunlong Yu Zhidan Bello Ayodeji Wang Zhigang Xu Weihui Xu Xiuhong 《Environmental science and pollution research international》2023,30(8):20265-20276
Environmental Science and Pollution Research - Microbes often form complex ecological networks in various habitats. Co-occurrence network analysis allows exploring the complex community... 相似文献