全文获取类型
收费全文 | 241篇 |
免费 | 4篇 |
国内免费 | 1篇 |
专业分类
安全科学 | 10篇 |
废物处理 | 11篇 |
环保管理 | 19篇 |
综合类 | 61篇 |
基础理论 | 73篇 |
环境理论 | 1篇 |
污染及防治 | 50篇 |
评价与监测 | 11篇 |
社会与环境 | 8篇 |
灾害及防治 | 2篇 |
出版年
2022年 | 1篇 |
2021年 | 2篇 |
2020年 | 2篇 |
2019年 | 4篇 |
2018年 | 8篇 |
2017年 | 4篇 |
2016年 | 10篇 |
2015年 | 3篇 |
2014年 | 4篇 |
2013年 | 17篇 |
2012年 | 8篇 |
2011年 | 13篇 |
2010年 | 14篇 |
2009年 | 14篇 |
2008年 | 12篇 |
2007年 | 14篇 |
2006年 | 19篇 |
2005年 | 9篇 |
2004年 | 5篇 |
2003年 | 18篇 |
2002年 | 2篇 |
2001年 | 5篇 |
2000年 | 1篇 |
1999年 | 2篇 |
1998年 | 4篇 |
1996年 | 1篇 |
1995年 | 1篇 |
1994年 | 3篇 |
1993年 | 3篇 |
1992年 | 3篇 |
1991年 | 2篇 |
1989年 | 1篇 |
1988年 | 2篇 |
1987年 | 5篇 |
1986年 | 1篇 |
1985年 | 4篇 |
1984年 | 5篇 |
1983年 | 4篇 |
1982年 | 1篇 |
1981年 | 2篇 |
1980年 | 2篇 |
1979年 | 2篇 |
1978年 | 1篇 |
1976年 | 1篇 |
1975年 | 1篇 |
1973年 | 1篇 |
1972年 | 1篇 |
1965年 | 1篇 |
1923年 | 3篇 |
排序方式: 共有246条查询结果,搜索用时 46 毫秒
191.
Rodrigo Pereira Cavalcante Lucas da Rocha Sandim Danielle Bogo Antônio Marcos Jacques Barbosa Marly Eiko Osugi Matildes Blanco Silvio Cesar de Oliveira Maria de Fatima Cepa Matos Amilcar Machulek Jr Valdir Souza Ferreira 《Environmental science and pollution research international》2013,20(4):2352-2361
In the present study, selected advanced oxidation processes (AOPs)—namely, photo-Fenton (with Fe2+, Fe3+, and potassium ferrioxalate—FeOx—as iron sources), solar photo-Fenton, Fenton, and UV/H2O2—were investigated for degradation of the antineoplastic drug mitoxantrone (MTX), frequently used to treat metastatic breast cancer, skin cancer, and acute leukemia. The results showed that photo-Fenton processes employing Fe(III) and FeOx and the UV/H2O2 process were most efficient for mineralizing MTX, with 77, 82, and 90 % of total organic carbon removal, respectively. MTX probably forms a complex with Fe(III), as demonstrated by voltammetric and spectrophotometric measurements. Spectrophotometric titrations suggested that the complex has a 2:1 Fe3+:MTX stoichiometric ratio and a complexation constant (K) of 1.47 × 104 M–1, indicating high MTX affinity for Fe3+. Complexation partially inhibits the involvement of iron ions and hence the degradation of MTX during photo-Fenton. The UV/H2O2 process is usually slower than the photo-Fenton process, but, in this study, the UV/H2O2 process proved to be more efficient due to complexing of MTX with Fe(III). The drug exhibited no cytotoxicity against NIH/3T3 mouse embryonic fibroblast cells when oxidized by UV/H2O2 or by UV/H2O2/FeOx at the concentrations tested. 相似文献
192.
Harold S. Javitz John G. Watson Jacques P. Guertin Peter K. Mueller 《Journal of the Air & Waste Management Association (1995)》2013,63(5):661-667
This paper summarizes the results of an Electric Power Research Institute funded research effort to determine the feasibility of using receptor models for the apportionment of power plant contributions to air quality, deposition quality, and light extinction on local and regional scales. Sufficient information currently exists (or was developed during the course of this study) to establish feasibility for the apportionment of power plant contributions to local-scale air quality and to strongly suggest the usefulness of receptor modeling for regional-scale air quality, light extinction, and dry deposition quality apportionment. Insufficient information existed to determine whether or not receptor modeling can be useful for the allocation of wet deposition quality. A series of seven future research recommendations were prepared for the purpose of advancing receptor modeling from theoretical feasibility to practical utility. Two recommendations address model evaluation: (1) prepare a user-oriented receptor model application and testing package, and (2) perform computer simulation testing of past, current, and proposed receptor model applications. Two recommendations address model development: (1) develop a receptor model requiring minimal information about source profiles, and (2) develop a “hybrid” model (i.e., a model that combines source and receptor oriented methods). Finally, three recommendations address source characterization: (1) develop procedures for individual particle characterization, (2) develop sampling and analysis methods for source profile determination, and (3) measure source profiles of coal- and oil-fired power plants, and other sources that confound identification of emissions from coal- and oilfired power plants. 相似文献
193.
Awa Ndiaye Wilfried Sanchez Jean-Dominique Durand Hélène Budzinski Olivier Palluel Khady Diouf Papa Ndiaye Jacques Panfili 《Environmental science and pollution research international》2012,19(9):4133-4147
The study highlights the potential of the black-chinned tilapia to be used as a sentinel to assess environmental contaminants based on the use of a set of biomarkers. The usefulness of fish species as sentinels for assessing aquatic environment contamination was tested using a set of biomarkers in Senegalese environments characterized by multi-pollution sources. The black-chinned tilapia (Sarotherodon melanotheron) was selected as a sentinel because of its abundance, wide distribution in all coastal aquatic ecosystems and physiological properties. The potential influence of confounding factors such as salinity on biomarker in the tilapia has been examined. Individuals were sampled during two seasons (dry and wet) in eight sites characterized by various degrees of anthropogenic contamination and different salinities (from 0 to 102?psu). Biomarkers??including growth rate (GR), condition factor (CF), biotransformation enzymes such as 7-ethoxyresorufin-O-deethylase (EROD) and glutathione-S-transferase (GST), lipid peroxidation (TBARS) and acetylcholinesterase (AChE)??were measured. Chemical contaminant [polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs)] levels showed different sources of contamination with relatively high concentrations of PAHs in the Hann Bay and Foundiougne locations. The most sensitive biomarker present in different sites according to the principal component analysis is EROD. Few variations of the AChE activity and TBARS levels were found. No clear relationship was found between biomarker responses and salinity, but GR and CF were lower in hypersaline conditions. Tilapia is responsive to environmental contaminants such as PAHs, OCPs and PCBs. The S. melanotheron multiparametric approach showed a better discrimination of sites. 相似文献
194.
Vieira CD de Carvalho MA Cussiol NA Alvarez-Leite ME dos Santos SG Gomes RM Silva MX Nicoli JR Farias Lde M 《Waste management (New York, N.Y.)》2011,31(6):1327-1332
In Brazil, few studies on microbial content of dental solid waste and its antibiotic susceptibility are available. An effort has been made through this study to evaluate the hazardous status of dental solid waste, keeping in mind its possible role in cross-infection chain. Six samples of solid waste were collected at different times and seasons from three dental health services. The microbial content was evaluated in different culture media and atmospheric conditions, and the isolates were submitted to antibiotic susceptibility testing. A total of 766 bacterial strains were isolated and identified during the study period. Gram-positive cocci were the most frequent morphotype isolated (48.0%), followed by Gram-negative rods (46.2%), Gram-positive rods (5.0%), Gram-negative-cocci (0.4%), and Gram-positive coccobacillus (0.1%). Only two anaerobic bacteria were isolated (0.3%). The most frequently isolated species was Staphylococcus epidermidis (29.9%), followed by Stenotrophomonas maltophilia (8.2%), and Enterococcus faecalis (6.7%). High resistance rate to ampicillin was observed among Gram-negative rods (59.4%) and Gram-positive cocci (44.4%). For Gram-negative rods, high resistance was also noted to aztreonam (47.7%), cefotaxime (47.4%), ceftriaxone and cefazolin (43.7%), and ticarcillin-clavulanic acid (38.2%). Against Gram-positive cocci penicillin exhibit a higher resistance rate (45.0%), followed by ampicillin, erythromycin (27.2%), and tetracycline (22.0%). The present study demonstrated that several pathogenic bacteria are present in dental solid waste and can survive after 48 h from the waste generation time and harbor resistance profiles against several clinical recommended antibiotics. 相似文献
195.
Ghanem A Bados P Estaun AR de Alencastro LF Taibi S Einhorn J Mougin C 《Chemosphere》2007,69(9):1368-1373
Indirect soil pollution by heavy metals and organics may occur when sewage sludge is used as fertilizer. It is essential to define the nature and amounts of pollutants contained in sewage sludge in order to assess environmental risk. Here, we present results from a one-year monitoring of herbicides (glyphosate, diuron and atrazine) and their major degradates in sewage sludge sampled from three wastewater treatment plants and one composting unit in the vicinity of Versailles, France. The concentrations of these compounds were determined, as well as these of the surfactant nonylphenol. We demonstrated the presence of glyphosate and aminomethylphosphonic acid at the mg kg(-1) (dry matter) level in all samples. Diuron was detected at the microg kg(-1) (d.m.) level, whereas its degradate and triazine compounds were below the limits of quantification. Nonylphenol amounts were higher than the future European limit value of 50 mg kg(-1) (d.m.). 相似文献
196.
Introduced trout sever trophic connections in watersheds: consequences for a declining amphibian 总被引:1,自引:0,他引:1
Trophic linkages between terrestrial and aquatic ecosystems are increasingly recognized as important yet poorly known features of food webs. Here we describe research to understand the dynamics of lake food webs in relation to a native riparian amphibian and its interaction with introduced trout. The mountain yellow-legged frog Rana muscosa is endemic to alpine watersheds of the Sierra Nevada Mountains and the Transverse Ranges of California, but it has declined to a small fraction of its historical distribution and abundance. Although remaining frogs and introduced trout feed in different habitats of alpine lakes, our stable-isotope analyses clearly show that the same resource base of benthic invertebrates sustains their growth. During one period, insect emergence from naturally fishless lakes was nearly 20-fold higher compared to adjacent lakes with trout, showing that fish reduce availability of aquatic prey to amphibious and terrestrial consumers. Although trout cannot prey on adult frogs due to gape limitation, foraging post-metamorphic frogs are 10 times more abundant in the absence of trout, suggesting an important role for competition for prey by trout in highly unproductive alpine watersheds. Most Sierran lakes contain fish, and those that do not are usually small isolated ponds; in our study, these two lake types supported the lowest densities of post-metamorphic frogs, and these frogs were less reliant on local, benthic sources of productivity. Since Rana muscosa was formerly the most abundant vertebrate in the Sierra Nevada, the reduction in energy flow from lake benthos to this consumer due to fish introductions may have had negative consequences for its numerous terrestrial predators, many of which have also declined. We suggest that disruptions of trophic connections between aquatic and terrestrial food webs are an important but poorly understood consequence of fish introduction to many thousands of montane lakes and streams worldwide and may contribute to declines of native consumers in riparian habitats. 相似文献
197.
Modelling nature-like fishway flow around unsubmerged obstacles using a 2D shallow water model 总被引:1,自引:0,他引:1
Tien?Dung?Tran Jacques?Chorda Pascale?Laurens Ludovic?CassanEmail author 《Environmental Fluid Mechanics》2016,16(2):413-428
In the scope to create efficient nature like fish ramps using large-scale roughness elements, the present study is an audit of modelling such complex 3D free surface flows using an industrial 2D code solving shallow water equations. Validation procedure is based upon the comparison between numerous experimental measurements and numerical runs around large-scale roughness patterns disposed on the flume bottom in order to determine what 2D reliable numerical results can be expected. In this paper, we focused on cases of unsubmerged obstacles. The results demonstrate that 2D shallow water modelling using an industrial code such as TELEMAC-2D can be a convenient way for the hydraulic engineer to help design a nature-like fishway. This article emphasizes the limitations due to 2D depth integration of velocities and turbulence modelling and gives the domain of validity of the method. 相似文献
198.
Vona Méléder Jacques Populus Brigitte Guillaumont Thierry Perrot Pascal Mouquet 《Marine Biology》2010,157(7):1525-1541
Predictive modelling to map subtidal communities is an alternative to “traditional” methods, such as direct sampling, remote
sensing and acoustic survey, which are neither time- nor cost-effective for vast expanses. The principle of this modelling
is the use of a combination of environmental key parameters to produce rules to understand species distribution and hence
generate predictive maps. This study focuses on subtidal kelp forests (KF) on the coast of Brittany, France. The most significant
key parameters to predict KF frequency are (1) the nature of the substrate, (2) depth, (3) water transparency, (4) water surface
temperature and (5) hydrodynamics associated with the flexibility of algae in a flow. All these parameters are integrated
in a spatial model, built using a Geographical Information System. This model results in a KF frequency map, where sites with
optimum key parameters show a deeper limit of disappearance. After validation, the model is used in the context of Climate
Change to estimate the effect of environmental variation on this depth limit of KF. Thus, the effects of both an increase
in water temperature and a decrease in its transparency could lead to the complete disappearance of KF. 相似文献
199.
Doumas Patrick Munoz Marguerite Banni Mohamed Becerra Sylvia Bruneel Odile Casiot Corinne Cleyet-Marel Jean-Claude Gardon Jacques Noack Yves Sappin-Didier Valérie 《Regional Environmental Change》2018,18(3):677-692
Regional Environmental Change - Abandoned mines are a recurrent problem for nearby communities in Mediterranean regions because mine tailings represent a major source of polymetallic contamination.... 相似文献
200.
Ygor Jacques Agra Bezerra da Silva Clístenes Williams Araújo do Nascimento Caroline Miranda Biondi 《Environmental monitoring and assessment》2014,186(1):47-53
The use of appropriate analytical methods is of paramount importance for risk assessment and monitoring of potentially toxic metals in soils. In this sense, the objective of this study was to compare the effectiveness of two sample digestion methods, recommended by the Brazilian legislation for the management of contaminated areas (CONAMA 2009), aiming at the determination of environmentally available metal concentrations (USEPA 3050B, USEPA 3051A), as well as a total digestion method (USEPA 3052). Samples from 10 classes of soils were analyzed for Cu, Zn, Cd, Pb, Ni, and Hg. The results showed that the USEPA method 3051A is more efficient than the USEPA method 3050B in the extraction of levels considered environmentally available of Zn, Cu, Cd, Pb, and Ni. Besides providing a higher recovery of these elements, the method requires shorter digestion time, lower consumption of acids, and reduced risk of contamination. The USEPA method 3051A showed greater efficiency in Hg extraction in soils with higher clay content. Therefore, it is suitable for situations where a wide range of soils with different mineralogical characteristics are analyzed or in order to decrease the losses due to volatilization of the element in open systems. 相似文献