全文获取类型
收费全文 | 20341篇 |
免费 | 158篇 |
国内免费 | 126篇 |
专业分类
安全科学 | 374篇 |
废物处理 | 906篇 |
环保管理 | 2463篇 |
综合类 | 2976篇 |
基础理论 | 6054篇 |
环境理论 | 4篇 |
污染及防治 | 4577篇 |
评价与监测 | 1411篇 |
社会与环境 | 1768篇 |
灾害及防治 | 92篇 |
出版年
2022年 | 126篇 |
2021年 | 105篇 |
2020年 | 100篇 |
2019年 | 106篇 |
2018年 | 715篇 |
2017年 | 709篇 |
2016年 | 722篇 |
2015年 | 316篇 |
2014年 | 458篇 |
2013年 | 1202篇 |
2012年 | 672篇 |
2011年 | 1369篇 |
2010年 | 975篇 |
2009年 | 1010篇 |
2008年 | 1223篇 |
2007年 | 1487篇 |
2006年 | 589篇 |
2005年 | 595篇 |
2004年 | 548篇 |
2003年 | 598篇 |
2002年 | 613篇 |
2001年 | 660篇 |
2000年 | 485篇 |
1999年 | 257篇 |
1998年 | 190篇 |
1997年 | 206篇 |
1996年 | 205篇 |
1995年 | 236篇 |
1994年 | 234篇 |
1993年 | 180篇 |
1992年 | 195篇 |
1991年 | 183篇 |
1990年 | 203篇 |
1989年 | 187篇 |
1988年 | 151篇 |
1987年 | 162篇 |
1986年 | 153篇 |
1985年 | 156篇 |
1984年 | 158篇 |
1983年 | 143篇 |
1982年 | 125篇 |
1981年 | 120篇 |
1980年 | 115篇 |
1979年 | 124篇 |
1978年 | 100篇 |
1977年 | 113篇 |
1975年 | 87篇 |
1974年 | 87篇 |
1973年 | 96篇 |
1972年 | 86篇 |
排序方式: 共有10000条查询结果,搜索用时 125 毫秒
881.
Long-term survey of heavy-metal pollution, biofilm contamination and diatom community structure in the Riou Mort watershed, South-West France 总被引:4,自引:0,他引:4
Morin S Duong TT Dabrin A Coynel A Herlory O Baudrimont M Delmas F Durrieu G Schäfer J Winterton P Blanc G Coste M 《Environmental pollution (Barking, Essex : 1987)》2008,151(3):532-542
In a metal-polluted stream in the Riou Mort watershed in SW France, periphytic biofilm was analyzed for diatom cell densities and taxonomic composition, dry weight and metal bio-accumulation (cadmium and zinc). Periphytic diatom communities were affected by the metal but displayed induced tolerance, seen through structural impact (dominance of small, adnate species) as well as morphological abnormalities particularly in the genera Ulnaria and Fragilaria. Species assemblages were characterized by taxa known to occur in metal-polluted environments, and shifts in the community structure expressed seasonal patterns: high numbers of Eolimna minima, Nitzschia palea and Pinnularia parvulissima were recorded in Summer and Autumn, whereas the species Surirella brebissonii, Achnanthidium minutissimum, Navicula lanceolata and Surirella angusta were dominant in Winter and Spring. Commonly used indices such as the Shannon diversity index and Specific Pollution Sensitivity Index reflected the level of pollution and suggest seasonal periodicity, the lowest diversities being observed in Summer. 相似文献
882.
Fuga A Saiki M Marcelli MP Saldiva PH 《Environmental pollution (Barking, Essex : 1987)》2008,151(2):334-340
The Canoparmelia texana epiphytic lichenized fungi was used to monitor atmospheric pollution in the S?o Paulo metropolitan region, SP, Brazil. The cluster analysis applied to the element concentration values confirmed the site groups of different levels of pollution due to industrial and vehicular emissions. In the distribution maps of element concentrations, higher concentrations of Ba and Mn were observed in the vicinity of industries and of a petrochemical complex. The highest concentration of Co found in lichens from the S?o Miguel Paulista site is due to the emissions from a metallurgical processing plant that produces this element. For Br and Zn, the highest concentrations could be associated both to vehicular and industrial emissions. Exploratory analyses revealed that the accumulation of toxic elements in C. texana may be of use in evaluating the human risk of cardiopulmonary mortality due to prolonged exposure to ambient levels of air pollution. 相似文献
883.
Jörg Luster Manoj Menon Sandra Hermle Rainer Schulin Madeleine S. Günthardt-Goerg Bernd Nowack 《Water, Air, & Soil Pollution: Focus》2008,8(2):163-176
Soil translocation for recultivation of soil removed from construction sites and for the preparation of refilled lysimeters
inevitably involves disturbance of soil structure, and, if intermediate storage is included, also drying and rewetting of
the soil. We report on an experiment with model forest ecosystems, where uncontaminated forest subsoils were covered with
non-contaminated or freshly heavy metal (mainly Zn and Cu) contaminated topsoil in large lysimeters. Monitoring of the chemical
composition of the drainage water revealed two distinct soil conditioning phases. During an initial phase of about a year
strongly elevated nitrate and sulfate concentrations occurred that were attributed to a mineralisation flush caused by the
increased accessability of mineralisable nitrogen and sulfur in destroyed aggregates. These effects were significantly larger
in lysimeters with calcareous subsoil than in those with acidic subsoil. The second phase was characterised by a gradual decrease
in dissolved organic carbon and sulfate concentrations, in particular in the acidic subsoil. This decrease may be attributed
to the depletion of pools made accessible during aggregate destruction or the formation of new aggregates. These chemical
changes had only little effects on the concentrations of copper and zinc in the drainage water. Based on our results, it can
be concluded that large refilled lysimeters can be used for many purposes without risk of compromised results, if a conditioning
phase of about 1 year with sufficiently moist soil conditions is respected. Nevertheless, gradual changes in soil chemical
characteristics still occur after this initial phase. Implications for the recultivation of sites using relocated soils are
discussed. 相似文献
884.
885.
Increased salinity in spawning and nursery grounds in the Savannah River estuary was cited as the primary cause of a 97% decrease
in adult striped bass (Morone saxatilis) and a concomitant 96% decrease in striped bass egg production. Restoration efforts focused on environmental remediation
and stock enhancement have resulted in restored salinity patterns and increased egg and adult abundances. However, future
water needs or harbor development may preclude further recovery by reducing freshwater inflow or increasing salinity intrusion.
To assess the effect of potential changes in the salinity regime, we developed models relating discharge, tidal phase, and
salinity to striped bass egg and early larval survival and re-cast these in a quantitative Bayesian belief network. The model
indicated that a small upstream shift (≤1.67 km) in the salinity regime would have the least impact on striped bass early
life history survival, whereas shifts >1.67 km would have progressively larger impacts, with a 8.33-km shift potentially reducing
our estimated survival probability by >28%. Such an impact could have cumulative and long-term detrimental effects on the
recovery of the Savannah River striped bass population. The available salinity data were collected during average and low
flows, so our model represents some typical and some extreme conditions during a striped bass spawning season. Our model is
a relatively simplistic, “first-order” attempt at evaluating potential effects of changes in the Savannah River estuarine
salinity regime and points to areas of concern and potential future research. 相似文献
886.
887.
Cadmium stress alters gene expression of DNA mismatch repair related genes in Arabidopsis seedlings 总被引:1,自引:0,他引:1
Cadmium (Cd) is a non essential element, and is a widespread environmental pollutant. Exposure to Cd can result in a variety of adverse health effects in plant and humans. In the current study, Arabidopsis seedlings were used as a bio-indicator of Cd pollution. Seedlings were grown on MS media containing 0-6.0 mg L(-1) Cd for 18 days, and the gene expression patterns were used to link increased Cd exposure with progressive biological effects. Reduction of total soluble protein content in shoots of the Arabidopsis seedlings occurred with increase in Cd concentrations. For the gene expression patterns, seven genes known to be involved in cell division and DNA mismatch repair (MMR) system were investigated by semi-quantitative RT-PCR, and normalized using 18S rRNA gene expression. Expression of the proliferating cell nuclear antigen 2 (atPCNA 2), MutS 3 homolog (atMSH 3) and MutL1 homolog (atMLH1) genes in shoots of Arabidopsis was strongly induced by exposure to 0.75 mg L(-1) Cd, but were repressed by other Cd concentrations whereas exposure to 0.75-6 mg L(-1) of Cd resulted in a decreased expression of atPCNA1, atMSH 2, 6 and 7 genes independently of any observable biological effects, including survival, fresh weight and chlorophyll level of shoots. This work demonstrated that specific gene expression changes could serve as useful molecular biomarkers indicative of Cd exposure and related biological effects. 相似文献
888.
Ozonation of pentachlorophenol in unsaturated soils 总被引:1,自引:0,他引:1
A heterogeneous model was developed to describe interactions between ozone and hydrophobic organic compounds, exemplified by pentachlorophenol, in highly gas-saturated vadose zones where water moisture was limited to a thin film on soil particle surfaces. The soil was assumed to be free of soil organic matter. The model included a set of transient equations considering diffusion with simultaneous chemical reaction and hydrophobic partitioning. From dimensionless analysis, it was found that the film concentrations of ozone and the hydrophobic organic component were dependent on the Damk?hler numbers. Effects of Damk?hler numbers on the film profiles of components were examined. With the interfacial flux of ozone calculated from film profiles, dimensionless governing equations of ozone transport and contaminant removal across an experimental column were established. These equations were dependent on the Stanton number. One-dimensional column experiments were conducted to test the model. The optimal time for flow rate adjustment during the process was approximated. Finally, effects of ozone velocity and ozone gas concentration on the Stanton number were evaluated. 相似文献
889.
Lopez-Espinosa MJ Kiviranta H Araque P Ruokojärvi P Molina-Molina JM Fernandez MF Vartiainen T Olea N 《Chemosphere》2008,73(6):967-971
Seventeen polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) were quantified in adipose tissue samples of non-occupationally exposed women living in Southern Spain. Geometric mean levels of sum of congeners and WHO(PCDD/F)-TEQ(2005) were 410 and 17.9pgg(-1) fat, respectively. Among PCDDs, octachlorodibenzo-p-dioxin (OCDD) showed the highest concentration with a mean value of 265pgg(-1) fat, followed by 1,2,3,6,7,8-HxCDD (49.3pgg(-1) fat) and 1,2,3,4,6,7,8-HpCDD (45.2pgg(-1) fat). These three congeners were responsible for around 90% of the sum of all PCDD/F congeners in adipose tissue. The geometric mean 2,3,7,8-TCDD value was 1.87pgg(-1) fat. 2,3,4,7,8-PeCDF (8.43pgg(-1) fat) showed the highest concentration among the PCDFs, followed by 1,2,3,4,7,8-HxCDF (4.17pgg(-1) fat) and 1,2,3,6,7,8-HxCDF (3.28pgg(-1) fat), and these three congeners were responsible for 4% of the sum of all studied PCDD/F congeners in adipose tissue and 76% of the sum of ten PCDFs. 1,2,3,7,8,9-HxCDF was the only congener not quantified in any sample, while 1,2,3,4,7,8,9-HpCDF, 1,2,3,7,8-PeCDF, OCDF and 2,3,7,8-TCDF were found in 5, 16, 16 and 19 samples, respectively. All other congeners were quantifiable in all 20 samples. Congeners contributing most to the WHO(PCDD/F)-TEQ(2005) were 1,2,3,7,8-PeCDD (31.6%), 1,2,3,6,7,8-HxCDD (28.3%) and 2,3,4,7,8-PeCDF (14.6%). The body burden of log-transformed WHO(PCDD/F)-TEQ(2005) levels increased with age (B=0.02; 95% CI=0.01, 0.03; p=0.02). Although these adipose tissue PCDD/F levels are similar to previously published findings in Spain and other European countries, further research is needed to determine trends in the exposure of women to these chemical residues. 相似文献
890.
The impact of motorcycle traffic on soil and vegetation of stabilized coastal dunes, Israel 总被引:1,自引:0,他引:1
This study aimed to assess the response of soil and annual plant vegetation of stabilized coastal dunes in Israel, to varying
intensities of off-road motorcycle (ORM) traffic, and to assess their resistance and resilience to such a disturbance. A standard
experimental procedure that included 0, 20, 50, 100 and 200 ORM straight passes and 150 ORM turn passes was used. Plant ground
cover, mean plant height, species richness, species diversity, soil penetrable depth, organic matter and moisture contents
were measured on several dates within a period of 372 days after the experiment. Results have shown that: (1) ORM passes had
a significant immediate impact on annual plants that increased with traffic intensity. The impact on the soil was detected
only as an increase of penetrable depth. (2) The maximum impact on annual plants was observed in the wheel ruts and turn areas.
The impact on the area between the wheel ruts and on the margins outside the wheel ruts was indirect and smaller. (3) Annual
plant ground cover and mean plant height were less sensitive parameters than species richness and species diversity for determining
the impact of ORM traffic on the area. (4) One year after the experiment, soil and annual plant vegetation in all passes were
very similar to their pre-experimental condition. This indicates high resilience and recovery potential of the Mediterranean
stabilized coastal dune ecosystem to ORM disturbance. 相似文献