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681.
T.M. McIntire O.S. Ryder P.L. Gassman Z. Zhu S. Ghosal B.J. Finlayson-Pitts 《Atmospheric environment (Oxford, England : 1994)》2010,44(7):939-944
It is commonly assumed that atmospheric oxidation of hydrocarbon particles or hydrocarbon coatings on particles leads to polar products and increased water uptake, altering atmospheric visibility and increasing the likelihood they will act as cloud condensation nuclei (CCN). We show here through laboratory experiments that increased water uptake depends on the 3-dimensional structure of the particles. Laboratory studies of particles formed during ozonolysis of surface-bound alkenes, present as terminally unsaturated self-assembled monolayers (C8= SAM) on a silica substrate, were carried out at room temperature and 1 atm pressure. SAMs were exposed to ~1013 O3 molecules cm?3 for 40 min and resultant particles were analyzed using single particle Fourier transform infrared micro-spectroscopy (micro-FTIR) and secondary ion mass spectroscopy (SIMS). Spectroscopy results show that –COOH and other polar groups are formed but are buried inside a hydrophobic shell, consistent with earlier observations (McIntire et al., 2005, Moussa et al., 2009) that water uptake does not increase after reaction of the terminal alkene with O3. These insights into the 3-D structure of particles formed on oxidation have important implications for the ability of secondary organic aerosols to act as CCN. In addition, the nature of the surface of the particles is expected to determine their uptake into biological systems such as the surface of the lungs. 相似文献
682.
M. Tainio J.T. Tuomisto J. Pekkanen N. Karvosenoja K. Kupiainen P. Porvari M. Sofiev A. Karppinen L. Kangas J. Kukkonen 《Atmospheric environment (Oxford, England : 1994)》2010,44(17):2125-2132
The emission-exposure and exposure-response (toxicity) relationships are different for different emission source categories of anthropogenic primary fine particulate matter (PM2.5). These variations have a potentially crucial importance in the integrated assessment, when determining cost-effective abatement strategies. We studied the importance of these variations by conducting a sensitivity analysis for an integrated assessment model. The model was developed to estimate the adverse health effects to the Finnish population attributable to primary PM2.5 emissions from the whole of Europe. The primary PM2.5 emissions in the whole of Europe and in more detail in Finland were evaluated using the inventory of the European Monitoring and Evaluation Programme (EMEP) and the Finnish Regional Emission Scenario model (FRES), respectively. The emission-exposure relationships for different primary PM2.5 emission source categories in Finland have been previously evaluated and these values incorporated as intake fractions into the integrated assessment model. The primary PM2.5 exposure-response functions and toxicity differences for the pollution originating from different source categories were estimated in an expert elicitation study performed by six European experts on air pollution health effects. The primary PM2.5 emissions from Finnish and other European sources were estimated for the population of Finland in 2000 to be responsible for 209 (mean, 95% confidence interval 6–739) and 357 (mean, 95% CI 8–1482) premature deaths, respectively. The inclusion of emission-exposure and toxicity variation into the model increased the predicted relative importance of traffic related primary PM2.5 emissions and correspondingly, decreased the predicted relative importance of other emission source categories. We conclude that the variations of emission-exposure relationship and toxicity between various source categories had significant impacts for the assessment on premature deaths caused by primary PM2.5. 相似文献
683.
A.M.M. Manders M. Schaap X. Querol M.F.M.A. Albert J. Vercauteren T.A.J. Kuhlbusch R. Hoogerbrugge 《Atmospheric environment (Oxford, England : 1994)》2010,44(20):2434-2442
The oceans are a major source for particles that play an important role in many atmospheric processes. In Europe sea salt may contribute significantly to particulate matter concentrations. We have compiled sodium concentration data as a tracer for sea salt for 89 sites in Europe to provide more insight in the distribution of sea salt across Europe. The annual average sea salt concentrations above land were estimated to range between 0.3 and almost 13 μg m?3. Maximum concentrations are found at the Irish coast. At coastal sites along the Atlantic and North Sea coast concentrations tend to be around 5 μg m?3. More inland locations up to about 300 km away from the coast tend to show concentrations between 2 and 5 μg m?3, whereas sites further away from the coast are characterized by lower concentrations. An analysis of the representativity of the data with respect to a long term average showed that the long average is associated with a standard deviation of around 15%. The compilation of observations provides an improved overview of sea salt concentrations in Europe as well as an improved basis for model validation. Verification of the results of the LOTOS-EUROS model learned that the model represents well the spatial variability of the observed sea salt concentrations very well. However, the absolute concentrations are significantly overestimated due to large uncertainties in the emission and dry deposition parameterizations. Using the high explained variability in the gradients across Europe, the bias-corrected modelled distribution serves as a best estimate of the sea salt distribution across Europe for 2005. 相似文献
684.
Vo Thi Thanh Loc Simon R. Bush Le Xuan Sinh Nguyen Tri Khiem 《Environment, Development and Sustainability》2010,12(6):889-908
This paper investigates the structure, function and wealth distribution within the Pangasius hypophthalmus and Henicorhynchus spp./Labiobarbus spp. value chains in the Mekong Delta of Vietnam. The analysis is driven by key questions relating to the form and function
of value chains, their contribution to the livelihoods of farmers and fishers, the effectiveness of government policy and
the potential for value chain governance mechanisms, such as contracts and certification, to steer towards sustainable production.
The results indicate that actors in the high value Pangasius hypopthalmus export chain have a higher potential income, but face considerably higher economic vulnerability from global markets. Alternatively,
Henichorhychus/Labiobarbus spp. fishers are severely constrained in their ability to negotiate higher prices for their fish but appear to be less vulnerable
to economic and environmental change. The paper concludes that for value chain governance to improve the livelihoods of fishers
and farmers in both high and low value chains, new arrangements are needed that better accommodate customary institutions
and informal market relations. 相似文献
685.
Developed countries are major markets for developing country fresh produce. Demand by developed country consumers for spotless
produce has encouraged developing country consumers to rely increasingly on pesticides in producing fresh export vegetables.
However developed country pesticide standards enacted in response to reports of increased farmer and farm worker pesticide
poisoning and the food safety scandals of the 1980s and 1990s require changes in the way growers use pesticides. The EU has
especially developed stringent food safety standards relating to, among other things, pesticide usage. Under EU pesticide
standards (EU-PS) farmers are trained by their buyers on safe use of pesticides and then closely monitored under contract.
This paper looks at the impact of these standards on developing country farmers’ use of alternative pest management practices,
pesticide protective clothing and the actual usage of pesticides. It finds that compliance with EU-PS increases the use of
alternative pest management practices and protective clothing. However, EU-PS has mixed effect on the quantity of pesticides
used. The paper also finds that farmer’s education and access to information play an important role in the use of alternative
pest management practices. The paper concludes that EU-PS encourage the use of alternative pest management practices and pesticide
protective gear in production of fresh export vegetables. The findings imply that EU-PS promote environmentally-friendly methods
of production of fresh export vegetables in developing countries. 相似文献
686.
687.
J. Ram Pillarisetti Jeroen C. J. M. van den Bergh 《Environment, Development and Sustainability》2010,12(1):49-62
What is a ‘sustainable nation’ and how can we identify and rank ‘sustainable nations?’ Are nations producing and consuming in a sustainable way? Although several aggregate indexes have been proposed to answer such questions, comprehensive and internationally comparable data are not available for most of these. This paper quantitatively compares three aggregate indexes of sustainability: the World Bank’s ‘Genuine Savings’ measure, the ‘Ecological Footprint,’ and the ‘Environmental Sustainability Index.’ These three indexes are available for a large number of countries and also seem to be the most influential among the aggregate indexes. This paper first discusses the main limitations and weaknesses of each of these indexes. Subsequently, it shows that rankings of sustainable nations and aggregate assessments of unsustainable world population and world GDP shares vary considerably among these indexes. This disagreement leads to suggestions for analysis and policy. One important insight is that climate change, arguable the most serious threat currently faced by humanity, is not or arbitrarily captured by the indexes. 相似文献
688.
Exporting natural capital: the foreign eco-footprint on Costa Rica and implications for sustainability 总被引:1,自引:0,他引:1
As the world economy ‘globalizes’, trade has become a major mechanism by which much of the human population supports its needs.
While trade in resource commodities (natural income) can increase the well-being of people in both exporting and importing
countries, it can also lead to depletion of natural capital and the loss of ecosystems integrity. In recent years, various
researchers have attempted to address this problem using a consumption-based perspective on ecological change. Their work
shows that the loss of ecosystem integrity in almost any region of the world can be attributed to both local and international
consumer demand. This paper illustrates the utility of modified eco-footprint analysis in assessing export-related ecological
change in Costa Rica. We quantify ecological footprint of consumers around the world on the productive ecosystems of Costa
Rica, document the changing character of this footprint and highlight some of the linkages between production for export in
Costa Rica and ecological degradation. We then discuss the implications of the increasing trade-based entanglement of nations
for ecosystems and global sustainability. 相似文献
689.
Kris A. G. Wyckhuys Robert J. O’Neil 《Environment, Development and Sustainability》2010,12(3):297-311
In subsistence farming systems of the developing world, adoption of resource-conserving practices such as integrated pest
management (IPM) is often strikingly low. This has partially been ascribed to researchers’ limited understanding of how technologies
develop at the interface of the systems’ social and ecological components. In Honduras (Central America), there exists concern
about limited adoption and diffusion of IPM technologies in certain smallholder production systems. In this study, we determine
social and ecological drivers of IPM adoption in subsistence maize production in the country’s hillside environment. Honduran
small-scale maize production is typified by a key insect pest (the fall armyworm, Spodoptera frugiperda) being partly kept at bay through action of a diverse natural enemy complex, including ants, social wasps, carabid beetles,
and spiders. Local agricultural landscapes, primarily shaped through shifting cultivation, provide key resources to maintain
this natural enemy diversity. These local ecological conditions and related natural enemy abundance strongly influence farmers’
agroecological knowledge and pest management practices. In the meantime, farmer practices are also affected by local communication
networks, which help validate and spread IPM concepts and technologies. Based on our findings, we advocate a holistic approach
to improve IPM extension through mapping of agroecological opportunities, visualization of regional patterns in farmer knowledge,
and associated priority setting. Local IPM capacity could be built through institutional strengthening and adaptive comanagement,
while IPM training should be linked with natural resource management initiatives. These approaches may eventually improve
the way IPM is delivered to small-scale farmers who operate in the ecologically diverse environments of the tropics. 相似文献
690.
Eugenio Figueroa B. Enrique Calfucura T. 《Environment, Development and Sustainability》2010,12(5):647-667
Searching for practical means to assessing economic growth’s sustainability, we extend a standard theoretical model to calculate “true” income measures for Chile, during the 1985–2004 period, and use estimates of natural capital depreciation to obtain genuine national saving measures. We found that, for the period, Chile’s economic growth was sustainable, even when approximately 2.5% of the income recorded by national accounts corresponded to depreciation of natural resources plus costs of atmospheric pollution. This performance can be partially explained by policies implemented to force fiscal responsibility and to assure wise public investment and expending during a natural resource driven growth. This evidence reinforces recent findings contradicting the natural resource curse, and the indirect negative effect of resource abundance over growth that would operate through the quality of institutions. 相似文献