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71.
建立了固相萃取(SPE)/气相色谱质谱(GC/MS)联用检测灰尘中氯代多环芳烃(ClPAHs)的方法.以正己烷和二氯甲烷混合液为提取溶剂,索氏提取灰尘样品中的20种ClPAHs,活性硅胶层析柱与活性炭混合硅胶SPE柱协同净化.净化后的提取液采用GC/MS测定,SIM模式扫描,并用质谱特征离子定量分析.结果表明,填充量为0.2 g(W(活性炭)∶W(硅胶)=1∶40)的活性炭混合硅胶SPE小柱能有效地将ClPAHs分离出来,载样后采用反向溶剂洗脱,既提高了回收率又减少了洗脱剂甲苯的用量,净化效果好.处理灰尘样品后检测分析,20种ClPAHs的平均回收率稳定在60.4%—120.1%,相关系数>0.99,检出限为0.04—0.17 ng.g-1,相对标准偏差为1.6%—10.2%.本方法前处理简单,定性、定量准确可靠,可广泛应用于环境介质中氯代多环芳烃的检测. 相似文献
72.
73.
Effects of Nitrogen Supply on the Sensitivity to O3 of Growth and Photosynthesis of Japanese Beech (Fagus crenata) Seedlings 总被引:1,自引:0,他引:1
Masahiro Yamaguchi Makoto Watanabe Naoki Matsuo Junichi Naba Ryo Funada Motohiro Fukami Hideyuki Matsumura Yoshihisa Kohno Takeshi Izuta 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):131-136
To obtain basic information for evaluating critical levels of O3 under different nitrogen loads for protecting Japanese beech forests, two-year-old seedlings of Fagus crenata Blume were grown in potted andisol supplied with N as NH4NO3 solution at 0, 20 or 50 kg ha−1 year−1 and exposed to charcoal-filtered air or O3 at 1.0, 1.5 and 2.0 times the ambient concentration from 16 April to 22 September 2004. The O3 induced significant reductions in the whole-plant dry mass, net photosynthetic rate at 380 μmol mol−1 CO2 (A
380), carboxylation efficiency (CE) and concentrations of ribulose-1,5-bisphosphate carboxylase/oxygenase (Rubisco) and total soluble protein (TSP) in the leaves.
The concentrations of Rubisco and TSP were negatively correlated with the concentration of leaf acidic amino acid, suggesting
that O3 enhanced the degradation of protein such as Rubisco. The N supply to the soil did not significantly change the whole-plant
dry mass and A
380, whereas it significantly increased the CE and concentrations of Rubisco and total amino acid. No significant interactive effects of O3 and N supply to the soil were detected on the growth, photosynthetic parameters and concentrations of protein and amino acid
in the leaves. In conclusion, N supply to the soil at ≤50 kg ha−1 year−1 does not significantly change the sensitivity to O3 of growth and net photosynthesis of Fagus crenata seedlings. 相似文献
74.
Cyanogen chloride was formed by the reaction of humic acid with hypochlorous acid in the presence of ammonium ion. Furthermore, cyanogen chloride was also formed when ammonium ion and hypochlorous acid were added to raw water sampled at water treatment plants. 相似文献
75.
Sunamura E Hoshizaki S Sakamoto H Fujii T Nishisue K Suzuki S Terayama M Ishikawa Y Tatsuki S 《Die Naturwissenschaften》2011,98(5):361-368
Some invasive ants form large networks of mutually non-aggressive nests, i.e., supercolonies. The Argentine ant Linepithema humile forms much larger supercolonies in introduced ranges than in its native range. In both cases, it has been shown that little gene flow occurs between supercolonies of this species, though the mechanism of gene flow restriction is unknown. In this species, queens do not undertake nuptial flight, and males have to travel to foreign nests and cope with workers before gaining access to alien queens. In this study, we hypothesized that male Argentine ants receive interference from workers of alien supercolonies. To test this hypothesis, we conducted behavioral and chemical experiments using ants from two supercolonies in Japan. Workers attacked males from alien supercolonies but not those from their own supercolonies. The level of aggression against alien males was similar to that against alien workers. The frequency of severe aggression against alien males increased as the number of recipient workers increased. Cuticular hydrocarbon profiles, which serve as cues for nestmate recognition, of workers and males from the same supercolony were very similar. Workers are likely to distinguish alien males from males of their own supercolony using the profiles. It is predicted that males are subject to considerable aggression from workers when they intrude into the nests of alien supercolonies. This may be a mechanism underlying the restricted gene flow between supercolonies of Argentine ants. The Argentine ant may possess a distinctive reproductive system, where workers participate in selecting mates for their queens. We argue that the aggression of workers against alien males is a novel form of reproductive interference. 相似文献
76.
Takeshi Osawa Kazuhisa Yamasaki Ken Tabuchi Akira Yoshioka Mayura B. Takada 《Ambio》2018,47(7):806-815
Detecting dispersal pathways is important both for understanding species range expansion and for managing nuisance species. However, direct detection is difficult. Here, we propose detecting these crucial pathways using a virtual ecology approach, simulating species dynamics using models, and virtual observations. As a case study, we developed a dispersal model based on cellular automata for the pest insect Stenotus rubrovittatus and simulated its expansion. We tested models for species expansion based on four landscape parameters as candidate pathways; these are river density, road density, area of paddy fields, and area of abandoned farmland, and validated their accuracy. We found that both road density and abandoned area models had prediction accuracy. The simulation requires simple data only to have predictive power, allowing for fast modeling and swift establishment of management plans. 相似文献
77.
The recycling of waste plastics is important for the prevention of the exhaustion of fossil resources. In this paper, recycling techniques of carbon fiber-reinforced plastic (CFRP) using supercritical and subcritical fluids were reviewed. The matrix resin of CFRP such as epoxy resin or resol resin was decomposed by supercritical and subcritical fluids, and the carbon fiber without thermal damage was recovered from CFRP. Mainly, water or alcohol was used as decomposition medium. 相似文献
78.
Takeshi Itakura Kazumasa Hirata Masanori Aoki Ryo Sasai Hisao Yoshida Hideaki Itoh 《Environmental Chemistry Letters》2009,7(4):343-345
We demonstrated a complete decomposition method for ionic liquids (ILs; organic cation part: butyl-methyl or ethyl-methyl
imidazolium, and inorganic anion part: PF6 −, BF4
− or Br−) in aqueous media by combining a hydrothermal mineralization method with a photocatalytic decomposition (PD) method. As a
result, the hydrothermal treatment with Ca(OH)2 mineralizer could effectively remove the inorganic anion part, such as PF6
− or BF4
− and the PD could decompose the organic cation part effectively. Therefore, the detoxification of ILs in aqueous media was
accomplished by the present method. 相似文献
79.
Shinya Inazumi Hiroyasu Ohtsu Tomoki Shiotani Takeshi Katsumi 《Journal of Material Cycles and Waste Management》2011,13(2):139-149
It is very important that waste should be controlled and appropriately handled in a waste disposal stream, considering its
impact on the environment. In this research, the LCA-EA model was applied to the current waste disposal stream of the BMR
as well as other waste disposal stream scenarios, so that treatment cost, environmental load and environmental cost were assessed
quantatively. The results of this study showed that in the current waste diposal stream in Bangkok, there were large contributions
from carbon dioxide and methane to the greenhouse gas emissions from the stream. The study was able to quantify the reductions
in environmental load associated with various waste disposal stream scenarios, using the baseline scenario as a standard. 相似文献
80.
Radon adsorption by activated charcoal collectors such as PicoRad radon detectors is known to be largely affected by temperature and relative humidity. Quantitative models are, however, still needed for accurate radon estimation in a variable environment. Here we introduce a temperature calibration formula based on the gas adsorption theory to evaluate the radon concentration in air from the average temperature, collection time, and liquid scintillation count rate. On the basis of calibration experiments done by using the 25 m3 radon chamber available at the National Institute of Radiological Sciences in Japan, we found that the radon adsorption efficiency may vary up to a factor of two for temperatures typical of indoor conditions. We expect our results to be useful for establishing standardized protocols for optimized radon assessment in dwellings and workplaces. 相似文献