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71.
72.
Chester W. Spicer Michael W. Holdren Kenneth A. Cowen Darrell W. Joseph Jan Satola Bradley Goodwin Howard Mayfield Alexander Laskin M. Lizabeth Alexander John V. Ortega Matthew Newburn Robert Kagann Ram Hashmonay 《Atmospheric environment (Oxford, England : 1994)》2009,43(16):2612-2622
Aircraft emissions affect air quality on scales from local to global. More than 20% of the jet fuel used in the U.S. is consumed by military aircraft, and emissions from this source are facing increasingly stringent environmental regulations, so improved methods for quickly and accurately determining emissions from existing and new engines are needed. This paper reports results of a study to advance the methods used for detailed characterization of military aircraft emissions, and provides emission factors for two aircraft: the F-15 fighter and the C-130 cargo plane. The measurements involved outdoor ground-level sampling downstream behind operational military aircraft. This permits rapid change-out of the aircraft so that engines can be tested quickly on operational aircraft. Measurements were made at throttle settings from idle to afterburner using a simple extractive probe in the dilute exhaust. Emission factors determined using this approach agree very well with those from the traditional method of extractive sampling at the exhaust exit. Emission factors are reported for CO2, CO, NO, NOx, and more than 60 hazardous and/or reactive organic gases. Particle size, mass and composition also were measured and are being reported separately. Comparison of the emissions of nine hazardous air pollutants from these two engines with emissions from nine other aircraft engines is discussed. 相似文献
73.
Cora J. Young Michael D. Hurley Timothy J. Wallington Scott A. Mabury 《Atmospheric environment (Oxford, England : 1994)》2009,43(24):3717-3724
Relative rate techniques were used to determine k(Cl + CF3CFCFCF3) = (7.27 ± 0.88) × 10?12, k(Cl + CF3CF2CFCF2) = (1.79 ± 0.41) × 10?11, k(OH + CF3CFCFCF3) = (4.82 ± 1.15) × 10?13, and k(OH + CF3CF2CFCF2) = (1.94 ± 0.27) × 10?12 cm3 molecule?1 s?1 in 700 Torr of air or N2 diluent at 296 K. The chlorine atom- and OH radical-initiated oxidation of CF3CFCFCF3 in 700 Torr of air gives CF3C(O)F in molar yields of 196 ± 11 and 218 ± 20%, respectively. Chlorine atom-initiated oxidation of CF3CF2CFCF2 gives molar yields of 97 ± 9% CF3CF2C(O)F and 97 ± 9% COF2. OH radical-initiated oxidation of CF3CF2CFCF2 gives molar yields of 110 ± 15% CF3CF2C(O)F and 99 ± 8% COF2. The atmospheric fate of CF3CF2C(O)F and CF3C(O)F is hydrolysis to give CF3CF2C(O)OH and CF3C(O)OH. The atmospheric lifetimes of CF3CFCFCF3 and CF3CF2CFCF2 are determined by reaction with OH radicals and are approximately 24 and 6 days, respectively. The contribution of CF3CFCFCF3 and CF3CF2CFCF2 to radiative forcing of climate change will be negligible. 相似文献
74.
Elizabeth A. Stone Curtis J. Hedman Rebecca J. Sheesley Martin M. Shafer James J. Schauer 《Atmospheric environment (Oxford, England : 1994)》2009,43(27):4205-4213
The high-molecular weight water-soluble organic compounds present in atmospheric aerosols underwent functional-group characterization using liquid chromatography tandem mass spectrometry (LC-MS/MS), with a focus on understanding the chemical structure and origins of humic-like substances (HULIS) in the atmosphere. Aerosol samples were obtained from several locations in North America at times when primary sources contributing to organic aerosol were well-characterized: Riverside, CA, Fresno, CA, urban and peripheral Mexico City, Atlanta, GA, and Bondville, IL. Chemical analysis targeted identification and quantification of functional groups, such as aliphatic, aromatic, and bulk carboxylic acids, organosulfates, and carbohydrate-like substances that comprise species with molecular weights (MW) 200–600 amu. Measured high-MW functional groups were compared to modeled primary sources with the purpose of identifying associations between aerosol sources, high-MW aerosol species, and HULIS. Mobile source emissions were linked to high-molecular weight carboxylic acids, especially aromatic acids, biomass burning was associated with carboxylic acids and carbohydrate-like substances, and secondary organic aerosol (SOA) correlated well with the total amount of HULIS measured, whereas organosulfates showed no correlation with aerosol sources and exhibited unique spatial trends. These results suggested the importance of motor vehicles, biomass burning, and SOA as important sources of precursors to HULIS. Structural characteristics of atmospheric HULIS were compared to terrestrial humic and fulvic acids and revealed striking similarities in chemical structure, with the exception of organosulfates which were unique to atmospheric HULIS. 相似文献
75.
Castello L Viana JP Watkins G Pinedo-Vasquez M Luzadis VA 《Environmental management》2009,43(2):197-209
Fishers and small-scale fisheries worldwide have been marginalized historically. Now it is clear that integrating fishers
in management processes is key to resource conservation, but it is less clear how to do it. Here, based on a literature review and new information, we present and analyze a case in which the participation
of fishers in the management process was crucial in recovering an overexploited small-scale fishery for the pirarucu (Arapaima spp.) in the Amazon Basin, Brazil. In 8 years of experimental management, from 1999 to 2006, the population of pirarucu increased
9-fold (from about 2200 to 20,650 individuals), harvest quotas increased 10-fold (from 120 to 1249 individuals), and fishers’
participation in the management process increased and they benefited from increased monetary returns. Additionally, the number
of communities conducting the management scheme increased from 4 in 1999 to 108 in 2006, following the demands of fishers
and regional government agencies. Based on our analysis, we suggest that the participation of fishers in the management of
other small-scale fisheries in the world can be improved by focusing on (1) applying the knowledge and skills of fishers in
resource monitoring and management, (2) bridging knowledge systems among all involved stakeholders, (3) collaborating with
fishers that are interested in, and capable of conducting, resource conservation schemes, and (4) conducting management under
conditions of uncertainty. 相似文献
76.
Hegetschweiler KT van Loon N Ryser A Rusterholz HP Baur B 《Environmental management》2009,43(2):299-310
Urban forests are popular recreation areas in Europe. Several of these temperate broad-leaved forests also have a high conservation
value due to sustainable management over many centuries. Recreational activities, particularly the use of fireplaces, can
cause extensive damage to soil, ground vegetation, shrubs, and trees. Firewood collection depletes woody debris, leading to
a loss of habitat for specialized organisms. We examined the effects of fireplace use on forest vegetation and the amount
of woody debris by comparing disturbed and control plots in suburban forests in northwestern Switzerland. At frequently used
fireplaces, we found reduced species densities in the ground vegetation and shrub layer and changes in plant species composition
due to human trampling within an area of 150–200 m2. Picnicking and grilling also reduced the height and changed the age structure of shrubs and young trees. The amount of woody
debris was lower in disturbed plots than in control plots. Pieces of wood with a diameter of 0.6–7.6 cm were preferentially
collected by fireplace users. The reduction in woody debris volume extended up to a distance of 16 m from the fire ring, covering
an area of 800 m2 at each picnic site. In order to preserve the ecological integrity of urban forests and to maintain their attractiveness
as important recreation areas, we suggest depositing logging residues to be used as firewood and to restrict visitor movements
near picnic sites. 相似文献
77.
Zhao Ma Dennis R. Becker Michael A. Kilgore 《Journal of Environmental Planning and Management》2009,52(8):1035-1051
Following the intent of the National Environmental Policy Act of 1969, many states have adopted policies and procedures directing state agencies and local government units to evaluate the potential environmental impacts of development projects prior to their undertaking. In contrast to a rich literature on federal requirements, current understanding of state environmental review is narrowly focused and outdated. This paper seeks to provide information on the landscape of state environmental review policy frameworks. The paper identifies 37 states with formal environmental review requirements through a document review of state statutes, administrative rules and agency-prepared materials, and confirms this finding through a survey of state administrators. A two-tier classification is used to distinguish states based on the approach taken to address environmental review needs and the scope and depth of relevant policies and procedures implemented. This paper also provides a discussion of policy and programme attributes that may contribute to effective practice, and of the potential for adopting relevant legislation in states where environmental review is currently lacking. 相似文献
78.
Agri-environment programs aim to secure environmental and social stewardship services through payments to farmers. A critical
component of many agri-environment programs is an agri-environment index (AEI) used to quantify benefits and target investments.
An AEI will typically comprise multiple indicators, which are weighted and combined using a utility function, to measure the
benefit of investment options (e.g., projects, farms, regions). This article presents a review of AEIs with 11 case studies
from agri-environment programs in the United States, Australia, and the United Kingdom. We identify a generic procedure used
to define AEIs and explore the implications of alternative methodological approaches. We conclude that AEIs have become an
extremely important policy instrument and make suggestions for their improvement. 相似文献
79.
Jason A. Dittman James B. Shanley George R. Aiken Janet E. Towse 《Environmental pollution (Barking, Essex : 1987)》2009,157(6):1953-1956
Stream water samples were collected over a range of hydrologic and seasonal conditions at three forested watersheds in the northeastern USA. Samples were analyzed for dissolved total mercury (THgd), DOC concentration and DOC composition, and UV254 absorbance across the three sites over different seasons and flow conditions. Pooling data from all sites, we found a strong positive correlation of THgd to DOC (r2 = 0.87), but progressively stronger correlations of THgd with the hydrophobic acid fraction (HPOA) of DOC (r2 = 0.91) and with UV254 absorbance (r2 = 0.92). The strength of the UV254 absorbance-THgd relationship suggests that optical properties associated with dissolved organic matter may be excellent proxies for THgd concentration in these streams. Ease of sample collection and analysis, the potential application of in-situ optical sensors, and the possibility for intensive monitoring over the hydrograph make this an effective, inexpensive approach to estimate THgd flux in drainage waters. 相似文献
80.
On experimental setup in bioelectromagnetics 总被引:1,自引:1,他引:0
Bioeffects created by electromagnetic field (EMF) are the subject of intensive studies. This paper critically considers estimations
of exposure to EMF in bioelectromagnetic experiments. Results of calculations presented herein show the significant role of
the presence of conducting bodies (the exposure system) near an object under test on EMF energy absorption as well as mutual
interactions between simultaneously exposed objects. Our aims herein are twofold: firstly to find a way to refer measurement
results to free-space conditions in order to enable comparison of results obtained in different laboratories, and secondly
to show that EMF energy absorption in any exposed object is different and that this difference is a function of the size of
the exposure system, the number of exposed objects, and the particular properties (i.e., the electromagnetic structure) of
the objects. In the authors’ opinion the existence of interactions caused by the presence of the exposure system and other
exposed objects is a reason why remarkable differences are observed between experiments performed even under supposedly identical
conditions. The presented considerations and conclusion suggest wider participation of physicists and engineers in bioelectromagnetic
experiments in order to ensure the correctness of metrological aspects of these experiments. 相似文献