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1.
Magnuson ML Kelty CA Urbansky ET Owens JH Kelty KC Speth TF 《Journal of environmental monitoring : JEM》2002,4(1):102-108
Analytical chemistry is an important tier of environmental protection and has been traditionally linked to compliance and/or exposure monitoring activities for environmental contaminants. The adoption of the risk management paradigm has led to special challenges for analytical chemistry applied to environmental risk analysis. Namely, methods developed for regulated contaminants may not be appropriate and/or applicable to risk management scenarios. This paper contains examples of analytical chemistry applied to risk management challenges broken down by the analytical approach and analyte for some selected work in our laboratory. Specific techniques discussed include stable association complex electrospray mass spectrometry (cESI-MS), gas chromatography-mass spectrometry (GC-MS), split-flow thin cell (SPLITT) fractionation and matrix-assisted laser desorption time of flight mass spectrometry (MALDI-ToF-MS). Specific analytes include haloacetic acids (HAA9), perchlorate, bromate, triazine degradation products, metal-contaminated colloids and Cryptosporidium parvum oocysts. 相似文献
2.
Habibiandehkordi Reza Lobb David A. Sheppard Steve C. Flaten Don N. Owens Philip N. 《Environmental science and pollution research international》2017,24(22):18372-18382
Environmental Science and Pollution Research - Vegetated buffer strips (VBSs) are widely encouraged as a cost-effective strategy to address phosphorus (P) pollution associated with agricultural... 相似文献
3.
JoAnn S. Lighty Robert M. Britt David W. Pershing Warren D. Owens Vic A. Cundy 《Journal of the Air & Waste Management Association (1995)》2013,63(2):187-193
With landfill costs increasing and regulations on landfilling becoming more stringent, alternatives to conventional hazardous waste treatment strategies are becoming more desirable. Incineration Is presently a permanent, proven solution for the disposal of most organic contaminants, but also a costly one, especially in the case of solids which require some auxiliary fuel. The goal of this research is to develop an understanding of the phenomena associated with the evolution of contaminants from solids In the primary combustor of an Incineration system. A four-fold approach is being used. First, a bench-scale particle characterization reactor was developed to study the transport phenomena on a particle basis, where the controlling processes are mainly intraparticle. Second, a bed-characterization reactor was built to examine the controlling transport phenomena within a bed of particles, where the processes are primarily interparticle. The results of these studies can be applied to any primary combustor. A pilot-scale rotary kiln was developed to study the evolution of contaminants from solids within a realistic temperature and rotation environment. Finally, in situ measurements are being obtained from a full-scale rotary-kiln. This paper describes results obtained in a study using a commercial sorbent contaminated with toluene. The data are from the particle-characterization reactor and the rotary-kiln simulator. The results show that the method of contamination and charge size do not have a large effect on desorption, while temperature and contaminant concentration are important parameters In the evolution of contaminants in a rotary kiln. 相似文献
4.
Fang J Shan XQ Wen B Lin JM Owens G Zhou SR 《Environmental pollution (Barking, Essex : 1987)》2011,159(5):1248-1256
The effects of TiO2 nanoparticles on the transport of Cu through four different soil columns were studied. For two soils (HB and DX), TiO2 nanoparticles acted as a Cu carrier and facilitated the transport of Cu. For a third soil (BJ) TiO2 nanoparticles also facilitated Cu transport but to a much lesser degree, but for a fourth soil (HLJ) TiO2 nanoparticles retarded the transport of Cu. Linear correlation analysis indicated that soil properties rather than sorption capacities for Cu primary governed whether TiO2 nanoparticles-facilitated Cu transport. The TiO2-associated Cu of outflow in the Cu-contaminated soil columns was significantly positively correlated with soil pH and negatively correlated with CEC and DOC. During passage through the soil columns 46.6-99.9% of Cu initially adsorbed onto TiO2 could be “stripped” from nanoparticles depending on soil, where Cu desorption from TiO2 nanoparticles increased with decreasing flow velocity and soil pH. 相似文献
5.
Owens LB Barker DJ Loerch SC Shipitalo MJ Bonta JV Sulc RM 《Journal of environmental quality》2012,41(1):106-113
Pasture management practices can affect forage quality and production, animal health and production, and surface and groundwater quality. In a 5-yr study conducted at the North Appalachian Experimental Watershed near Coshocton, Ohio, we compared the effects of two contrasting grazing methods on surface and subsurface water quantity and quality. Four pastures, each including a small, instrumented watershed (0.51-1.09 ha) for surface runoff measurements and a developed spring for subsurface flow collection, received 112 kg N ha(-1) yr(-1) and were grazed at similar stocking rates (1.8-1.9 cows ha(-1)). Two pastures were continuously stocked; two were subdivided so that they were grazed with frequent rotational stocking (5-6 times weekly). In the preceding 5 yr, these pastures received 112 kg N ha(-1) yr(-1) after several years of 0 N fertilizer and were grazed with weekly rotational stocking. Surface runoff losses of N were minimal. During these two periods, some years had precipitation up to 50% greater than the long-term average, which increased subsurface flow and NO(3)-N transport. Average annual NO(3)-N transported in subsurface flow from the four watersheds during the two 5-yr periods ranged from 11.3 to 22.7 kg N ha(-1), which was similar to or less than the mineral-N received in precipitation. Flow and transport variations were greater among seasons than among watersheds. Flow-weighted seasonal NO(3)-N concentrations in subsurface flow did not exceed 7 mg L(-1). Variations in NO(3)-N leached from pastures were primarily due to variable precipitation rather than the effects of continuous, weekly rotational, or frequent rotational stocking practices. This suggests that there was no difference among these grazing practices in terms of NO(3)-N leaching. 相似文献
6.
Respiration and physiological state in marine bacteria 总被引:3,自引:0,他引:3
The relationship between oxygen consumption (R) and respiratory electron-transport-system (ETS) activity was investigated in batch cultures of 5 species of marine bacteria, Vibrio adaptatus, V. anguillarum, a partially identified Vibrio sp. SA774, Serratia marinorubra, and Pseudomonas perfectomarinus. Although cellular levels of R and ETS varied widely among the species tested, the R:ETS ratios for growing or senescent populations were relatively constant among the species; these ratios were 5.02 in growth and 0.426 in senescence, with coefficients of variation of 29 and 20%, respectively. The lower senescent-phase R:ETS ratio was due to a depression of the respiration rates following growth termination. The regression log (R per cell) = 0.832 log (ETS per cell) + 0.727 for the growing populations was similar to that determined for marine zooplankton. The slight dependency of the R:ETS ratio on organism dry weight found for zooplankton was supported by our data. Planktonic respiration rates estimated from measured ETS-depth profiles in the eastern tropical North Pacific Ocean using the senescent-phase R:ETS ratio were similar to published oxygen consumption rates in the deep sea.Contribution No. M79-61 from the University of Washington's Department of Oceanography, and No. 79032 from the Bigelow Laboratory for Ocean Sciences. 相似文献
7.
J.?C.?MatanoskiEmail author R.?R.?Hood R.?L.?Owens J.?E.?Purcell 《Marine Biology》2004,145(2):303-313
Behavior is commonly studied at the group level using several individuals, but there is increasing evidence that the behavior of a few individuals often has a disproportionate effect on the response of a population to its environment. The present study used a suite of statistical techniques, random series analysis, analysis of variance, spectral analysis, and goodness-of-fit tests of frequency histograms, to quantitatively describe the time-dependent changes in individual behavior. Each technique reveals a different facet of the behavior and, when simultaneously applied to the data, distinguishes significant differences among the behaviors of several individuals. The approach was developed and tested on the swimming behavior of four specimens of the scyphomedusa Aurelia aurita (Linnaeus, 1758), which were observed for 19 days, beginning 16 January 1998, and videotaped under identical environmental conditions during that period. The analyses showed that each medusa swam in a unique pattern, varying swimming at characteristic frequencies. Application of the approach to individual-based numerical modeling, to the role of endogenous stimuli in the behavioral repertoire, and to in situ studies of animal behavior is discussed.Communicated by J.P. Grassle, New Brunswick 相似文献
8.
Ravi Naidu Euan Smith S. M. Imamul Huq Gary Owens 《Environmental geochemistry and health》2009,31(Z1):61-68
The bioavailability of arsenic (As) in the soil environment is largely governed by its adsorption–desorption reactions with
soil constituents. We have investigated the sorption–desorption behaviour of As in four typical Bangladeshi soils subjected
to irrigation with As-contaminated groundwater. The total As content of soils (160 samples) from the Laksham district ranged
from <0.03 to approximately 43 mg kg−1. Despite the low total soil As content, the concentration of As in the pore water of soils freshly irrigated with As-contaminated
groundwater ranged from 0.01 to 0.1 mg l−1. However, when these soils were allowed to dry, the concentration of As released in the pore water decreased to undetectable
levels. Remoistening of soils to field moisture over a 10-day period resulted in a significant (up to 0.06 mg l−1) release of As in the pore water of soils containing >10 mg As kg−1 soil, indicating the potential availability of As. In soils containing <5 mg As kg−1, As was not detected in the pore water. A comparison of Bangladeshi soils with strongly weathered long-term As-contaminated
soils from Queensland, Australia showed a much greater release of As in water extracts from the Australian soils. However,
this was attributed to the much higher loading of As in these Australian soils. The correlation of pore water As with other
inorganic ions (P, S) showed a strongly significant (P < 0.001) relationship with P, although there was no significant relationship between As and other inorganic cations, such
as Fe and Mn. Batch sorption studies showed an appreciable capacity for both AsV and AsIII sorption, with AsV being retained in much greater concentrations than AsIII. 相似文献
9.
C. B. Leger V. A. Cundy A. M. Sterling A. N. Montestruc A. L. Jakway W. D. Owens 《补救:环境净化治理成本、技术与工艺杂志》1991,1(3):275-291
There currently exists a need for better characterization and simulation of the processes that occur during the incineration of hazardous wastes in the environment of a rotary kiln. Addressing this need, a comprehensive research program was formed with the goal of developing a rudimentary predictive capability for rotary kiln incineration of hazardous wastes. This comprehensive program is headed by Louisiana State University and includes interaction with the University of Utah and also various industrial participants. Such cooperation allows use of laboratory, pilot, and field scale equipment. While laboratory scale experiments provide the necessary decoupling of complex phenomena and a high degree of experimental control, and pilot scale studies provide more realism at the expense of experimental control, the problems of scale-up make generalization of results to field scale units very tenuous. The unique aspect of the LSU program is the coupling of the laboratory and pilot scale units with afield scale unit in order to overcome these generalizations. In this study, plastic packs containing a mixture of toluene and sorbent were fed to a field-scale rotary kiln incinerator at a rate of one pack every 10 minutes. Selected continuous gas samples and temperatures were obtained from the exit of the rotary kiln, from the afterburner, and from the stack. These measurements were obtained during various operating conditions. These data provide, for the first time, an ability to compare conditions in the kiln to simultaneous conditions in the afterburner and stack. This paper outlines several new experimental features of our field-scale tests conducted in October 1990. Oxygen responses from the kiln, the afterburner, and the stack are compared during various operating conditions. 相似文献
10.