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41.
The role of metals in dioxin formation from combustion of newspapers and polyvinyl chloride in an incinerator 总被引:3,自引:0,他引:3
Newspapers impregnated with NaCl mixed with various chloride metals (CuCl2, MgCl2, MnCl2, FeCl3, NiCl2, and CoCl2) and electric wire coated with polyvinyl chloride (PVC) were combusted in a well-controlled incinerator. Exhaust gas samples collected at the outlet of the incinerator were analyzed for dioxins (PCDDs, PCDFs, and coplanar PCBs) by gas chromatography/mass spectrometry. The amount of total dioxins formed from newspaper samples ranged from 34.2 ng/g (with NaCl+CoCl2) to 67.0 ng/g (with NaCl+CuCl2). PCDFs composed 88-94% of the total dioxins formed in the exhaust gases. The highest levels of PCDF isomers obtained were Cl3-CDF from the sample with NaCl+CuCl2 (14.8 ng/g), Cl2-CDF from the sample with NaCl+MgCl2 (12.3 ng/g), and Cl(1)-CDF from samples with NaCl+MnCl2 (12.6 ng/g), with NaCl+FeCl3 (11.8 ng/g), and with NaCl+NiCl2 (13.3 ng/g), and with NaCl+CoCl2 (8.62 ng/g). The total of Cl4-8-CDDs comprised 76-88% of the total Cl1-8-CDDs. In particular, Cl7-CDDs had the highest levels except for the sample with NaCl+NiCl2. Total dioxins formed from samples of electric wire coated with PVC and PVC alone were 38.3 ng/g and 112 ng/g, respectively, suggesting that the presence of copper reduced dioxin formation. 相似文献
42.
Takafumi Fujita Takayuki Kawano Liwei Huang Yoshihiro Kojima Hitoki Matsuda Koichi Ushiroebisu 《Journal of Material Cycles and Waste Management》2007,9(1):15-20
To control the emission of halides into the environment, an experiment on the nonthermal plasma decomposition of the halides
CF4, CHF3, C2HCl3, and CHClF2 was conducted in a wire-in-tube corona reactor. It was found that the decomposition of C2HCl3 and CHClF2 was easy compared with the decomposition of CF4 and CHF3. With the addition of H2 in N2 gas, the decomposition ratio of CF4, C2HCl3, and CHClF2 increased. In contrast, the decomposition ratio of CHF3 in a hydrogen-rich atmosphere was lower than that in an N2 atmosphere. It was demonstrated that the yields of HF and/or HCl formed during halide decomposition clearly increased in
the presence of H2 in N2 gas. Furthermore, in order to prevent the production of unwanted products from halide decomposition, a combination of plasma
decomposition and in situ alkaline absorption was devised by coating a layer of Ca(OH)2 onto the surface of the grounding electrode. It was demonstrated that the Ca(OH)2 sorbent played an effective role as a scavenger, participating in halide decomposition by capturing reaction products such
as HCl and HF, therefore resulting in increased halide decomposition. 相似文献
43.
Toshiyuki Nomura Shunsuke Araki Takanori Nagao Yasuhiro Konishi 《Journal of Material Cycles and Waste Management》2007,9(1):34-39
The dewatering of waste sludge continues to be a major problem in wastewater treatment. In this study, the solubilization
treatment of waste sludge and extracellular polymeric substances using a solubilizing reagent was examined experimentally.
For this purpose, a compression test of thickened waste sludge obtained after solubilization treatment was carried out. The
total solid content of the dewatered cake was over 30% when using hydrochloric acid or acetic acid as the solubilizing reagent;
however, it was about 20% when using sodium hydroxide. The thickened waste sludge was effectively solubilized when the concentration
of acetic acid in the sludge, assuming that it was diluted by free water and not bound water in the sludge, was greater than
0.3 kmol/m3. A flocculated sedimentation test using the supernatant water after solubilization treatment was also carried out, revealing
that it functions in a similar manner to commercial flocculant in aggregating solid particles under gravity. This result indicates
that the supernatant water can act as a bioflocculant. Methane fermentation of the supernatant water was subsequently carried
out. The findings showed that by using acetic acid as a solubilizing reagent, solubilized organic substances in the supernatant
water could be recovered as a bioenergy resource. 相似文献
44.
每年世界上都会发生大量森林火灾.虽然森林火灾对自然环境造成严重破坏,但现有的火灾防治措施仍不足以防止火灾发生.山区大的绿化区常常在强干燥空气条件下由于火蔓延的作用而被毁灭.很多案例中,尽管消防部门直升飞机和一般飞机被投入使用,仍需要花费很长时间来抑制大规模森林火灾.燃烧的木块可以很容易从下风方向的山脊越过山谷,并在强风作用下广为散播.因此,如何阻止由于燃烧木块而引发的快速火蔓延,是非常重要的研究课题.通常,当燃烧木块在新的地点点燃当地可燃物的初期,火势还是相对微弱的,尺寸也很小,因此,有可能可以在火灾早期借助直升飞机或一般飞机来以水攻火.本文的目标,就是研究在燃烧木块到达的下风区利用直升飞机和一般飞机中的水的方法.本文通过实验室实验和计算机模拟研究了阻止火从一个山脊蔓延到另一个下风方向的山脊的有效方法. 相似文献
45.
Effect of ultraviolet-absorbing vinyl film on organophosphorus insecticides dichlorvos and fenitrothion residues in spinach 总被引:3,自引:0,他引:3
Amano S Katami T Shibamoto T 《Journal of environmental science and health. Part. B》2002,37(4):291-296
Dichlorvos and fenitrothion residues found in spinach grown in greenhouse covered either by regular vinyl film or UV-absorbing vinyl film (UV-A) were analyzed by gas chromatography. After one day, dichlorvos residues in spinach covered with regular vinyl film and UV-A degraded by 97% and 80%, respectively, and degraded 100% after three days covered with regular vinyl film and six days covered with UV-A. After three days, fenitrothion residue in spinach covered with regular vinyl film degraded by 72% and then by 97% after six days; residue in spinach covered with UV-A degraded by 50% after three days and by 95% after six days. These results indicate that UV-A used to prevent the occurrence of insects and fungi in greenhouses reduced the degradation rates of dichlorvos and fenitrothion. 相似文献
46.
Takayuki Miura Julien Schaeffer Jean-Claude Le Saux Philippe Le Mehaute Françoise S. Le Guyader 《Food and environmental virology》2018,10(2):176-186
We investigated removal of noroviruses, sapoviruses, and rotaviruses in a full-scale membrane bioreactor (MBR) plant by monitoring virus concentrations in wastewater samples during two gastroenteritis seasons and evaluating the adsorption of viruses to mixed liquor suspended solids (MLSS). Sapoviruses and rotaviruses were detected in 25% of MBR effluent samples with log reduction values of 3- and 2-logs in geometric mean concentrations, respectively, while noroviruses were detected in only 6% of the samples. We found that norovirus and sapovirus concentrations in the solid phase of mixed liquor samples were significantly higher than in the liquid phase (P < 0.01, t test), while the concentration of rotaviruses was similar in both phases. The efficiency of adsorption of the rotavirus G1P[8] strain to MLSS was significantly less than norovirus GI.1 and GII.4 and sapovirus GI.2 strains (P < 0.01, t test). Differences in the adsorption of viruses to MLSS may cause virus type-specific removal during the MBR treatment process as shown by this study. 相似文献
47.
Leaching of heavy metals in acid mine drainage. 总被引:1,自引:0,他引:1
Acid mine drainage is one of the most serious environmental problems that the coal and metal mining industry is currently facing. The generation of low pH drainage enhances the dissolution of heavy metals in water. The samples used in this research originated from three pits at mine dumps. In a study reported in this paper, three types of tests; namely static test, kinetic test and column test were conducted to estimate acid generation and acid neutralization reaction rates, and to predict the solubility of metals and their release rates. Static test showed that all samples had a pH of net acid generation (NAG pH) <4, a net acid producing potential (NAPP) >10 kg H2SO4tonne(-1), and a S-content >3%, which can be classified as a high acid-forming capacity. Simulated runoff in the column tests was equivalent to 5-year average rainfall in Indonesia, the resultant leachates showed acidic behaviour (pH < 3.5). Based on the results, it was found that high mobilization of heavy metals (Cr, Cu, Zn, Cd and Pb) takes place under strong acidic conditions (pH approximately equal 2). 相似文献
48.
Masahiro Shimada Takahiko Iida Kensuke Kawarada Takayuki Okayama Masami Fushitani 《Journal of Material Cycles and Waste Management》2001,3(2):135-143
We have already reported the adsorptivity and pore structure of activated carbon made from waste newspaper in order to use
the waste paper for purposes other than paper-making stock. However, manufacturing the activated carbon may not necessarily
be an advantageous method based on environmental concerns and the effective use of the resource because the reaction during
the activating process is endothermic and the amount of carbon consumed is significant. Here, we examine the pore structure
and adsorption properties of waste newspaper used as an adsorbent in the form of a carbonized material. Waste newspaper was
carbonized for 2 h in the temperature range 400°–1000°C. The specific surface area of the carbonized material obtained, 418 m2/g, was highest for the sample carbonized at 800°C, which was equal to or greater than that of commercially available charcoal.
Moreover, the iodine adsorption number of 581 mg/g was the highest and the rate of adsorption was the fastest for the sample
carbonized at 800°C. However, the humidity control capability was highest for the material carbonized at 600°–700°C. It has
been determined that it is advantageous to carbonize waste paper at 800°C in order to use the carbonized material as an adsorbent,
while carbonization at 600°–700°C is more advantageous for use as a humidity control material.
Received: June 23, 2000 / Accepted: January 17, 2001 相似文献
49.
Masahiro Shimada Takahiko Iida Kensuke Kawarada Yoshifumi Chiba Toshihiro Mamoto Takayuki Okayama 《Journal of Material Cycles and Waste Management》2000,2(2):100-108
In an earlier report, we presented a method for preparing activated carbon from waste newspaper as a way to recycle used paper
for a purpose other than producing raw material for paper-making. In this article, we consider the porous structure of the
activated carbon that affects its adsorption properties for various substances. The specific surface area of activated carbon
prepared from waste newspaper was 838 m2/g, the micropore volume was 0.368 ml/g, and the mesopore volume was 0.138 ml/g, which is about the same as commercially available
activated carbon. The activated carbon prepared from waste newspaper usually has a high content of ash, which makes little
contribution to the adsorption properties. In particular, as compared with reagent-activated carbon, the quantities of mesopores
with a pore radius of 3–25 nm and macropores with a pore radius of 25–250 nm were 8 and 14 times larger, respectively. Activated
carbon prepared from waste newspaper has a well-developed porous structure, particularly in the mesopore and macropore ranges.
Received: July 12, 1999 / Accepted: March 8, 2000 相似文献
50.
Takahiro Yamaguchi Masahiro Okihashi Yoshimasa Konishi Kotaro Uchida Mai Hoang Ngoc Do 《Journal of environmental science and health. Part. B》2017,52(6):430-433
The residual levels of antibiotics in Vietnamese eggs were monitored from 2014 to 2015. A total of 111 egg packages, distributed by 11 different companies, were collected from supermarkets in Ho Chi Minh City and the levels of 28 antibiotics were analyzed using liquid chromatography-tandem mass spectrometry (LC-MS/MS) screening method. Sixteen samples tested positive for antibiotics; a total of eight compounds (enrofloxacin, ciprofloxacin, norfloxacin, sulfadimethoxine, sulfamethazine, sulfamonomethoxine, tilmicosin and trimethoprim) were detected. Enrofloxacin was detected in eight samples, with two samples exhibiting concentrations exceeding 1,000 µg kg?1. Tilmicosin was detected in three samples at a range of 49–568 µg kg?1. We observed that two of the 11 companies frequently sold antibiotic-contaminated eggs (detection rates of 56 and 60%), suggesting that a number of companies do not regulate the use of antibiotics in egg-laying hens. Our findings indicate that livestock farmers require instruction regarding antibiotic use and that continual antibiotic monitoring is essential in Vietnam. 相似文献