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211.
Concentrations of 86 congeners of polychlorinated biphenyls (PCBs) were determined for 25 adult female and 25 adult male burbot (Lota lota) from Lake Erie. Significant differences in mean proportions of total PCB concentration between males and females ages 14–17 were found for 26 congeners. Males generally had higher mean proportions of hexachloro congeners, whereas females had higher mean proportions of more highly chlorinated congeners. In contrast, only four congeners exhibited differences between males and females ages 6–13 in mean proportions of total PCB. Therefore, the sexual difference in PCB congener distribution widened for older burbot. Males ages 14–17 also had higher proportions of certain hexachloro congeners than the other three demographic groups (males ages 6–13, females ages 6–13, and females ages 14–17) we examined. The reverse was true for more highly chlorinated congeners. The results supported a previous hypothesis that older male burbot spent a substantial amount of time feeding in the vicinity of mouths of rivers with sediment contaminated with PCBs. However, additional studies are needed to clarify and corroborate this apparent “hot spot” effect, such as seasonal movements, spatial distributions, and diet of burbot; and PCB congener distributions of various species of prey fishes captured at various locations throughout the eastern basin of Lake Erie and at different locations in the contaminated rivers. 相似文献
212.
Charles E. Billings Leslie Silverman Richard Dennis Lester H. Levenbaum 《Journal of the Air & Waste Management Association (1995)》2013,63(4):318-330
The trends in and relationships between ambient air concentrations of sulfur dioxide and sulfate aerosols at 48 urban sites and 27 nonurban sites throughout the U.S. between 1963 and 1972 have been analyzed. The substantial decreases in ambient SO2 concentrations measured at urban sites in the eastern and midwestern U.S. are consistent with the corresponding reductions in local SO2 emissions, but these decreases have been accompanied by only modest decreases in ambient sulfate concentrations. Large differences in the amounts of SO2 emitted within individual air quality control regions are associated with much smaller differences in the corresponding ambient sulfate concentrations. Substantial changes in the patterns of SO2 emissions between air quality regions result in essentially no differences between ambient sulfate concentrations in those air quality regions. Comparisons of several air quality regions in the eastern and western U.S. with similar SO2 emission levels and patterns of emissions clearly demonstrates the higher ambient sulfate concentration levels in eastern air quality control regions. Relationships between SO2, sulfates, and vanadium concentrations at eastern nonurban U.S. sites cannot be explained by local emission sources. These various observed results can be best explained by long distance sulfur oxide transport with chemical conversion of SO2 to sulfates occurring over ranges of hundreds of kilometers. This conclusion has been suggested earlier and the present analysis strongly supports previous discussions. An impact of long range transport of sulfates is to emphasize the need for Consistent strategies for reduction of sulfur oxides throughout large geographical regions. Additions of large capacities involving elevated sources in mid-continental or western regions could result in significant increases in sulfate concentrations well downwind of such sources. Some of the types of research activities required to quantitate crucial experimental parameters are discussed. 相似文献
213.
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215.
Water movement within the unsaturated zone in four agricultural areas of the United States 总被引:2,自引:0,他引:2
Millions of tons of agricultural fertilizer and pesticides are applied annually in the USA. Due to the potential for these chemicals to migrate to groundwater, a study was conducted in 2004 using field data to calculate water budgets, rates of groundwater recharge and times of water travel through the unsaturated zone and to identify factors that influence these phenomena. Precipitation was the only water input at sites in Indiana and Maryland; irrigation accounted for about 80% of total water input at sites in California and Washington. Recharge at the Indiana site (47.5 cm) and at the Maryland site (31.5 cm) were equivalent to 51 and 32%, respectively, of annual precipitation and occurred between growing seasons. Recharge at the California site (42.3 cm) and Washington site (11.9 cm) occurred in response to irrigation events and was about 29 and 13% of total water input, respectively. Average residence time of water in the unsaturated zone, calculated using a piston-flow approach, ranged from less than 1 yr at the Indiana site to more than 8 yr at the Washington site. Results of bromide tracer tests indicate that at three of the four sites, a fraction of the water applied at land surface may have traveled to the water table in less than 1 yr. The timing and intensity of precipitation and irrigation were the dominant factors controlling recharge, suggesting that the time of the year at which chemicals are applied may be important for chemical transport through the unsaturated zone. 相似文献
216.
Snowmobile use in Yellowstone National Park has been shown to impact air quality, with implications for the safety and welfare
of Park staff and other Park resource values. Localized impacts have been documented at several high-use sites in the Park,
but the broader spatial variability of snowmobile emissions and air quality was not understood. Measurements of 87 volatile
organic compounds (VOCs) were made for ambient air sampled across the Park and West Yellowstone, Montana, during 2 days of
the 2002–2003 winter use season, 1 year before the implementation of a new snowmobile policy. The data were compared with
similar data from pristine West Coast sites at similar latitudes. Backward trajectories of local air masses, alkyl nitrate-parent
alkane ratios, and atmospheric soundings were used to identify the VOC sources and assess their impact. Different oversnow
vehicle types used in the Park were sampled to determine their relative influence on air mass pollutant composition. VOCs
were of local origin and demonstrated strong spatiotemporal variability that is primarily influenced by levels of snowmobile
traffic on given road segments at different times of day. High levels of snowmobile traffic in and around West Yellowstone
produced consistently high levels of benzene, toluene, and carbon monoxide. 相似文献
217.
218.
Richard J. Horwitz Thomas E. Johnson Paul F. Overbeck T. Kevin O’Donnell W. Cully Hession Bernard W. Sweeney 《Journal of the American Water Resources Association》2008,44(3):724-741
Abstract: The joint influences of riparian vegetation and urbanization on fish assemblages were analyzed by depletion sampling in paired forested and nonforested reaches of 25 small streams along an urbanization gradient. Nonforested reaches were narrower than their forested counterparts, so densities based on surface area differ from linear densities (based on reach length). Linear densities (based on number or biomass of fish) of American eel, white sucker and tesselated darter, and the proportion of biomass of benthic invertivores were significantly higher in nonforested reaches, while linear densities of margined madtom and the number of pool species were significantly higher in forested reaches. Observed riparian effects may reflect differences in habitat and algal productivity between forested and nonforested reaches. These results suggest that relatively small‐scale riparian restoration projects can affect local geomorphology and the abundance of fish. Dense vegetative cover in riparian zones and similar or analogous habitats in both forested and nonforested reaches, the relatively small scale of the nonforested reaches, and the low statistical power to detect differences in abundance of rare species may have limited the observed differences between forested and nonforested reaches. There was a strong urbanization gradient, with reductions of intolerant species and increases of tolerant species and omnivores with increasing urbanization. Interactions between riparian vegetation type and urbanization were found for blacknose dace, creek chub, tesselated darter, and the proportion of biomass of lithophilic spawners. The study did not provide consistent support for the hypotheses that responses of fish to riparian vegetation would be overwhelmed by urban degradation or insignificant at low urbanization. 相似文献
219.
Barbra C. Utley George Vellidis Richard Lowrance Matt C. Smith 《Journal of the American Water Resources Association》2008,44(3):742-753
Abstract: Sediment oxygen demand (SOD) is believed to be an important process affecting dissolved oxygen (DO) concentrations in blackwater streams of the southeastern coastal plain. Because very few data on SOD are available, it is common for modelers to take SOD values from the literature for use with DO models. In this study, SOD was measured in seven blackwater streams of the Suwannee River Basin within the Georgia coastal plain for between August 2004 and April 2005. SOD was measured using four in situ chambers and was found to vary on average between 0.1 and 2.3 g O2/m/day across the seven study sites throughout the study period. SOD was found to vary significantly between the watersheds within the Suwannee River Basin. However, land use was not found to be the driving force behind SOD values. Statistical analyses did find significant interaction between land use and watersheds suggesting that an intrinsically different factor in each of the watersheds may be affecting SOD and the low DO concentrations. Further research is needed to identify the factors driving SOD dynamics in the blackwater streams of Georgia’s coastal plain. Results from this study will be used by the Georgia Department of Natural Resources – Environmental Protection Division as model input data for the development and evaluation of DO total maximum daily loads in the Georgia coastal plain. 相似文献
220.
George N. Zaimes Richard C. Schultz Thomas M. Isenhart 《Journal of the American Water Resources Association》2008,44(4):935-947
Abstract: Phosphorus and sediment are major nonpoint source pollutants that degrade water quality. Streambank erosion can contribute a significant percentage of the phosphorus and sediment load in streams. Riparian land‐uses can heavily influence streambank erosion. The objective of this study was to compare streambank erosion along reaches of row‐cropped fields, continuous, rotational and intensive rotational grazed pastures, pastures where cattle were fenced out of the stream, grass filters and riparian forest buffers, in three physiographic regions of Iowa. Streambank erosion was measured by surveying the extent of severely eroding banks within each riparian land‐use reach and randomly establishing pin plots on subsets of those eroding banks. Based on these measurements, streambank erosion rate, erosion activity, maximum pin plot erosion rate, percentage of streambank length with severely eroding banks, and soil and phosphorus losses per unit length of stream reach were compared among the riparian land‐uses. Riparian forest buffers had the lowest streambank erosion rate (15‐46 mm/year) and contributed the least soil (5‐18 tonne/km/year) and phosphorus (2‐6 kg/km/year) to stream channels. Riparian forest buffers were followed by grass filters (erosion rates 41‐106 mm/year, soil losses 22‐47 tonne/km/year, phosphorus losses 9‐14 kg/km/year) and pastures where cattle were fenced out of the stream (erosion rates 22‐58 mm/year, soil losses 6‐61 tonne/km/year, phosphorus losses 3‐34 kg/km/year). The streambank erosion rates for the continuous, rotational, and intensive rotational pastures were 101‐171, 104‐122, and 94‐170 mm/year, respectively. The soil losses for the continuous, rotational, and intensive rotational pastures were 197‐264, 94‐266, and 124‐153 tonne/km/year, respectively, while the phosphorus losses were 71‐123, 37‐122, and 66 kg/km/year, respectively. The only significant differences for these pasture practices were found among the percentage of severely eroding bank lengths with intensive rotational grazed pastures having the least compared to the continuous and rotational grazed pastures. Row‐cropped fields had the highest streambank erosion rates (239 mm/year) and soil losses (304 tonne/km/year) and very high phosphorus losses (108 kg/km/year). 相似文献