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431.
Trace element pollution records in some UK lake sediments, their history, influence factors and regional differences 总被引:8,自引:0,他引:8
Sediment cores were taken from six sites across the UK. Apart from Banbury Reservoir in London, all the other sites are relatively remote lakes. Trace elements Pb, Zn, Cu, Cd, Cr, Ni, Sn, As and V, major elements such as Fe, Mn, Ti and Al were analysed, and organic content measured as loss-on-ignition was determined in all of these cores. The result shows that these relatively remote sites have experienced enhanced atmospheric deposition of anthropogenically derived trace elements for over 100 years, and the contamination might start before industrialisation. Trace metal contamination remains the highest level at Banbury Reservoir showing "pollution source" influence. Despite the considerable reduction in atmospheric deposition in recent years, although some of the element concentrations in the surface sediments have declined, they are still much higher than their natural background values. In these sites, trace element pollution records have been influenced by many different factors. Redox condition could affect As distribution in the sediments. Sediment matrix could also affect trace element pollution signal. Apart from direct atmospheric deposition, the distributions of trace elements in the sediments have been affected by forestry activities and catchment erosion, and more contaminated soil in-wash could increase sediment pollution whilst less contaminated soil could dilute sediment pollution. In some sites, data suggest that catchment in-wash is an important source of elements for the lakes. 相似文献
432.
433.
Tapping the leakages: Methane losses, mitigation options and policy issues for Russian long distance gas transmission pipelines 总被引:1,自引:0,他引:1
Stefan Lechtenbhmer Carmen Dienst Manfred Fischedick Thomas Hanke Roger Fernandez Don Robinson Ravi Kantamaneni Brian Gillis 《International Journal of Greenhouse Gas Control》2007,1(4):387-395
The Russian natural gas industry is the world's largest producer and transporter of natural gas. This paper aims to characterize the methane emissions from Russian natural gas transmission operations, to explain projects to reduce these emissions, and to characterize the role of emissions reduction within the context of current GHG policy. It draws on the most recent independent measurements at all parts of the Russian long distance transport system made by the Wuppertal Institute in 2003 and combines these results with the findings from the US Natural Gas STAR Program on GHG mitigation options and economics.With this background the paper concludes that the methane emissions from the Russian natural gas long distance network are approximately 0.6% of the natural gas delivered. Mitigating these emissions can create new revenue streams for the operator in the form of reduced costs, increased gas throughput and sales, and earned carbon credits. Specific emissions sources that have cost-effective mitigation solutions are also opportunities for outside investment for the Joint Implementation Kyoto Protocol flexibility mechanism or other carbon markets. 相似文献
434.
Schmidt G Pesch R Schröder W Conrad A Kolossa-Gehring M Feigenspan S Dobler L Wiesmüller GA Birke M Utermann J 《Environmental geochemistry and health》2011,33(4):399-408
This study aimed at statistically investigating the association between the internal exposure of children and young adults
to uranium (U) and epidemiologically relevant external determinants of exposure. The investigation was performed with data
from two studies within the framework of the German health-related environmental monitoring program: The German Environmental Survey for Children (GerES IV) conducted by the Federal Environment Agency (Umweltbundesamt) with data on 1,780 children 3–14 years of age and their home environment and the German Environmental Specimen Bank (ESB, section: human specimens) with data on 2,253 students 20–29 years of age. Both studies provided data on the U levels in human urine for all probands.
GerES IV furthermore provided an extensive environmental and demographic database on, e.g., U levels in drinking water. The
data from GerES IV and ESB were linked by GIS to spatially relevant exposure information, including background values of U
in stream sediments and in upper and lower soils, U levels in mosses and particulate matter in the lower atmosphere, precipitation
and elevation as well as forest density. Bivariate correlation analysis and two decision tree models showed moderate but significant
associations between U in human urine and U levels in drinking water, stream sediments and upper and lower soils. Future investigations
considering additional epidemiologically relevant data sets may differentiate the results. Furthermore, the sample design
of future environmental epidemiology studies should take the spatial evaluation of the data into greater account. 相似文献
435.
Sujay S. Kaushal Paul M. Mayer Philippe G. Vidon Rose M. Smith Michael J. Pennino Tamara A. Newcomer Shuiwang Duan Claire Welty Kenneth T. Belt 《Journal of the American Water Resources Association》2014,50(3):585-614
Nonpoint source pollution from agriculture and urbanization is increasing globally at the same time climate extremes have increased in frequency and intensity. We review >200 studies of hydrologic and gaseous fluxes and show how the interaction between land use and climate variability alters magnitude and frequency of carbon, nutrient, and greenhouse gas pulses in watersheds. Agricultural and urban watersheds respond similarly to climate variability due to headwater alteration and loss of ecosystem services to buffer runoff and temperature changes. Organic carbon concentrations/exports increase and organic carbon quality changes with runoff. Nitrogen and phosphorus exports increase during floods (sometimes by an order of magnitude) and decrease during droughts. Relationships between annual runoff and nitrogen and phosphorus exports differ across land use. CH4 and N2O pulses in riparian zones/floodplains predominantly increase with: flooding, warming, low oxygen, nutrient enrichment, and organic carbon. CH4, N2O, and CO2 pulses in streams/rivers increase due to similar factors but effects of floods are less known compared to base flow/droughts. Emerging questions include: (1) What factors influence lag times of contaminant pulses in response to extreme events? (2) What drives resistance/resilience to hydrologic and gaseous pulses? We conclude with eight recommendations for managing watershed pulses in response to interactive effects of land use and climate change. 相似文献
436.
A pilot-scale, ponded wetland consisting of an open pond and a vegetated pond in series was constructed on a cotton farm in northern New South Wales, Australia, and assessed for its potential to remove pesticides from irrigation tailwater. Ten incubation periods ranging from 7 to 13 days each were conducted over two cotton growing seasons to monitor removal of residues of four pesticides applied to the crop. Residue reductions ranging 22–53% and 32–90% were observed in the first and second seasons respectively. Average half-lives during this first season were calculated as 21.3 days for diuron, 25.4 days for fluometuron and 26.4 days for aldicarb over the entire wetland. During the second season of monitoring, pesticide half-lives were significantly reduced, with fluometuron exhibiting a half-life of 13.8 days, aldicarb 6.2 days and endosulfan 7.5 days in the open pond. Further significant reductions were observed in the vegetated pond and also following an algal bloom in the open pond, as a result of which aldicarb and endosulfan were no longer quantifiable. Partitioning onto sediment was found to be a considerable sink for the insecticide endosulfan. These results demonstrate that macrophytes and algae can reduce the persistence of pesticides in on-farm water and provide some data for modelling. 相似文献
437.
Manfred Thönnessen 《Environmental Sciences Europe》2006,18(1):5-12