Polycyclic aromatic hydrocarbons in effluents from wastewater treatment plants and receiving streams in Tianjin, China

Surface water, suspended particulate matter, pore water, and sediment samples were collected and analyzed for polycyclic aromatic hydrocarbons (PAHs) in Yongding New River, South Drainage Canal and North Drainage Canal, which receive most of wastewater from industrial city of Tianjin. PAH concentrations in effluent samples of wastewater treatment plants (WTP) discharging into the South Drainage Canal and North Drainage Canal were quantified for the first time. The results showed that the discharge of the WTPs recently only contributed to the PAH contamination in the canals near the outlets of the WTPs. PAH levels in sediments of the streams were greatly higher than those in soils by riverbank probably due to receiving large amounts of untreated wastewater. Unusually high benz[a] anthracene concentration strongly influenced the seasonal and spatial variation of total PAH concentrations in South Drainage Canal. Paired samples t test of ??Nap, Fl, Phe, Fluo and ??Nap, Phe, Fluo, Chry concentrations, which were dominant components in the air samples from non-heating and heating season, respectively, in the suspended particulate matters from the streams showed that PAH source from air deposition was more important for Yongding New River than that for South Drainage Canal and North Drainage Canal. Source apportionment based on PAH profiles indicated that coal combustion was the major PAH contamination source, and coke oven sources and wood combustion also contributed to the PAH contamination of the streams. This was further indicated by organic petrography analysis.     

Pollution characteristics and health risk assessment of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons during heating season in Beijing

Polycyclic aromatic hydrocarbons(PAHs) and their nitrated derivatives(NPAHs) attract continuous attention due to their outstanding carcinogenicity and mutagenicity. In order to investigate the diurnal variations, sources, formation mechanism, and health risk assessment of them in heating season, particulate matter(PM) were collected in Beijing urban area from December 26, 2017 to January 17, 2018. PAHs and NPAHs in PM were quantitatively analyzed via gas chromatography-mass spectrometry(GC-MS). ...     

Effect of alkaline earth metal promoter on catalytic activity of MnO2 for the complete oxidation of toluene

Herein, Na⁺ and Ca²⁺ are introduced to MnO₂ through cation-exchange method. The presence of Na⁺ and Ca²⁺ significantly enhance the catalytic activity of MnO₂ in toluene oxidation. Among them, the Ca-MnO₂ catalyst exhibits the best catalytic activity (T₅₀ = 194°C, T₉₀ = 215°C, E_a = 57.2 kJ/mol, reaction rate 8.40 × 10^?10 mol/(sec?m²) at 210°C. T₅₀ and T₉₀: the temperature of 50% and 90% toluene conversion; E_a: apparent activation energy) and possess high tolerance against 2.0 vol.% water vapor. Results reveal that the increased acidic sites of the MnO₂ sample can enhance the adsorption of gaseous toluene, and the mobility of oxygen species and the content of reactive oxygen species in the catalyst are significantly improved due to the formed oxygen vacancy. Thus these two factors result in excellent catalytic performance for toluene oxidation combining with the weak CO₂ adsorption ability.     

Effects of bio-organic fertilizers on pineapple heart rot and bacterial community structure北大核心CSCD

Heart rot is a common soil-borne disease in the pineapple industry, but the situation can be alleviated by the application of bio-fertilizers with beneficial microbiomes. Clarifying the controlling mechanism of bio-organic fertilizer on the high incidence of heart rot is critical in monocultural pineapple cropping patterns. In our study, the soil of continuous cropping pineapple orchards was collected. Three types of carriers (rapeseed cake, peat soil, and coconut bran), biocontrol strains (Bacillus subtilis HL2 and Streptomyces strain HL3), and organic fertilizer (YJ) were composted into different bio-fertilizers (KC, KN, KY, LC, LN, and LY), which were used in pot experiments. The controlling effect of the bio-fertilizer was determined based on the response of pineapple heart rot and bacterial communities to different fertilizing methods. Our results revealed that the incidence of heart rot in bio-fertilizer KC was the lowest, which decreased by 20% and 13.3%, respectively, compared to HF (chemical fertilizer, 16-16-16) and YJ (organic fertilizer). The richness and diversity of soil bacterial communities in all biofertilized treatments (KC, KN, KY, LC, LN, and LY) were significantly higher than those in HF. However, the α-diversity indices of the bio-fertilizers (KC, KN, and KY) were higher than those of LC, LN, and LY, and the bacterial community composition was significantly different. The bacteria GP4, GP6, Bacillus, and Azohydromonas were enriched in KC, KN, and KY, while the relative abundance of Streptomyces increased significantly in LC, LN, and LY. Furthermore, Spearman correlation analysis showed that the relative abundance of these bacterial groups was significantly negatively correlated with the incidence of pineapple heart rot. In summary, the application of bio-organic fertilizers can decrease the incidence of pineapple heart rot by altering the soil bacterial community structure and stimulating beneficial soil microorganisms, which is important for reconstructing the ecological balance in continuous pineapple orchards. © 2022 Authors. All rights reserved.     

Alkyl polyglycosides enhanced the dark fermentation of excess sludge and plant waste to produce hydrogen: performance and mechanism

Environmental Science and Pollution Research - Alkyl polyglycosides (APG), a biodegradable biosurfactant, have been widely used in environmental pollution control. However, the application of APG...     

Analysis of the mechanism of the impact of internet development on green economic growth: evidence from 269 prefecture cities in China

As the digital economy develops rapidly and the network information technology advances, new development models represented by the network economy have emerged, which have a crucial impact on green economic growth. However, the relevant previous studies lacked the role of analyzing the direct and indirect effects of internet development on green economic growth at the prefecture-level city level. For this purpose, this paper aims to examine the intrinsic mechanism of the impact of internet development on green economic growth and provide empirical support for cities and regions in China to increase internet construction. Furthermore, the mixed model (EBM), which includes both radial and non-radial distance functions, is applied to calculate the green economic growth index. Fixed effect model and mediation effect model are also employed to test influence mechanisms of the internet development on green economic growth using panel data of 269 prefecture-level cities in China from 2004 to 2019. The statistical results reveal that internet development has contributed significantly to green economic growth. When the internet development level increases by 1 unit, the green economic growth level increases by an average of 5.0372 units. However, regional heterogeneity is evident between internet development and green economic growth, that is, the promoting effect of internet development on green economic growth is gradually enhanced from the eastern region to the western region. We also find that internet development guides industrial structure upgrading improves environmental quality and accelerates enterprise innovation, which indirectly contributes to green economic growth. And internet development mainly achieves green economic growth through enterprise innovation. Based on the above findings, we concluded that policymakers should not only strengthen the guiding role of social actors to promote the stable development of the internet industry, but also foster the construction of the three models of “internet+industry integration,” “internet+environmental governance,” and “internet+enterprise innovation” to promote green economic growth.

     

The role of N6-methyladenosine methylation in environmental exposure-induced health damage

Environmental Science and Pollution Research - The health risks caused by environmental pollution have long been of substantial concern. With the development of epigenetics, a large number of...     

Research progress of vapor phase corrosion inhibitors in marine environment

Environmental Science and Pollution Research - Marine corrosion is a kind of material failure phenomenon caused by the interaction between metal structure and marine environment. As an efficient...     

Spatial decoupling of facilitation and competition at the origin of gapped vegetation patterns

Spatially periodic vegetation patterns, forming gaps, bands, labyrinths, or spots, are characteristic of arid and semiarid landscapes. Self-organization models can explain this variety of structures within a unified conceptual framework. All these models are based on the interplay of positive and negative effects of plants on soil water, but they can be divided according to whether they assume the interactions to be mediated by water redistribution through runoff/diffusion or by plants' organs. We carried out a multi-proxy approach of the processes operating in a gapped pattern in southwest Niger dominated by a shrub species. Soil moisture within the root layer was monitored in time and space over one month of the rainy season. Soil water recharge displayed no spatial variation with respect to vegetation cover, but the stock half-life under cover was twice that of bare areas. A kernel of facilitation by the aboveground parts of shrubs was parameterized, and soil water half-life was significantly correlated to the cumulated facilitative effects of shrubs. The kernel range was found to be smaller than the canopy radius (81%). This effect of plants on soil water dynamics, probably through a reduction of evaporation by shading, is shown to be a better explanatory variable than potentially relevant soil and topography parameters. The root systems of five individuals of Combretum micranthum G. Don were excavated. Root density data were used as a proxy to parameterize a kernel function of interplant competition. The range of this kernel was larger than the canopy radius (125%). The facilitation-to-competition range ratio, reflecting the above-to-belowground ratio of plant lateral extent, was smaller than 1 (0.64), a result supporting models assuming that patterning may emerge from an adaptation of plant morphology to aridity and shallow soils by means of an extended lateral root system. Moreover, observed soil water gradients had directions opposite to those assumed by alternative mathematical models based on underground water diffusion. This study contributes to the growing awareness that combined facilitative and competitive plant interactions can induce landscape-scale patterns and shape the two-way feedback loops between environment and vegetation.     

恒液位推流式改良SBR工艺处理生活污水

通过对恒液位推流式改良SBR工艺处理生活污水工程应用的研究,结果表明:恒液位推流式改良SBR工艺在降低工程成本和减少设备量的同时能较好的去除污水中的污染物,具有良好的脱氮除磷效果,COD去除率可达85%~93%;TP的去除率可达84%;TN的去除率可达82%。