全文获取类型
收费全文 | 2803篇 |
免费 | 35篇 |
国内免费 | 31篇 |
专业分类
安全科学 | 81篇 |
废物处理 | 104篇 |
环保管理 | 373篇 |
综合类 | 606篇 |
基础理论 | 559篇 |
环境理论 | 3篇 |
污染及防治 | 809篇 |
评价与监测 | 161篇 |
社会与环境 | 157篇 |
灾害及防治 | 16篇 |
出版年
2023年 | 33篇 |
2022年 | 32篇 |
2021年 | 47篇 |
2020年 | 36篇 |
2019年 | 38篇 |
2018年 | 81篇 |
2017年 | 85篇 |
2016年 | 100篇 |
2015年 | 106篇 |
2014年 | 118篇 |
2013年 | 141篇 |
2012年 | 123篇 |
2011年 | 183篇 |
2010年 | 151篇 |
2009年 | 158篇 |
2008年 | 156篇 |
2007年 | 162篇 |
2006年 | 115篇 |
2005年 | 100篇 |
2004年 | 106篇 |
2003年 | 77篇 |
2002年 | 91篇 |
2001年 | 82篇 |
2000年 | 45篇 |
1999年 | 25篇 |
1998年 | 32篇 |
1997年 | 30篇 |
1996年 | 30篇 |
1995年 | 49篇 |
1994年 | 29篇 |
1993年 | 13篇 |
1992年 | 23篇 |
1991年 | 29篇 |
1990年 | 17篇 |
1989年 | 23篇 |
1988年 | 13篇 |
1987年 | 10篇 |
1986年 | 10篇 |
1985年 | 7篇 |
1984年 | 9篇 |
1983年 | 7篇 |
1982年 | 13篇 |
1981年 | 12篇 |
1980年 | 6篇 |
1979年 | 11篇 |
1978年 | 6篇 |
1970年 | 8篇 |
1969年 | 6篇 |
1959年 | 6篇 |
1958年 | 5篇 |
排序方式: 共有2869条查询结果,搜索用时 31 毫秒
71.
Jacqueline T. Bangm Jessica L. Reiner Hannes Both Theresa M. Cantu Marco A. Gouws Matthew P. Guillette Jeremy P. Koelmel Wilmien J. Luus-Powell Jan Myburgh Olivia Rynders Joseph R. Sar Willem J. Smit John A. Bowden 《环境科学学报(英文版)》2017,29(11):59-67
This study examined concentrations of 15 perfluoroalkyl acids (PFAAs) in tissues from male Mozambique tilapia (Oreochromis mossambicus) collected at Loskop Dam, Mpumalanga, South Africa in 2014 and 2016. Nine of the 15 PFAAs were detected frequently and were included in statistical analysis and included two of the most commonly known PFAAs, perfluorooctanesulfonic acid (PFOS) (median, 41.6 ng/g) and perfluorooctanoic acid (PFOA) (median, 0.0825 ng/g). Of the tissues measured, plasma (2016 and 2014 median, 22.2 ng/g) contained the highest PFAA burden followed by (in descending order): liver (median, 11.6 ng/g), kidney (median, 9.04 ng/g), spleen (median, 5.92 ng/g), adipose (median, 2.54 ng/g), and muscle (median, 1.11 ng/g). Loskop Dam tilapia have been affected by an inflammatory disease of the adipose tissue known as pansteatitis, so this study also aimed to investigate relationships between PFAA tissue concentrations and incidence of pansteatitis or fish health status. Results revealed that healthy tilapia exhibited an overall higher (p-value < 0.05) PFAA burden than pansteatitis-affected tilapia across all tissues. Further analysis showed that organs previously noted in the literature to contain the highest PFAA concentrations, such as kidney, liver, and plasma, were the organs driving the difference in PFAA burden between the two tilapia groups. Care must be taken in the interpretations we draw from not only the results of our study, but also other PFAA measurements made on populations (human and wildlife alike) under differing health status. 相似文献
72.
Ericson I Gómez M Nadal M van Bavel B Lindström G Domingo JL 《Environment international》2007,33(5):616-623
Fluorinated organic compounds (FOCs) are a group of chemicals widely used as surfactants, lubricants, polymers, and fire-fighting foams. Recent studies have shown the ubiquitous distribution of FOCs in the environment, wildlife, and humans. We here report the results of a pilot study conducted to provide preliminary data on the levels of 13 FOCs in the blood of 48 residents in Catalonia, Spain, in relation to gender and age (25+/-5 and 55+/-5 years). The highest mean concentration was obtained for perfluorooctane sulfonate (PFOS, 7.64 ng/ml), followed by perfluorohexane sulfonate (PFHxS, 3.56 ng/ml) and perfluorooctanoic acid (PFOA, 1.80 ng/ml). Four other FOCs showed mean levels between 0.30 and 0.44 ng/ml, whereas those of the remaining 6 compounds were below the detection limit. Regarding gender, the blood levels of PFHxS and PFOA were significantly higher (p<0.05) in men than in women, while differences according to age were only noted for PFHxS (p<0.05) and perfluorooctane sulfonamide (PFOSA) (p<0.001), for which the levels were higher in the younger (25+/-5 years) group of subjects. A significant correlation between PFOS levels and those of the remaining detected FOCs (except PFDA) was found. In general terms, the current FOC concentrations were lower than those found in recent studies concerning levels of these chemicals in human blood and serum of subjects from different countries. 相似文献
73.
Bogers R De Vries-Buitenweg S Geuijen I van de Waart B Kuiper R Van Der Linden S Puijker L Murk A Van Der Burg B Legler J 《Environment international》2007,33(3):292-301
Adult male fathead minnow were exposed for 14 or 28-days under flow-through conditions to undiluted filtered water samples from the rivers Meuse and Rhine in the Netherlands. The experiment included two vessels per treatment each containing 10 fish and samples of five fish were taken after 14 and 28 days. Additional groups were exposed to 17alpha-ethinylestradiol (EE2) as a reference and untreated drinking water as a negative control. Major endpoints examined included induction of vitellogenin (VTG) synthesis, VTG mRNA activity, hepato- and gonadosomatic indices (HSI and GSI) and gonadal histology. No significant difference was recorded in body weight or mean GSI values between the various treatments. Only exposure to Meuse water resulted in significantly higher HSI means after 14 days. Histological examination showed no apparent effects on gonadal tissue except for eosinophilic blood plasma in fish exposed to Meuse water or EE2. After 14 and 28 days, elevated VTG and VTG mRNA levels were measured in most livers of the fish exposed to Meuse water, but not in the fish exposed to Rhine water. This was confirmed by measuring estrogenic responses in the in vitro ER CALUX assay. Induction of VTG synthesis proved to be the most sensitive endpoint in the Non Spawning Male Fish Assay for in vivo detection of bio-available estrogenic activity supplementary to a sensitive in vitro assay. The other endpoints examined varied too much and required a higher number of fish or replicates to achieve sufficient power for statistical testing making them less animal friendly. 相似文献
74.
Hesti Lestari Tata Meine van Noordwijk Denis Ruysschaert Rachmat Mulia Subekti Rahayu Elok Mulyoutami Atiek Widayati Andree Ekadinata Riswan Zen Adji Darsoyo Rahayu Oktaviani Sonya Dewi 《Mitigation and Adaptation Strategies for Global Change》2014,19(6):693-713
Tripa is the last remaining peat-swamp forest that harbours a potentially viable Sumatran orangutan (Pongo abelii) sub-population in a formally but not effectively protected area. It appears to be a simple showcase where current efforts to financially support reducing emissions from deforestation and forest degradation (REDD+) converge with biodiversity and social co-benefits. In practice, however, situation is more complex. REDD+ efforts interact with global palm oil trade and regulatory approaches (the moratorium) to achieve national goals for emissions reduction under umbrella of nationally appropriate mitigation actions (NAMA). To contextualize this debate, we assessed (i) land-use history and formal basis of palm-oil companies’ rights; (ii) carbon (C) stocks, historical emission levels and potential emissions that can be avoided; (iii) economic benefits of land-use options and opportunity costs of avoiding emissions; (iv) biodiversity and environmental services; and (v) alternative options for “high C stock development” and employment generation. Natural forest cover declined (54 % in 1995, 18 % in 2009) while oil palm increased 4–39 %. Aboveground C stocks decreased from 148 Mg ha?1 in 1990 to 61 Mg ha?1 in 2009, leading to average annual emissions of 14.5 Mg (carbon dioxide) CO2e ha?1 year?1. While 41 % of these emissions yield less than American Dollar (USD) 5 of current economic benefits per Mg CO2e emitted and might be compensated by REDD+, nearly all new emissions derive from a breach of existing laws, regulations and voluntary palm-oil standards. Substantial investment in alternative employment is needed, rather than carbon payments per se, to support livelihoods in a low carbon emissions economy. 相似文献
75.
Philippe Louâpre Stéphanie Llopis Véronique Martel Joan van Baaren 《Die Naturwissenschaften》2014,101(11):875-882
In many insect species, sperm-depleted males (SDMs, i.e. males that have exhausted their sperm after a given number of matings) remain sexually active and continue to mate females. Here, we investigated the behavioural modifications that occur in both sexes of the parasitoid Asobara tabida Nees (Hymenoptera: Braconidae), after matings by fertile males and sperm-depleted males. We show that (i) virgin females, mated females and females mated to a SDM exhibited different behaviours and that (ii) males responded differently to females depending on whether the females had previously mated with an SDM or not. Our findings demonstrate that SDM influenced the reproductive behaviour of both males and females, especially with regard to male responsiveness and female attractiveness. These findings are discussed in the context of adaptive behaviour and fitness maximization in both males and females. 相似文献
76.
77.
Hole LR Brunner SH Hanssen JE Zhang L 《Environmental pollution (Barking, Essex : 1987)》2008,154(3):473-481
The conditional time averaged gradient method was used to measure air-surface exchange of nitrogen and sulphur compounds at a semi-alpine site in Southern Norway. Dry deposition velocities were then obtained from the bi-weekly concentration gradient measurements. Annual deposition velocities were found to be 1.4, 11.8 and 4.0 mm s(-1) for NH3, HNO3 and SO2, respectively, if all data were included, and to be 10.8, 11.8 and 13.0 mm s(-1), respectively, if only positive values were included. Measured deposition velocities were compared to two sets of values estimated from a big-leaf dry deposition module applying to two different land types (short grass and forbs, and tundra), driven by measured micrometeorological parameters. The deposition module gives reasonable values for this site throughout the year, but does not reproduce the large variability as shown in the measured data. No apparent seasonal variations were found from either measurements or module estimates due to the very low productivity of the studied area. 相似文献
78.
Holtze MS Sørensen SR Sørensen J Aamand J 《Environmental pollution (Barking, Essex : 1987)》2008,154(2):155-168
The benzonitriles dichlobenil, bromoxynil and ioxynil are important broad-spectrum or selective herbicides used in agriculture, orchards and public areas worldwide. The dichlobenil metabolite 2,6-dichlorobenzamide is the most frequently encountered groundwater contaminant in Denmark, which suggests that the environmental fate of these three structurally related benzonitrile herbicides should be addressed in detail. This review summarises the current knowledge on microbial degradation of dichlobenil, bromoxynil and ioxynil with particular focus on common features of degradation rates and pathways, accumulation of persistent metabolites and diversity of the involved degrader organisms. 相似文献
79.
Teuchies J de Deckere E Bervoets L Meynendonckx J van Regenmortel S Blust R Meire P 《Environmental pollution (Barking, Essex : 1987)》2008,155(1):20-30
A historical input of trace metals into tidal marshes fringing the river Scheldt may be a cause for concern. Nevertheless, the specific physicochemical form, rather than the total concentration, determines the ecotoxicological risk of metals in the soil. In this study the effect of tidal regime on the distribution of trace metals in different compartments of the soil was investigated. As, Cd, Cu and Zn concentrations in sediment, pore water and in roots were determined along a depth profile. Total sediment metal concentrations were similar at different sites, reflecting pollution history. Pore water metal concentrations were generally higher under less flooded conditions (mean is (2.32 ± 0.08) × 10−3 mg Cd L−1 and (1.53 ± 0.03) × 10−3 mg Cd L−1). Metal concentrations associated with roots (mean is 202.47 ± 2.83 mg Cd kg−1 and 69.39 ± 0.99 mg Cd kg−1) were up to 10 times higher than sediment (mean is 20.48 ± 0.19 mg Cd kg−1 and 20.42 ± 0.21 mg Cd kg−1) metal concentrations and higher under dryer conditions. Despite high metal concentrations associated with roots, the major part of the metals in the marsh soil is still associated with the sediment as the overall biomass of roots is small compared to the sediment. 相似文献
80.
Kinetic extractions to assess mobilization of Zn, Pb, Cu, and Cd in a metal-contaminated soil: EDTA vs. citrate 总被引:4,自引:0,他引:4
Labanowski J Monna F Bermond A Cambier P Fernandez C Lamy I van Oort F 《Environmental pollution (Barking, Essex : 1987)》2008,152(3):693-701
Kinetic EDTA and citrate extractions were used to mimic metal mobilization in a soil contaminated by metallurgical fallout. Modeling of metal removal rates vs. time distinguished two metal pools: readily labile (QM1) and less labile (QM2). In citrate extractions, total extractability (QM1+QM2) of Zn and Cd was proportionally higher than for Pb and Cu. Proportions of Pb and Cu extracted with EDTA were three times higher than when using citrate. We observed similar QM1/QM2 ratios for Zn and Cu regardless of the extractant, suggesting comparable binding energies to soil constituents. However, for Pb and Cd, more heterogeneous binding energies were hypothesized to explain different kinetic extraction behaviors. Proportions of citrate-labile metals were found consistent with their short-term, in-situ mobility assessed in the studied soil, i.e., metal amount released in the soil solution or extracted by cultivated plants. Kinetic EDTA extractions were hypothesized to be more predictive for long-term metal migration with depth. 相似文献