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801.
载硫活性炭微观结构和表面形态研究 总被引:1,自引:0,他引:1
为了增强活性炭脱除燃煤电厂烟气中汞的能力,利用汞和硫可以生成稳定的HgS的性质,研究了通过热沉淀增加了活性炭中的硫含量的改性方法,并以SEM、BET、TGA等方法,研究了改性对活性炭表面形貌、硫在活性炭中的分布、活性炭比表面积等性能的影响。结果表明,热沉淀改性方法可以增加活性炭中的硫含量;硫粘附在活性炭的炭链上量较多,孔壁较少;改性工艺降低了活性炭的比表面积,且改性活性炭的比表面积随着温度的升高而增大;载硫后,活性炭中元素硫和炭的结合被增强。 相似文献
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Huai Chen Ning Wu Shouping Yao Yongheng Gao Dan Zhu Yanfen Wang Wan Xiong Xingzhong Yuan 《Atmospheric environment (Oxford, England : 1994)》2009,43(32):4995-5000
The littoral zones of lakes have been regarded as hotspots of methane (CH4) fluxes through several studies. In the present study, we measured CH4 fluxes in six kinds of littoral zones of Huahu Lake on the Qinghai-Tibetan Plateau in the peak growing season of 2006 and 2007. We found that CH4 efflux (ranging from −0.1 to 90 mg CH4 m−2 h−1) from the littoral zones of this lake was relatively high among those of boreal and temperate lakes. Our results also showed that emergent plant zones (Hippuris vulgaris and Glyceria maxima stands) recorded the highest CH4 flux rate. The CH4 flux in the floating mat zone of Carex muliensis was significantly lower than those of the emergent plant zones. CH4 fluxes in the floating-leaved zone of Polygonum amphibium and bare lakeshore showed no significant difference and ranked last but one, only higher than that of the littoral meadow (Kobresia tibetica). Plant biomass and standing water depths were important factors to explain such spatial variations in CH4 fluxes. No significant temporal variations in CH4 fluxes were found due to the insignificant variations of physical factors in the peak growing season. These results may help in our understanding of the importance of the littoral zone of lakes, especially the emergent plant zone, as a hotspot of CH4 emission. 相似文献
805.
Jian Gao Tao Wang Xuehua Zhou Waishing Wu Wenxing Wang 《Atmospheric environment (Oxford, England : 1994)》2009,43(4):829-836
Particle size distribution is important for understanding the sources and effects of atmospheric aerosols. In this paper we present particle number size distributions (10 nm–10 μm) measured at a suburban site in the fast developing Yangtze River Delta (YRD) region (near Shanghai) in summer 2005. The average number concentrations of ultrafine (10–100 nm) particles were 2–3 times higher than those reported in the urban areas of North America and Europe. The number fraction of the ultrafine particles to total particle count was also 20–30% higher. The sharp increases in ultrafine particle number concentrations were frequently observed in late morning, and the particle bursts on 5 of the 12 nucleation event days can be attributed to the homogeneous nucleation leading to new particle formation. The new particle formation events were characterized with a larger number of nucleation-mode particles, larger particle surface area, and larger condensational sink than usually reported in the literature. These suggest an intense production of sulfuric acid from photo-oxidation of sulfur dioxide in the YRD. Overall, the growth rate of newly formed particles was moderate (6.4 ± 1.6 nm h?1), which was comparable to that reported in the literature. 相似文献
806.
Measurement of black carbon aerosols near two Chinese megacities and the implications for improving emission inventories 总被引:1,自引:0,他引:1
Xuehua Zhou Jian Gao Tao Wang Waishing Wu Wenxing Wang 《Atmospheric environment (Oxford, England : 1994)》2009,43(25):3918-3924
Knowledge of the distribution and sources of black carbon (BC) is essential to understanding its impact on radiative forcing and the establishment of a control strategy. In this study, we analyze atmospheric BC and its relationships with fine particles (PM2.5) and trace gases (CO, NOy and SO2) measured in the summer of 2005 in two areas frequently influenced by plumes from Beijing and Shanghai, the two largest cities in China. The results revealed different BC source characteristics for the two megacities. The average concentration of BC was 2.37 (±1.79) and 5.47 (±4.00) μg m?3, accounting for 3.1% and 7.8% of the PM2.5 mass, in Beijing and Shanghai, respectively. The good correlation between BC, CO and NOy (R2 = 0.54–0.77) and the poor correlation between BC and SO2 suggest that diesel vehicles and marine vessels are the dominant sources of BC in the two urban areas during summer. The BC/CO mass ratio in the air mass from Shanghai was found to be much higher than that in the air mass from Beijing (0.0101 versus 0.0037 ΔgBC/ΔgCO), which is attributable to a larger contribution from diesel burning (diesel-powered vehicles and marine vessels) in Shanghai. Based on the measured ratios of BC/CO and annual emissions of CO, we estimate that the annual emissions of BC in Beijing and Shanghai are 9.51 Gg and 18.72 Gg, respectively. The improved emission rates of BC will help reduce the uncertainty in the assessment of the impact of megacities on regional climate. 相似文献
807.
现代武器往往产生大量噪声,对使用这些武器或在这些武器周围作业的人员构成很大威胁,防护不当会导致这些人员的听力受到不同程度的损害。本文介绍了部分现代武器产生的噪声以及对人员可能造成的伤害,分析了防护装备的作用和局限性。 相似文献
808.
聚硅氯化铝(PASC)的形态分布及转化规律:Ⅰ.Al—Ferron逐时络合比色?… 总被引:23,自引:2,他引:21
采用Al-Ferron逐时络合比色法比较研究了PASC与PAC中铝的形态分布及转化规律。实际结果表明,在PASC中,由于聚硅酸与铝水解聚合产物的相互作用,使得铝的水解聚合形态分布及转化情况发生了变化。 相似文献
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810.
Utilization of washed MSWI fly ash as partial cement substitute with the addition of dithiocarbamic chelate 总被引:1,自引:0,他引:1
The management of the big amount of fly ash as hazardous waste from the municipal solid waste incinerator (MSWI) has encountered many problems in China. In this study, a feasibility research on MSWI fly ash utilization as partial cement substitute in cement mortars was therefore carried out. MSWI fly ash was subjected to washing process to reduce its chlorine content (from 10.16% to 1.28%). Consequently, it was used in cement mortars. Ten percent and 20% replacement of cement by washed ash showed acceptable strength properties. In TCLP and 180-day monolithic tests, the mortars with washed ash presented a little stronger heavy metal leachability, but this fell to the blank level (mortar without washed ash) with the addition of 0.25% chelate. Therefore, this method is proposed as an environment-friendly technology to achieve a satisfactory solution for MSWI fly ash management. 相似文献