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901.
Brominated flame retardants and organochlorines in the European environment using great tit eggs as a biomonitoring tool 总被引:1,自引:0,他引:1
Van den Steen E Pinxten R Jaspers VL Covaci A Barba E Carere C Cichoń M Dubiec A Eeva T Heeb P Kempenaers B Lifjeld JT Lubjuhn T Mänd R Massa B Nilsson JA Norte AC Orell M Podzemny P Sanz JJ Senar JC Soler JJ Sorace A Török J Visser ME Winkel W Eens M 《Environment international》2009,35(2):310-317
Large-scale studies are essential to assess the emission patterns and spatial distribution of organohalogenated pollutants (OHPs) in the environment. Bird eggs have several advantages compared to other environmental media which have previously been used to map the distribution of OHPs. In this study, large-scale geographical variation in the occurrence of OHPs, such as polychlorinated biphenyls (PCBs), polybrominated diphenyl ethers (PBDEs) and organochlorine pesticides (OCPs), was investigated throughout Europe using eggs of a terrestrial residential passerine species, the great tit (Parus major). Great tit eggs from 22 sampling sites, involving urban, rural and remote areas, in 14 European countries were collected and analysed (5-8 eggs per sampling site). The environmentally most important congeners/compounds of the analysed pollutants were detectable in all sampling locations. For PCBs, PBDEs and OCPs, no clear geographical contamination pattern was found. Sum PCB levels ranged from 143 ng/g lipid weight (lw) to 3660 ng/g lw. As expected, PCB concentrations were significantly higher in the sampled urban compared to the remote locations. However, the urban locations did not show significantly higher concentrations compared to the rural locations. Sum PBDEs ranged from 4.0 ng/g lw to 136 ng/g lw. PBDEs were significantly higher in the urbanized sampling locations compared to the other locations. The significant, positive correlation between PCB and PBDE concentrations suggests similar spatial exposure and/or mechanisms of accumulation. Significantly higher levels of OCPs (sum OCPs ranging from 191 ng/g lw to 7830 ng/g lw) were detected in rural sampling locations. Contamination profiles of PCBs, PBDEs and OCPs differed also among the sampling locations, which may be due to local usage and contamination sources. The higher variance among sampling locations for the PCBs and OCPs, suggests that local contamination sources are more important for the PCBs and OCPs compared to the PBDEs. To our knowledge, this is the first study in which bird eggs were used as a monitoring tool for OHPs on such a large geographical scale. 相似文献
902.
Understanding the fate and transport of petroleum hydrocarbons from coal tar within gasholders 总被引:1,自引:0,他引:1
Coal tars have been identified as posing a threat to human health due to their toxic, mutagenic and carcinogenic characteristics. Workers involved in former gasholders decommissioning are potentially exposed to relevant concentrations of volatile and semi-volatile hydrocarbons upon opening up derelict tanks and during tar excavation/removal. While information on contaminated sites air-quality and its implications on medium-long term exposure is available, acute exposure issues associated with the execution of critical tasks are less understood. Calculations indicated that the concentration of a given contaminant in the gasholder vapour phase only depends on the coal tar composition, being only barely affected by the presence of water in the gasholder and the tar volume/void space ratio. Fugacity modelling suggested that risk-critical compounds such as benzene, naphthalene and other monocyclic and polycyclic aromatic hydrocarbons may gather in the gasholder air phase at significant concentrations. Gasholder emissions were measured on-site and compared with the workplace exposure limits (WELs) currently in use in UK. While levels for most of the toxic compounds were far lower than WELs, benzene air-concentrations where found to be above the accepted threshold. In addition due to the long exposure periods involved in gasholder decommissioning and the significant contribution given by naphthalene to the total coal tar vapour concentration, the adoption of a WEL for naphthalene may need to be considered to support operators in preventing human health risk at the workplace. The Level I fugacity approach used in this study demonstrated its suitability for applications to sealed environments such as gasholders and its further refining could provide a useful tool for land remediation risk assessors. 相似文献
903.
Humans can consume a number of types of biota tissues, which have varying propensities to accumulate radionuclides. As a result, depending upon the biota species, the radionuclide and the tissue under consideration, it may be necessary to estimate the percent radionuclide load in specific edible tissues, and in cases where whole organisms are consumed, to estimate the radionuclide load in the whole body of an organism, based on data that have been collected for individual tissues. To accomplish this, data were compiled that can be used to estimate the partitioning patterns and percent loads of various groups of elements in edible tissues of freshwater fishes. General trends in partitioning, such as those provided in this paper, can be used to predict radionuclide transfer to humans and the corresponding potential radiological dose to humans via dietary pathways, in this case following the consumption of fish. 相似文献
904.
J.T. Smith N.V. Sasina A.I. Kryshev N.V. Belova A.V. Kudelsky 《Journal of environmental radioactivity》2009
Empirical relations between the 90Sr concentration factor (CF) and the calcium concentration in freshwater aquatic systems have previously been determined in studies based on data obtained prior to the Chernobyl accident. The purpose of the present research is to review and compare these models, and to test them against a database of post-Chernobyl measurements from rivers and lakes in Ukraine, Russia, Belarus and Finland. It was found that two independently developed models, based on pre-Chernobyl empirical data, are in close agreement with each other, and with empirical data. Testing of both models against new data obtained after the Chernobyl accident confirms the models’ predictive ability. An investigation of the influence of fish size on 90Sr accumulation showed no significant relationship, though the data set was somewhat limited. 相似文献
905.
C. Naccari M. Cristani F. Cimino T. Arcoraci D. Trombetta 《Environment international》2009,35(3):594-598
The aim of this study was to evaluate the accumulation of toxic (As, Cd and Pb) and essential (Cu, Mn and Zn) metals in samples (feathers, liver, kidney, lung, intestine and muscle) of common buzzards (Buteo buteo) from Sicily, used as bio-indicators for monitoring environmental metals pollution. All samples of buzzards were collected at the “Recovery Center of Wild Fauna” of Palermo, through the Zooprophilactic Institute. The quantitative determinations of metals were carried out using an atomic absorbtion spectrophotometer (AAS). The results obtained showed the presence of metals in all samples analyzed. For toxic metals the highest levels of Pb and As were found in liver and those of Cd in kidney; for essential metals Zn levels were higher than Cu and Mn in all tissues analyzed. Significant differences are observed in metal levels between female and male and juvenile and adult bird samples.Highest metal levels found in liver, kidney and muscle can be considered indicative of chronic exposure to metals while the presence of metals in feathers can be consequential to storing and elimination processes. The results obtained suggest that common buzzards (Buteo buteo) may be very useful as bio-indicators for monitoring environmental pollution. 相似文献
906.
The influence of long-term exposure of model plantations at elevated atmospheric CO2 (550 ppm) on soil respiration under natural conditions has been studied using an automated Free-Air CO2 Enrichment (FACE) system at the Hokkaido University, Japan. In the course of the experiment, an attempt has been made to simulate the effect of forthcoming climate change on the process of CO2 emission from different soil types. 相似文献
907.
Keigo Akimoto Fuminori Sano Takashi Homma Kenichi Wada Miyuki Nagashima Junichiro Oda 《Sustainability Science》2012,7(2):157-168
This study focuses on analyses of greenhouse gas (GHG) emission reductions, from the perspective of interrelationships among
time points and countries, in order to seek effective reductions. We assessed GHG emission reduction potentials and costs
in 2020 and 2030 by country and sector, using a GHG emission reduction-assessment model of high resolution regarding region
and technology, and of high consistency with intertemporal, interregional, and intersectoral relationships. Global GHG emission
reduction potentials relative to baseline emissions in 2020 are 8.4, 14.7, and 18.9 GtCO2eq. at costs below 20, 50, and 100 $/tCO2eq., corresponding to +19, −2, and −7 %, respectively, relative to 2005. The emission reduction potential for 2030 is greater
than that for 2020, mainly because many energy supply and energy-intensive technologies have long lifetimes and more of the
current key facilities will be extant in 2020 than in 2030. The emission reduction potentials in 2030 are 12.6, 22.0, and
26.6 GtCO2eq. at costs below 20, 50, and 100 $/tCO2eq., corresponding to +19, −2, and −7 %, respectively, relative to 2005. The emission reduction potential for 2030 is greater
than that for 2020, mainly because many energy supply and energy-intensive technologies have long lifetimes and more of the
current key facilities will be extant in 2020 than in 2030. The emission reduction potentials in 2030 are 12.6, 22.0, and
26.6 GtCO2eq. at costs below 20, 50, and 100 /tCO2eq., corresponding to +33, +8, and −3 %, respectively, relative to 2005. Global emission reduction potentials at a cost below
50 $/tCO2eq. for nuclear power and carbon capture and storage are 2.3 and 2.2 GtCO2eq., respectively, relative to baseline emissions in 2030. Longer-term perspectives on GHG emission reductions toward 2030
will yield more cost-effective reduction scenarios for 2020 as well. 相似文献
908.
909.
The influence of socioeconomic, environmental, and demographic factors on municipality-scale land-cover change in Mexico 总被引:3,自引:0,他引:3
Martha Bonilla-Moheno T. Mitchell Aide Matthew L. Clark 《Regional Environmental Change》2012,12(3):543-557
Land-cover change is the result of complex multi-scale interactions between socioeconomic, demographic, and environmental factors. Demographic change, in particular, is thought to be a major driver of forest change. Most studies have evaluated these interactions at the regional or the national level, but few studies have evaluated these dynamics across multiple spatial scales within a country. In this study, we evaluated the effect of demographic, environmental, and socioeconomic variables on land-cover change between 2001 and 2010 for all Mexican municipalities (n?=?2,443) as well as by biome (n?=?4). We used a land-cover classification based on 250-m MODIS data to examine the change in cover classes (i.e., woody, mixed woody, and agriculture/herbaceous vegetation). We evaluated the trends of land-cover change and identified the major factors correlated with woody vegetation change in Mexico. At the national scale, the variation in woody vegetation was best explained by environmental variables, particularly precipitation; municipalities where woody cover increased tended to be in areas with low average annual precipitation (i.e., desert and dry forest biomes). Demographic variables did not contribute much to the model at the national scale. Elevation, temperature, and population density explained the change in woody cover when municipalities were grouped by biome (i.e., moist forest, dry forest, coniferous forest, and deserts). Land-cover change at the biome level showed two main trends: (1) the tropical moist biome lost woody vegetation to agriculture and herbaceous vegetation, and (2) the desert biome increased in woody vegetation within more open-canopy shrublands. 相似文献