首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   709篇
  免费   50篇
  国内免费   176篇
安全科学   76篇
废物处理   45篇
环保管理   55篇
综合类   349篇
基础理论   98篇
污染及防治   222篇
评价与监测   34篇
社会与环境   36篇
灾害及防治   20篇
  2023年   16篇
  2022年   49篇
  2021年   37篇
  2020年   34篇
  2019年   25篇
  2018年   31篇
  2017年   36篇
  2016年   40篇
  2015年   47篇
  2014年   41篇
  2013年   61篇
  2012年   68篇
  2011年   64篇
  2010年   45篇
  2009年   46篇
  2008年   44篇
  2007年   46篇
  2006年   27篇
  2005年   19篇
  2004年   21篇
  2003年   16篇
  2002年   25篇
  2001年   21篇
  2000年   5篇
  1999年   9篇
  1998年   12篇
  1997年   10篇
  1996年   8篇
  1995年   6篇
  1994年   2篇
  1993年   3篇
  1992年   2篇
  1991年   5篇
  1989年   2篇
  1988年   5篇
  1987年   2篇
  1984年   1篇
  1982年   2篇
  1973年   1篇
  1972年   1篇
排序方式: 共有935条查询结果,搜索用时 723 毫秒
781.
This paper reports on an examination of data on how local residents in Tuscaloosa, a mid‐sized city in the state of Alabama, United States, responded to Hurricane Ivan of September 2004. The evaluation revealed that an integrated connection to community‐level communication resources—comprising local media, community organisations and interpersonal networks—has a direct impact on the likelihood of engaging in pre‐hurricane preparedness activities and an indirect effect on during‐hurricane preparedness activities. Neighbourhood belonging mediated the relation between an integrated connection to community‐level communication resources and during‐hurricane preparedness activities. Neighbourhood belonging was determined to increase the likelihood of taking preparedness actions during Hurricane Ivan, but not prior to it. In addition, we discovered an interesting pattern for two different types of risk perceptions: social and personal risk perceptions. Social risk perceptions increase the likelihood of taking preventative steps before a hurricane while personal risk perceptions are positively related to engaging in preventative action during a hurricane.  相似文献   
782.
• Principles and methods for fluorescence EEM are systematically outlined. • Fluorophore peak/region/component and energy information can be extracted from EEM. • EEM can fingerprint the physical/chemical/biological properties of DOM in MBRs. • EEM is useful for tracking pollutant transformation and membrane retention/fouling. • Improvements are still needed to overcome limitations for further studies. The membrane bioreactor (MBR) technology is a rising star for wastewater treatment. The pollutant elimination and membrane fouling performances of MBRs are essentially related to the dissolved organic matter (DOM) in the system. Three-dimensional excitation-emission matrix (3D-EEM) fluorescence spectroscopy, a powerful tool for the rapid and sensitive characterization of DOM, has been extensively applied in MBR studies; however, only a limited portion of the EEM fingerprinting information was utilized. This paper revisits the principles and methods of fluorescence EEM, and reviews the recent progress in applying EEM to characterize DOM in MBR studies. We systematically introduced the information extracted from EEM by considering the fluorescence peak location/intensity, wavelength regional distribution, and spectral deconvolution (giving fluorescent component loadings/scores), and discussed how to use the information to interpret the chemical compositions, physiochemical properties, biological activities, membrane retention/fouling behaviors, and migration/transformation fates of DOM in MBR systems. In addition to conventional EEM indicators, novel fluorescent parameters are summarized for potential use, including quantum yield, Stokes shift, excited energy state, and fluorescence lifetime. The current limitations of EEM-based DOM characterization are also discussed, with possible measures proposed to improve applications in MBR monitoring.  相似文献   
783.

Identification of different pollution sources in groundwater is challenging, especially in areas with diverse land uses and receiving multiple inputs. In this study, principal component analysis (PCA) was combined with geographic information system (GIS) to explore the spatial and temporal variation of groundwater quality and to identify the sources of pollution and main factors governing the quality of groundwater in a multiple land-use area in southwestern China. Groundwater samples collected from 26 wells in 2012 and 38 wells in 2018 were analyzed for 13 water quality parameters. The PCA results showed that the hydro-geochemical process was the predominant factor determining groundwater quality, followed by agricultural activities, domestic sewage discharges, and industrial sewage discharges. Agriculture expansion from 2012 to 2018 resulted in increased apportionment of agricultural pollution. In contrast, economic restructure and infrastructure improvement reduced the contributions of domestic sewage and industrial pollution. Anthropogenic activities were found the major causes of elevated nitrogen concentrations (NO3?, NO2?, NH4+) in groundwater, highlighting the necessity of controlling N sources through effective fertilizer managements in agricultural areas and reducing sewage discharges in urban areas. The applications of GIS and PCA successfully identified the sources of pollutants and major factors driving the variations of groundwater quality in tested years.

  相似文献   
784.
Environmental Science and Pollution Research - A submerged anaerobic membrane bioreactor (SAnMBR) was used to treat low-concentration domestic sewage. The effects of hydraulic retention time (HRT)...  相似文献   
785.
微山湖养殖湖区水体中多环芳烃的分布及来源   总被引:1,自引:0,他引:1  
郑曦  韩宝平  蒋欢  刘抗 《四川环境》2010,29(6):21-24
采用HPLC定量分析微山湖养殖湖区水体中16种优先控制PAHs的总量浓度范围在5348.8~12970.8ng/L之间,平均值为8671.5ng/L,处于中等偏高污染水平;养殖湖区水体中的多环芳烃主要来源于养殖船只的石油泄露及煤炭、木材与石油的不完全燃烧,PAHs的组成以2~3环为主。  相似文献   
786.
提升武汉城市圈各城市间资源集聚能力的空间关联程度,对于实现该区域的协调发展具有重要意义。基于此,运用修正的引力模型,采用社会网络分析法对1995~2015年武汉城市圈资源集聚能力的空间关联进行分析。研究表明:(1)武汉城市圈资源集聚能力的空间关联特征显著,网络密度呈现倒"U"型,网络等级逐年下降,网络效率呈现"U"型;(2)武汉城市圈资源集聚能力在网络中呈现"中心-边缘"的特征,武汉市的点度中心度最高,在网络中属于中心城市,而其它城市属于边缘城市;(3)板块一(武汉、孝感、天门)属于"双向溢出"板块,板块二(潜江、咸宁)属于"净受益"板块,板块三(仙桃、黄冈)属于"净溢出"板块,板块四(黄石、鄂州)属于"经纪人"板块。鉴于此,从多途径构建资源集聚能力空间关联"通道"、增强中心城市辐射带动功能和推动城市分工协作等3个方面提出了提升武汉城市圈资源集聚能力空间关联程度的政策建议。  相似文献   
787.
Carbamazepine degradation by photolysis and titanium dioxide photocatalysis   总被引:1,自引:0,他引:1  
We investigated the degradation of carbamazepine by photolysis/ultraviolet (UV)-C only and titanium dioxide photocatalysis. The degradation of carbamazepine by UV-only and titanium-dioxide-only (adsorption) reactions were inefficient, however, complete degradation of carbamazepine was observed by titanium dioxide photocatalysis within 30 min. The rate of degradation increased as initial carbamazepine concentration decreased, and the removal kinetics fit well with the Langmuir-Hinshelwood model. The addition of methanol, a radical scavenger, decreased carbamazepine removal, suggesting that the hydroxide radical played an important role during carbamazepine degradation. The addition of oxygen during titanium dioxide photocatalysis accelerated hydroxide radical production, thus improving mineralization activity. The photocatalytic degradation was more efficient at a higher pH, whereas the removal of carbamazepine and acridine (a major intermediate) were more efficient under aerobic conditions. The mineralization of carbamazepine during photocatalysis produced various ionic by-products such as ammonium and nitrate by way of nitrogen dioxide.  相似文献   
788.
吸附联合低温等离子体法去除甲苯废气   总被引:2,自引:0,他引:2  
对介质阻挡放电条件下产生的低温等离子体联合吸附去除低浓度甲苯废气进行了实验研究。考察了反应器内分别填充分子筛、陶瓷环和混合填料时,甲苯的吸附效果;比较了各种填充条件下,低温等离子体对甲苯的去除效果和副产物臭氧的产生量;并对填充混合填料时不同外加电压、不同操作条件下,吸附联合低温等离子体去除甲苯的过程进行系统的研究。结果表明,外加电压相同,混合填料对甲苯的去除率最高,大于97%,依次是分子筛、陶瓷环、无填充;同时混合填料的臭氧浓度小于其他填料;当电压为18 kV时,混合填料可获得较高的甲苯去除率,同时产生的臭氧副产物最少。  相似文献   
789.
Subway systems are considered as main public transportation facility in developed countries. Time spent by people in indoors, such as underground spaces, subway stations, and indoor buildings, has gradually increased in the recent past. Especially, operators or old persons who stay in indoor environments more than 15 hr per day usually influenced a greater extent by indoor air pollutants. Hence, regulations on indoor air pollutants are needed to ensure good health of people. Therefore, in this study, a new cumulative calculation method for the estimation of total amounts of indoor air pollutants emitted inside the subway station is proposed by taking cumulative amounts of indoor air pollutants based on integration concept. Minimum concentration of individual air pollutants which naturally exist in indoor space is referred as base concentration of air pollutants and can be found from the data collected. After subtracting the value of base concentration from data point of each data set of indoor air pollutant, the primary quantity of emitted air pollutant is calculated. After integration is carried out with these values, adding the base concentration to the integration quantity gives the total amount of indoor air pollutant emitted. Moreover the values of new index for cumulative indoor air quality obtained for 1 day are calculated using the values of cumulative air quality index (CAI). Cumulative comprehensive indoor air quality index (CCIAI) is also proposed to compare the values of cumulative concentrations of indoor air pollutants. From the results, it is clear that the cumulative assessment approach of indoor air quality (IAQ) is useful for monitoring the values of total amounts of indoor air pollutants emitted, in case of exposure to indoor air pollutants for a long time. Also, the values of CCIAI are influenced more by the values of concentration of NO2, which is released due to the use of air conditioners and combustion of the fuel. The results obtained in this study confirm that the proposed method can be applied to monitor total amounts of indoor air pollutants emitted, inside apartments and hospitals as well. Implications: Nowadays, subway systems are considered as main public transportation facility in developed countries. Time spent by people in indoors, such as underground spaces, subway stations, and indoor buildings, has gradually increased in the recent past. Especially, operators or old persons who stay in the indoor environments more than 15 hr per day usually influenced a greater extent by indoor air pollutants. Hence, regulations on indoor air pollutants are needed to ensure good health of people. Therefore, this paper presents a new methodology for monitoring and assessing total amounts of indoor air pollutants emitted inside underground spaces and subway stations. A new methodology for the calculation of cumulative amounts of indoor air pollutants based on integration concept is proposed. The results suggest that the cumulative assessment approach of IAQ is useful for monitoring the values of total amounts of indoor air pollutants, if indoor air pollutants accumulated for a long time, especially NO2 pollutants. The results obtained here confirm that the proposed method can be applied to monitor total amounts of indoor air pollutants emitted, inside apartments and hospitals as well.  相似文献   
790.
INTRODUCTION: Exposure to trace metals and polycyclic aromatic hydrocarbons (PAHs) adsorbed on particulates is of a serious health concern. Levels of some trace metals in total suspended particulate and 13 PAHs of fine particulate matter were measured from nomadic tents in the southern Tibetan Plateau in summer 2010. RESULTS AND DISCUSSION: The indoor air within the tents was seriously polluted, mainly due to yak dung combustion. Average trace metal concentrations were much higher (range of indoor/outdoor ratio 61-291) than those of the outdoor air. Additionally, enrichment factors of most trace metals of indoor air were similar to those of outdoor air, indicating outdoor air quality of the studied area was possibly influenced by pollutants emitted from local tents. Mean concentrations of total PAHs and BaP within tents was 5372.45 and 364.79 ng/m(3), hundred times higher than that of outdoor air of the Tibetan Plateau. Three- and four-ring PAHs were the predominant components. The diagnostic ratio of BaA/(BaA + Chr) was 0.33. Since Tibetan women typically spend longer time within the tents, they were exposed to PAHs (BaP exposure = 1.81 μg/m(3)) about two times of other family members. Among all the PAHs, Bap contributed the most (82.6%) of the total carcinogenicity. Similarly, the excess lifetime cancer risk for women and other family members were 2.75 × 10(-4) and 1.27 × 10(-4), respectively, indicating Tibetan herdsmen, especially women who are in charge of most house chores were at risk for adverse health effects.  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号