全文获取类型
收费全文 | 18811篇 |
免费 | 190篇 |
国内免费 | 171篇 |
专业分类
安全科学 | 516篇 |
废物处理 | 751篇 |
环保管理 | 2531篇 |
综合类 | 3004篇 |
基础理论 | 4962篇 |
环境理论 | 6篇 |
污染及防治 | 5026篇 |
评价与监测 | 1229篇 |
社会与环境 | 1024篇 |
灾害及防治 | 123篇 |
出版年
2022年 | 195篇 |
2021年 | 226篇 |
2020年 | 149篇 |
2019年 | 185篇 |
2018年 | 320篇 |
2017年 | 317篇 |
2016年 | 463篇 |
2015年 | 311篇 |
2014年 | 459篇 |
2013年 | 1421篇 |
2012年 | 555篇 |
2011年 | 786篇 |
2010年 | 639篇 |
2009年 | 611篇 |
2008年 | 797篇 |
2007年 | 793篇 |
2006年 | 724篇 |
2005年 | 611篇 |
2004年 | 728篇 |
2003年 | 666篇 |
2002年 | 573篇 |
2001年 | 771篇 |
2000年 | 499篇 |
1999年 | 315篇 |
1998年 | 254篇 |
1997年 | 239篇 |
1996年 | 241篇 |
1995年 | 268篇 |
1994年 | 288篇 |
1993年 | 227篇 |
1992年 | 257篇 |
1991年 | 234篇 |
1990年 | 261篇 |
1989年 | 247篇 |
1988年 | 197篇 |
1987年 | 181篇 |
1986年 | 166篇 |
1985年 | 175篇 |
1984年 | 202篇 |
1983年 | 192篇 |
1982年 | 190篇 |
1981年 | 186篇 |
1980年 | 137篇 |
1979年 | 161篇 |
1978年 | 133篇 |
1977年 | 120篇 |
1975年 | 121篇 |
1974年 | 116篇 |
1973年 | 110篇 |
1972年 | 133篇 |
排序方式: 共有10000条查询结果,搜索用时 546 毫秒
121.
Georgios D. Gikas Trisevgeni Yiannakopoulou Vassilios A. Tsihrintzis 《Environmental Modeling and Assessment》2006,11(3):219-233
SWAT ver. 2000 was used to predict hydrographs, and sediment, nitrate and total phosphorus loadings from a 1349 km2 mountainous/agricultural watershed in Northern Greece. The model was calibrated and verified using continuous meteorological
data from eight stations within the drainage area, and runoff, sediment and nutrient concentrations measured at nine stations
located within the main tributaries of the watershed, for the time period from May 1st, 1998 to January 31st, 2000. Model
validation methodology and resulting input parameters appropriate for Mediterranean drainage basins are presented. Predicted
by the model hydrographs, sedimentographs and pollutographs are plotted against observed values and show good agreement. Model
performance is evaluated using the root mean square error computation and scattergrams of predicted versus observed data.
The validated model is also used to test the effectiveness of three alternative cropping scenarios in reducing nutrient loadings
from the agricultural part of the watershed. The study showed that this model, if properly validated, can be used effectively
in testing management scenarios in Mediterranean drainage basins. 相似文献
122.
Sewage sludge dumped at Garroch Head in the Firth of Clyde contains significant quantities of chlorinated hydrocarbons, such as polychlorinated biphenyls (CBs). These compounds are lipophilic and resistant to degradation. They accumulate in the biota either from the water column or through the food chain, particularly in tissue with a high lipid content. Bottom dwelling fish, such as plaice, in the vicinity of the dump site will accumulate CBs from their environment. Eighteen of the 209 CBs were measured in plaice livers from the Garroch Head dump site and from Pladda, a site reasonably remote from the dump site but also in the Clyde, over a 7 year period prior to the cessation of dumping in December 1998. Concentrations of the congeners in the liver of fish caught at the dump site were, in general, higher than those in the liver of fish caught at Pladda. Concentrations in the plaice livers for the sum of 18 CBs ranged from 1611 to 8471 micrograms kg-1 lipid for Garroch Head samples and from 336.9 to 2635 micrograms kg-1 lipid for samples from Pladda. The data were evaluated using principal component analysis (PCA). Pattern analysis was undertaken by normalising to the recalcitrant CB 153. Livers from the dump site were found to have a higher proportion of the lower chlorinated CBs. CB patterns were similar at the Garroch Head dump site from year to year, but multivariate techniques showed that there were differences in pattern when normalised to CB 153. 相似文献
123.
Brito JA McNeill FE Chettle DR Webber CE Vaillancourt C 《Journal of environmental monitoring : JEM》2000,2(3):271-276
The study aims were to: (i) investigate long term human lead metabolism by measuring the change of lead concentration in the tibia and calcaneus; and (ii) assess whether improved industrial hygiene was resulting in a slow accumulation of lead in an exposed workforce. 109Cd excited K X-ray fluorescence was used to measure tibia lead and calcaneus lead concentrations in 101 workers in a secondary lead smelter. 51 subjects had had similar bone lead measurements 5 years previously. Most of the other subjects had been hired since the first survey. Measurements of whole blood lead were available for the large majority of subjects. Tibia lead concentrations fell significantly (p<0.001) in the 51 subjects with repeated bone lead measurements, from a mean of 39 microg Pb (g bone mineral)(-1) to 33 microg Pb (g bone mineral)(-1). The change correlated negatively with the initial tibia lead concentration, producing an estimate for an overall half-life of 15 years, with a 95% confidence interval of 9 to 55 years. Adding continuing lead exposure and recirculation of bone lead stores to the regression models produced half-life estimates of 12 and 9 years, respectively, for release of lead from the tibia. The repeat subjects showed no net change in calcaneus lead (64 microg Pb (g bone mineral)(-1) initially, 65 microg Pb (g bone mineral)(-1) 5 years later). Subjects not measured previously had average lead concentrations of 15 microg Pb (g bone mincral)(-1) in the tibia and 13 microg Pb (g bone mineral)(-1) in the calcaneus. The rate of clearance of lead from the tibia (9 to 15 years) is towards the more rapid end of previous estimates. The lack of a significant fall in the calcaneus lead was surprising. Attempts should be made to repeat this observation. If confirmed, it would have implications for models of lead metabolism. The relatively low lead concentrations in the non-repeat subjects are reassuring. However, observation after a longer period of employment would be desirable. 相似文献
124.
Young northern pike,yellow perch and crayfish as bioindicators in a mercury contaminated watercourse 总被引:2,自引:0,他引:2
J. W. Parks C. Curry D. Romani D. D. Russell 《Environmental monitoring and assessment》1991,16(1):39-73
Young-of-the-year and yearling northern pike (Esox lucius), yearling yellow perch (Perca flavescens) and adult crayfish (Orconectes virilis) were collected in the mercury-contaminated Wabigoon/English/Winnipeg River System, Ontario, and analyzed for total mercury. Analysis of mercury concentrations in these organisms produced consistent geographical trends; i.e. mercury concentrations in biota downstream of Dryden > English River system > Winnipeg River system > control sites. In the Wabigoon River system the bioavailability of mercury increases with distance downstream of the historical point source. Mercury concentrations in the biota studied were highly correlated with mercury concentrations in fish species which are of sport and commercial interest. The locations where young fish obtain their bodyburdens are known typically within 100 m. The biota studied compare favourably with the criteria proposed by Phillips (1980) as prerequisites for biological indicators. The wide distribution of young pike, perch and crayfish in North America, Europe and Asia may enhance their appeal as biomonitors.The views expressed are those of the authors and do not necessarily reflect the views of the Ontario Ministry of the Environment. No endorsement should be inferred. 相似文献
125.
J. E. Elliott D. G. Noble R. J. Norstrom P. E. Whitehead 《Environmental monitoring and assessment》1989,12(1):67-82
Eggs were collected from seven seabird species at colonies on the British Columbia coast from 1983 to 1986 and analyzed for organochlorine contaminants. Total PCB levels (wet weight) were highest in double-crested cormorants (Phalacrocorax auritus) from the Fraser estuary (2.91 mg kg-1) and the Strait of Georgia (3.79 mg kg-1). Highest DDE levels were in fork-tailed storm-petrels (Oceanodroma furcata) from the Queen Charlotte Islands (1.68 mg kg-1). Organochlorine levels were generally lower in eggs from the mid 1980s than in those collected in the early 1970s. Organochlorine levels in Pacific alcids and hydrobatids foraging in offshore locations were compared to those in the same or ecologically similar species from the Canadian Atlantic coast. DDT- and HCH-related compounds were higher in Pacific populations while levels of dieldrin, oxychlordane, and HCB were generally lower. With the exception of -HCH, levels of all measured organochlorines were lower in cormorants breeding in the Fraser River estuary than in cormorants from the St. Lawrence River estuary on the Atlantic coast. 相似文献
126.
Edward D. Goldberg 《Environmental monitoring and assessment》1988,11(3):293-298
Information needed for the resolution of environmental problems is a commodity with an economic value. The minimum necessary information implies minimal costs. The formulation of the information is considered for the case of biocides that can disrupt marine ecosystems. 相似文献
127.
Morgenstern P Versteegh AF de Korte GA Hoogerbrugge R Mooibroek D Bannink A Hogendoorn EA 《Journal of environmental monitoring : JEM》2003,5(6):885-890
An indicative survey has been carried out in The Netherlands investigating the presence of methyl tertiary butyl ether (MTBE) in drinking water and the corresponding sources. In total, 71 different sites used for the preparation of drinking water in The Netherlands were sampled in two successive seasons in 2001 involving the analysis of 156 samples. (ground water (n = 88), surface water (n = 17), bank filtrate water (n = 6) and drinking water (n = 45)). To combine high sample throughput with high selectivity and sensitivity, off-line purge and trap for sampling and gas chromatography mass spectrometry equipped with an automated thermal desorption sampler (TDS-GC-MS) was selected as the preferred analytical methodology. The developed procedure enabled the analysis of at least 40 samples per day and provided a limit of quantification of 2 ng l(-1). In the first period 63 samples of raw water were analyzed. Concentrations ranged between < 10 ng l(-1) and 420 ng l(-1) with a median concentration below 10 ng l(-1). The second period was focused at the re-sampling of positive locations (MTBE > 10 ng l(-1)) and a few additional drinking water utilities of which both the raw and drinking water of the utilities were analyzed. The median concentration of MTBE in the selected set of drinking water samples was 20 ng l(-1) (n = 45). At one location MTBE was found at a level of 2900 ng l(-1) caused by point source contamination of the ground water (11 900 ng l(-1)). Special attention has been paid to the quality of the results by analyzing all samples in duplicate and the analysis of control samples during each series of analyses. 相似文献
128.
Ponce de León CA DeNicola K Montes Bayón M Caruso JA 《Journal of environmental monitoring : JEM》2003,5(3):435-440
Different techniques have been employed in order to evaluate the most efficient procedure for the extraction of selenium from soil as required for speciation. Selenium contaminated sediments from Stewart Lake Wetland, California were used. A strong acid mineralization of the samples gives quantitative total selenium, which is then used to estimate recoveries for the milder extraction methods. The different extraction methodologies involve the sequential use of water, buffer (phosphate, pH 7) and either acid solution (e.g. HNO3 or HCl) or basic solutions (e.g. ammonium acetate, NaOH or TMAH). Pyrophosphate extraction was also evaluated and showed that selenium was not associated with humic acids. The extractants were subsequently analyzed by size exclusion chromatography (SEC) with UV (254 and 400 nm) and on-line ICP-MS detection; anion exchange chromatography, and ion-pair reversed phase chromatography with ICP-MS detection. For sequential extractions the extraction efficiencies showed that the basic extractions were more efficient than the acidic. The difference between the acidic and the basic extraction efficiency is carried to the sulfite extraction, suggesting that whatever is not extracted by the acid is subsequently extracted by the sulfite. The species identified with the different chromatographies were selenate, selenite, elemental selenium and some organic selenium. 相似文献
129.
Biomass burning, in a broad sense, encompasses different burning practices, including open and confined burnings, and different types of vegetation. Emission factors of gaseous or particulate trace compounds are directly dependent both on the fuel type and the combustion process. Emission factors are generally calculated by stoichiometric considerations using the carbon mass balance method, applied either to combustion chamber experiments or to field experiments based on ground-level measurements or aircraft sampling in smoke plumes. There have been a number of experimental studies in the last 10 years to investigate wildfires in tropical, temperate, or boreal regions. This article presents an overview of measurement methods and experimental data on emission factors of reactive or radiatively active trace compounds, including trace gases and particles. It focuses on fires in tropical regions, that is, forest and savanna fires, agricultural burns, charcoal production, use of fuelwood, and charcoal combustion. 相似文献
130.
V. M. Artyomov E. M. Artyomov Sh. D. Fridman 《Environmental monitoring and assessment》1994,29(3):221-228
The paper considers the methodology and results of experimental determination of dry deposition and ammonia uptake by isolated plant leaves. Analytical expressions are proposed which allow a transition from rates obtained in an isolated chamber to dry ammonia deposition by standing crops leaves. 相似文献