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61.
Application of magnetite-activated persulfate oxidation for the degradation of PAHs in contaminated soils 总被引:2,自引:0,他引:2
In this study, feasibility of magnetite-activated persulfate oxidation (AP) was evaluated for the degradation of polycyclic aromatic hydrocarbons (PAHs) in batch slurry system. Persulfate oxidation activated with soluble Fe(II) (FP) or without activation (SP) was also tested. Kinetic oxidation of PAHs was tracked in spiked sand and in aged PAH contaminated soils at circumneutral pH. Quartz sand was spiked with: (i) single model pollutant (fluorenone) and (ii) organic extract isolated from two PAH contaminated soils (H and NM sampled from ancient coking plants) and was subjected to oxidation. Oxidation was also performed on real H and NM soils with and without an extraction pretreatment. Results indicate that oxidation of fluorenone resulted in its complete degradation by AP while abatement was very low (<20%) by SP or FP. In soil extracts spiked on sand, significant degradation of 16 PAHs was observed by AP (70-80%) in 1 week as compared to only 15% by SP or FP systems. But no PAH abatement was observed in real soils whatever the treatment used (AP, FP or SP). Then soils were subjected to an extraction pretreatment but without isolation of organic extract from soil. Oxidation of this pretreated soil showed significant abatement of PAHs by AP. On the other hand, very low degradation was achieved by FP or SP. Selective degradation of PAHs was observed by AP with lower degradation efficiency towards high molecular weight PAHs. Analyses revealed that no by-products were formed during oxidation. The results of this study demonstrate that magnetite can activate persulfate at circumneutral pH for an effective degradation of PAHs in soils. However, availability of PAHs and soil matrix were found to be the most critical factors for degradation efficiency. 相似文献
62.
Thomas R. Hanna Michael J. Pilat 《Journal of the Air & Waste Management Association (1995)》2013,63(7):533-536
Aerosol size distributions were measured in the air exhausted from a horizontal spike Soderberg aluminum reduction cell at the Kaiser Aluminum and Chemical Corporation plant in Tacoma, Wash. The particle size distributions were measured with the University of Washington cascade impactor, developed specifically for source testing. The particle mass concentrations and size distributions were found to vary significantly with changes in the cell process operations. For a typical aerosol size distribution at the exit of the cell hood the mass mean particle diameter was 5.5 microns and the particle size standard geometric deviation was 25. 相似文献
63.
Hanna Eriksson H?gg Steve W. Lyon Teresia W?llstedt Carl-Magnus M?rth Bj?rn Claremar Christoph Humborg 《Ambio》2014,43(3):337-351
Dynamic model simulations of the future climate and projections of future lifestyles within the Baltic Sea Drainage Basin (BSDB) were considered in this study to estimate potential trends in future nutrient loads to the Baltic Sea. Total nitrogen and total phosphorus loads were estimated using a simple proxy based only on human population (to account for nutrient sources) and stream discharges (to account for nutrient transport). This population-discharge proxy provided a good estimate for nutrient loads across the seven sub-basins of the BSDB considered. All climate scenarios considered here produced increased nutrient loads to the Baltic Sea over the next 100 years. There was variation between the climate scenarios such that sub-basin and regional differences were seen in future nutrient runoff depending on the climate model and scenario considered. Regardless, the results of this study indicate that changes in lifestyle brought about through shifts in consumption and population potentially overshadow the climate effects on future nutrient runoff for the entire BSDB. Regionally, however, lifestyle changes appear relatively more important in the southern regions of the BSDB while climatic changes appear more important in the northern regions with regards to future increases in nutrient loads. From a whole-ecosystem management perspective of the BSDB, this implies that implementation of improved and targeted management practices can still bring about improved conditions in the Baltic Sea in the face of a warmer and wetter future climate. 相似文献
64.
Hanna Barchanska Anna Kowalska Barbara Poloczek 《Environmental science and pollution research international》2014,21(6):4751-4758
Simple and effective extraction methods based on matrix solid-phase dispersion (MSPD), dispersive liquid–liquid microextraction (DLLME), and solid-phase extraction (SPE) coupled with high-performance liquid chromatography with diode array detector (HPLC-DAD) were developed to determine triketone herbicides—sulcotrione (SUL), mesotrione (MES), tembotrione (TEMB), and their degradation products—in plant tissues and water samples. The extraction procedures were employed to enable quantification of the accumulation of selected triketone herbicides and their degradation products in a model aquatic plant, Egeria densa. To obtain comprehensive information about the triketones' influence on an aquatic plant, changes in chlorophyll concentration in plants exposed to these triketones were monitored. The average recovery ranged from 58 to 115 % (coefficients of variation 7–12 %) for plant tissues and from 52 to 96 % (coefficients of variation 8–20 %) for water samples. The limit of detection (LOD) for the MSPD–HPLC-DAD procedure was in the range of 0.06–0.23 μg/g, whereas for DLLME–HPLC-DAD and SPE–HPLC-DAD, LOD was in the range of 0.06–0.26 μg/mL. Symptoms of the phytotoxicity of sulcotrione, mesotrione, tembotrione, and their degradation products (decrease of chlorophyll concentration in plant sprouts) were observed for E. densa cultivated in water with herbicide concentrations of 100 μg/L. Moreover, the tembotrione degradation product exhibited a high level of accumulation and low metabolism in plant tissues in comparison to the other triketones and their degradation products. 相似文献
65.
Justyna Maliszewska Joanna Wyszkowska Hanna Kletkiewicz Justyna Rogalska 《Journal of environmental science and health. Part. B》2013,48(8):676-680
AbstractMembers of TRP receptor family are involved in response to acidification. Here, we determined the effect of capsaicin, one of the TRP receptor activators, on hemolymph acid-base status in the American cockroach. Periplaneta americana adult individuals were injected with lactic acid (5% or 10%) and exposed to 100?µM capsaicin solution. Hemolymph pH was measured 15?min, 1, 4, 8 and 24?h after lactic acid and capsaicin application with a glass microelectrode. The results demonstrated that cockroaches recover from acidosis within 4?h from acid injection. Capsaicin impaired the buffering capacity of insects’ hemolymph, resulting in significant drop of hemolymph pH observed even 24?h after application. Joint action of capsaicin and acidosis reveals new insight into possible mechanism of capsaicin action on TRP receptors in insects. 相似文献
66.
67.
Intracerebral tumours of the fetus are very rare conditions, most often presenting clinically as polyhydramnios and hydrocephalus. These conditions can be diagnosed with ultrasound and clearly differentiated from hydrocephalus and other intracranial lesions. The following report is of a case of an intracerebral tumour (glioblastoma multiforme) diagnosed at 33 weeks in utero using ultrasound. The prognosis for this condition is universally poor. 相似文献
68.
Hanna Kokko 《Behavioral ecology and sociobiology》1997,41(2):99-107
In various models of sexual selection mediated by the viability indicator (“good genes”) mechanism, a sexually selected trait
will truly reflect male quality if its expression is costly for the male. However, in long-lived species, the expression of
a trait often increases with age while the genotype of the male remains unchanged. This fact may obscure the indicator mechanism.
Hitherto, game theory models of honesty in sexual advertisement have not taken life-history effects into account, whereas
life-history models of reproductive effort have only seldom considered the dependence of mating success on the actions of
other individuals. Here, the two approaches are combined, and I examine whether honesty is maintained if males can divide
their advertisement effort over their lifetime. The model shows that an increase in the expression of the sexually selected
trait over several years is an evolutionarily stable strategy (ESS) under a wide range of situations, so that a correlated
preference for old age can emerge through a viability indicator mechanism. Honesty in the strict sense is not preserved: an
optimally behaving low-quality male will in some cases advertise more than a high-quality male of equal age, to the extent
that the strongest advertisement found in the population can be associated with a low-quality male. Due to life-history trade-offs,
however, honesty in an average sense holds true over the lifetime of individuals: “cheater” age classes will remain small
enough, that a female will obtain a higher expected mate quality if she trusts in the trait as an indicator of viability.
Received: 25 June 1996 / Accepted after revision: 15 April 1997 相似文献
69.
Marit?StrandenEmail author Tonette?R?stelien Ilme?Liblikas Tor?J.?Almaas Anna-Karin?Borg-Karlson Hanna?Mustaparta 《Chemoecology》2003,13(3):143-154
Summary. Some plant volatiles are produced in response to
herbivory of several insect species, including heliothine
larvae. In the present study of female heliothine moths, four
co-located receptor neurone types were identified, of which
three types responded strongest to the inducible compounds
E--ocimene, E,E--farnesene and E,E-TMTT, respectively.
The fourth type responded strongest to geraniol,
which is a common floral volatile. The narrow tuning of
each receptor neurone type was demonstrated by responses
to a few structurally-related monoterpenes, sesquiterpenes,
homo-terpenes and monoterpene alcohols, respectively, out
of hundreds of plant constituents tested. The four neurone
types showed the same relation of spike amplitudes and
ranking of effective compounds in the three heliothine
species; the polyphagous Heliothis virescens and
Helicoverpa armigera and the oligophagous Helicoverpa
assulta. The results indicate the presence of functionally
similar types of plant odour-receptor neurones in the three
related species, and suggest conservation or reappearance of
functionally similar olfactory receptors in related species,
independent of the evolution of polyphagy and oligophagy. 相似文献
70.
There is genetic variation in the female mating rate in the green-veined white butterfly (Pieris napi), and females benefit from male ejaculates that contain both sperm and accessory gland substances. Although polyandry corresponds to higher lifetime fecundity than monandry, some females abstain from remating irrespective of the number of available mates. Explaining genetic variation in mating rates requires that monandrous females perform better than polyandrous ones under some conditions. We experimentally explored the reproductive performance of females either with a low or high intrinsic mating rate by allowing them to mate, feed, and lay eggs freely in a laboratory. Individual females followed different life histories: during the early days of reproduction, females with a low mating rate produced more eggs than females with a high mating rate. Hence, refraining from the benefits of multiple mating may be beneficial, if the time for reproduction is limited, or other female traits associated with polyandry are traded off against longevity. Given the day length of 10 h, a model shows that even if polyandrous females enjoy higher lifetime reproductive success, changeable and unpredictable weather will favor monandry if each period of suitable weather lasts, on average, less than 5 days. Thus, a combination of life history cost and unpredictability of fitness may explain the maintenance of monandry in the wild. Our results are also consistent with the observation that frequency of monandry increases with latitude. 相似文献