全文获取类型
收费全文 | 555篇 |
免费 | 27篇 |
国内免费 | 296篇 |
专业分类
安全科学 | 27篇 |
废物处理 | 29篇 |
环保管理 | 54篇 |
综合类 | 377篇 |
基础理论 | 123篇 |
污染及防治 | 200篇 |
评价与监测 | 14篇 |
社会与环境 | 33篇 |
灾害及防治 | 21篇 |
出版年
2023年 | 17篇 |
2022年 | 23篇 |
2021年 | 25篇 |
2020年 | 20篇 |
2019年 | 29篇 |
2018年 | 24篇 |
2017年 | 27篇 |
2016年 | 30篇 |
2015年 | 37篇 |
2014年 | 45篇 |
2013年 | 49篇 |
2012年 | 48篇 |
2011年 | 53篇 |
2010年 | 42篇 |
2009年 | 45篇 |
2008年 | 56篇 |
2007年 | 41篇 |
2006年 | 28篇 |
2005年 | 27篇 |
2004年 | 21篇 |
2003年 | 18篇 |
2002年 | 22篇 |
2001年 | 17篇 |
2000年 | 9篇 |
1999年 | 19篇 |
1998年 | 19篇 |
1997年 | 30篇 |
1996年 | 9篇 |
1995年 | 5篇 |
1994年 | 9篇 |
1993年 | 11篇 |
1992年 | 6篇 |
1991年 | 5篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1987年 | 1篇 |
1986年 | 2篇 |
1984年 | 1篇 |
1983年 | 2篇 |
1982年 | 2篇 |
1981年 | 2篇 |
排序方式: 共有878条查询结果,搜索用时 0 毫秒
771.
Practical performance and its effciency of arsenic removal from groundwater
using Fe-Mn binary oxide
A treatment unit packed by granular adsorbent of Fe-Mn binary oxide incorporated into diatomite (FMBO(1:1)-diatomite) was studied to remove arsenic from anaerobic groundwater without any pre-treatment or post-treatment. The raw anaerobic groundwater containing 35-45 μg/L of arsenic was collected from suburb of Beijing. Arsenic(III) constituted roughly 60%-80% of the total arsenic content. Approximately 7,000 bed volumes (ratio of efluent volume to adsorbent volume) treated water with arsenic concentration b... 相似文献
772.
Junwen Chen Huacong Liu Yaohui Bai Jing Qi Weixiao Qi Huijuan Liu Jianfeng Peng Jiuhui Qu 《环境科学学报(英文版)》2022,34(5):103-113
Lake mixing influences aquatic chemical properties and microbial community composition,and thus, we hypothesized that it would alter microbial community assembly and interaction. To clarify this issue, we explored the community assembly processes and cooccurrence networks in four seasons at two depths(epilimnion and hypolimnion) in a mesotrophic and stratified lake(Chenghai Lake), which formed stratification in the summer and turnover in the winter. During the stratification period, the epilimni... 相似文献
773.
Removal of tetracycline from water by Fe-Mn binary oxide 总被引:2,自引:0,他引:2
Significant concerns have been raised over the presence of antibiotics including tetracyclines in aquatic environments. A series of Fe-Mn binary oxide with different Fe:Mn molar ratios was synthesized by a simultaneous oxidation and coprecipitation process for TC removal. Results showed that Fe-Mn binary oxide had higher removal efficiency than that of hydrous iron oxide and hydrous manganese oxide, and that the oxide with a Fe:Mn molar ratio of 5:1 was the best in removal than other molar ratios. The tetracycline removal was highly pH dependent. The removal of tetracycline decreased with the increase of initial concentration, but the absolute removal quantity was more at high concentration. The presence of cations and anions such as Ca2+, Mg2+, CO32- and SO42- had no significant effect on the tetracycline removal in our experimental conditions, while SiO32- and PO43- had hindered the adsorption of tetracycline. The mechanism investigation found that tetracycline removal was mainly achieved by the replacement of surface hydroxyl groups by the tetracycline species and formation of surface complexes at the water/oxide interface. This primary study suggests that Fe-Mn binary oxide with a proper Fe:Mn molar ratio will be a very promising material for the removal of tetracycline from aqueous solutions. 相似文献
774.
北三河水系沉积物中金属的污染状况研究 总被引:3,自引:2,他引:3
北三河水系包括接纳了北京、天津大量再生水和污水的温榆河、凉水河和北运河等河流,其沉积物中金属的污染状况是水环境质量的重要指标之一.本研究调查分析了北三河水系8条河流沉积物中金属的污染状况及存在形态,采用地累积指数评价了金属的污染级别,利用相关性分析和主成分分析简要分析了金属的主要来源.研究结果表明,北三河水系沉积物中Fe、Mn、Zn、Cr、Cu、Ni、Pb、Co和Cd的平均浓度分别为24207、538、303、57、48、29、15.2、14和0.27 mg·kg-1.牛牧屯河部分沉积物中Fe、Zn、Cu、Cr和Ni的浓度高于沉积物质量基准(SQG)中的极有可能产生危害的浓度(PEC)值,很有可能对生物产生危害;而温榆河、还乡河、北运河、凉水河和潮白河中大部分金属浓度高于产生危害的阈值(TEC)而低于PEC水平,也应列入防控对象.河流沉积物中金属积累级别较高的河段多位于郊区和乡镇,可能因为这些区域污水处理率较低.Fe、Cr、Ni、Cu、Mn和Zn在沉积物中主要以残渣态存在,其比例分别可达92.5%、85.2%、87.9%、71.0%、63.4%和57.3%;Pb则主要以可提取态存在,其比例为62.6%.沉积物中Cu、Pb、Ni和Cd元素的存在主要受人类活动的影响,其在北三河水系沉积物中的分布主要受有机碳的控制;Cr和Co的存在则主要受自然因素的影响,其分布主要受铁锰氧化物或矿物质的影响. 相似文献
775.
A Zr-β-FeOOH adsorbent for both As(V) and As(III) removal was prepared by a chemical co-precipitation method.Compared with β-FeOOH,the addition of Zr enhanced the adsorption capacities for As(V) and As(III),especially As(III).The maximum adsorption capacities for As(III) and As(V) were 120 and 60mg/g respectively at pH 7.0,much higher than for many reported adsorbents.The adsorption data accorded with Freundlich isotherms.At neutral pH,for As(V),adsorption equilibrium was approached after 3 hr,while for As(III),adsorption equilibrium was approached after 5 hr.Kinetic data fitted well to the pseudo second-order reaction model.As(V) elimination was favored at acidic pH,whereas the adsorption of As(III) by Zr-β-FeOOH was found to be effective over a wide pH range of 4-10.Competitive anions hindered the adsorption according to the sequence:phosphate > silicate > bicarbonate > sulfate > nitrate,while Ca2+ and Mg2+ increased the removal of As(III) and As(V) slightly.The high adsorption capability and good performance in other aspects make Zr-β-FeOOH a potentially attractive adsorbent for the removal of both As(III) and As(V) from water. 相似文献
776.
Xixi Wang Shiyou Shang Zhongyi Qu Tingxi Liu Assefa M. Melesse Wanhong Yang 《Journal of environmental management》2010,91(7):1511-1525
Wetlands are one of the most important watershed microtopographic features that affect hydrologic processes (e.g., routing) and the fate and transport of constituents (e.g., sediment and nutrients). Efforts to conserve existing wetlands and/or to restore lost wetlands require that watershed-level effects of wetlands on water quantity and water quality be quantified. Because monitoring approaches are usually cost or logistics prohibitive at watershed scale, distributed watershed models such as the Soil and Water Assessment Tool (SWAT), enhanced by the hydrologic equivalent wetland (HEW) concept developed by Wang [Wang, X., Yang, W., Melesse, A.M., 2008. Using hydrologic equivalent wetland concept within SWAT to estimate streamflow in watersheds with numerous wetlands. Trans. ASABE 51 (1), 55–72.], can be a best resort. However, there is a serious lack of information about simulated effects using this kind of integrated modeling approach. The objective of this study was to use the HEW concept in SWAT to assess effects of wetland restoration within the Broughton's Creek watershed located in southwestern Manitoba, and of wetland conservation within the upper portion of the Otter Tail River watershed located in northwestern Minnesota. The results indicated that the HEW concept allows the nonlinear functional relations between watershed processes and wetland characteristics (e.g., size and morphology) to be accurately represented in the models. The loss of the first 10–20% of the wetlands in the Minnesota study area would drastically increase the peak discharge and loadings of sediment, total phosphorus (TP), and total nitrogen (TN). On the other hand, the justifiable reductions of the peak discharge and loadings of sediment, TP, and TN in the Manitoba study area may require that 50–80% of the lost wetlands be restored. Further, the comparison between the predicted restoration and conservation effects revealed that wetland conservation seems to deserve a higher priority while both wetland conservation and restoration may be equally important. 相似文献
777.
778.
针对某炼厂试点装置的设备完整性管理体系执行状况开展了初始状态评价。本次评价以美国职业安全与卫生署《化学品过程安全管理》设备完整性要素为基础,结合过程安全管理符合性导则与建议、机械完整性实施指南等业界最佳实践,编制评价问项,组建包含管理、工艺、设备人员和承包商在内的评价工作组,采取查阅档案、信息化平台纪录,面对面访谈,作业现场考察与验证,评价工作会等方式,以半定量的方式找出了设备完整性管理体系较高的残余风险,对设备完整性管理体系框架结构和管理文件体系以及绩效指标体系提出了针对性改进建议。 相似文献
779.
780.
墨西哥湾“深水地平线”钻井平台事故分析与反思 总被引:1,自引:0,他引:1
对美国墨西哥湾“深水地平线”钻井平台爆炸事故进行了原因分析,总结了事故的经验教训,并从技术、管理、应急救援体系、技术研发4个方面为中国石化提出了预防类似事故的建议措施。 相似文献