全文获取类型
收费全文 | 3091篇 |
免费 | 43篇 |
国内免费 | 25篇 |
专业分类
安全科学 | 164篇 |
废物处理 | 155篇 |
环保管理 | 623篇 |
综合类 | 353篇 |
基础理论 | 743篇 |
环境理论 | 5篇 |
污染及防治 | 766篇 |
评价与监测 | 216篇 |
社会与环境 | 116篇 |
灾害及防治 | 18篇 |
出版年
2023年 | 22篇 |
2022年 | 37篇 |
2021年 | 26篇 |
2020年 | 21篇 |
2019年 | 32篇 |
2018年 | 67篇 |
2017年 | 68篇 |
2016年 | 89篇 |
2015年 | 59篇 |
2014年 | 84篇 |
2013年 | 292篇 |
2012年 | 144篇 |
2011年 | 181篇 |
2010年 | 121篇 |
2009年 | 125篇 |
2008年 | 162篇 |
2007年 | 189篇 |
2006年 | 157篇 |
2005年 | 108篇 |
2004年 | 106篇 |
2003年 | 119篇 |
2002年 | 89篇 |
2001年 | 67篇 |
2000年 | 47篇 |
1999年 | 51篇 |
1998年 | 39篇 |
1997年 | 43篇 |
1996年 | 44篇 |
1995年 | 40篇 |
1994年 | 43篇 |
1993年 | 34篇 |
1992年 | 37篇 |
1991年 | 26篇 |
1990年 | 29篇 |
1989年 | 20篇 |
1988年 | 14篇 |
1987年 | 20篇 |
1986年 | 26篇 |
1985年 | 17篇 |
1984年 | 18篇 |
1983年 | 29篇 |
1982年 | 29篇 |
1981年 | 27篇 |
1980年 | 19篇 |
1979年 | 18篇 |
1977年 | 11篇 |
1976年 | 9篇 |
1975年 | 11篇 |
1974年 | 11篇 |
1971年 | 11篇 |
排序方式: 共有3159条查询结果,搜索用时 171 毫秒
181.
Timothy J. Pac James Baldock Brendan Brodie Jennifer Byrd Beatriz Gil Kevin A. Morris Denice Nelson Jaydeep Parikh Paulo Santos Miguel Singer Alan Thomas 《补救:环境净化治理成本、技术与工艺杂志》2019,29(2):75-91
This paper compiles a detailed set of in situ chemical oxidation (ISCO) lessons learned pertaining to design, execution, and safety based on global experiences over the last 20 years. While the benefits of a “correct” application are known (e.g., cost effectiveness, speed, permanence of treatment), history also provides examples of a variety of “incorrect” applications. These provide an opportunity to highlight recurring themes that resulted in failures. ISCO is, and will continue to provide, an important remedial tool for site remediation, particularly as a component of a multifaceted approach for addressing large and complex sites. Future success, however, requires an objective understanding of both the benefits and the limitations of the technology. The ability to learn from the mistakes of the past provides an opportunity to eliminate, or at least minimize, them in the future. Over the last 25 years of ISCO application, process understanding and knowledge have improved and evolved. This paper combines a thorough discussion of lessons learned through decades of ISCO implementation throughout all aspects of ISCO projects with an analysis of changes to the ISCO remediation market. By discussing the interplay of these two themes and providing recommendations from collective lessons learned, we hope to improve the future of safe, cost‐effective, and successful applications of ISCO. 相似文献
182.
Alberto Giubilini Patrick Birkl Thomas Douglas Julian Savulescu Hannah Maslen 《Journal of Agricultural and Environmental Ethics》2017,30(2):179-198
Antibiotic use in animal farming is one of the main drivers of antibiotic resistance both in animals and in humans. In this paper we propose that one feasible and fair way to address this problem is to tax animal products obtained with the use of antibiotics. We argue that such tax is supported both by (a) deontological arguments, which are based on the duty individuals have to compensate society for the antibiotic resistance to which they are contributing through consumption of animal products obtained with the use of antibiotics; and (b) a cost-benefit analysis of taxing such animal products and of using revenue from the tax to fund alternatives to use of antibiotics in animal farming. Finally, we argue that such a tax would be fair because individuals who consume animal products obtained with the use of antibiotics can be held morally responsible, i.e. blameworthy, for their contribution to antibiotic resistance, in spite of the fact that each individual contribution is imperceptible. 相似文献
183.
Tobias Frische Michael Faust Wiebke Meyer Thomas Backhaus 《Environmental science and pollution research international》2009,16(5):593-603
Background, aim and scope
Estrogenic and non-estrogenic chemicals typically co-occur in the environment. Interference by non-estrogenic chemicals may confound the assessment of the actual estrogenic activity of complex environmental samples. The aim of the present study was to investigate whether, in which way and how seriously the estrogenic activity of single estrogens and the observed and predicted joint action of estrogenic mixtures is influenced by toxic masking and synergistic modulation caused by non-estrogenic chemical confounders.Materials and methods
The yeast estrogen screen (YES) was adapted so that toxicity and estrogenicity could be quantified simultaneously in one experimental run. Mercury, two organic solvents (dimethyl sulfoxide (DMSO) and 2,4-dinitroaniline), a surfactant (LAS-12) and the antibiotic cycloheximide were selected as toxic but non-estrogenic test chemicals. The confounding impact of selected concentrations of these toxicants on the estrogenic activity of the hormone 17ß-estradiol was determined by co-incubation experiments. In a second step, the impact of toxic masking and synergistic modulation on the predictability of the joint action of 17ß-estradiol, estrone and estriol mixtures by concentration addition was analysed.Results
Each of the non-estrogenic chemicals reduced the apparent estrogenicity of both single estrogens and their mixtures if applied at high, toxic concentrations. Besides this common pattern, a highly substance- and concentration-dependent impact of the non-estrogenic toxicants was observable. The activity of 17ß-estradiol was still reduced in the presence of only low or non-toxic concentrations of 2,4-dinitroaniline and cycloheximide, which was not the case for mercury and DMSO. A clear synergistic modulation, i.e. an enhanced estrogenic activity, was induced by the presence of slightly toxic concentrations of LAS-12. The joint estrogenic activity of the mixture of estrogens was affected by toxic masking and synergistic modulation in direct proportion to the single estrogens, which allowed for an adequate adaptation of concentration addition and thus unaffected predictability of the joint estrogenicity in the presence of non-estrogenic confounders.Discussion
The modified YES proved to be a reliable system for the simultaneous quantification of yeast toxicity and estrogen receptor activation. Experimental results substantiate the available evidence for toxic masking as a relevant phenomenon in estrogenicity assessment of complex environmental samples. Synergistic modulation of estrogenic activity by non-estrogenic confounders might be of lower importance. The concept of concentration addition is discussed as a valuable tool for estrogenicity assessment of complex mixtures, with deviations of the measured joint estrogenicity from predictions indicating the need for refined analyses.Conclusions
Two major challenges are to be considered simultaneously for a reliable analysis of the estrogenic activity of complex mixtures: the identification of known and suspected estrogenic compounds in the sample as well as the substance- and effect-level-dependent confounding impact of non-estrogenic toxicants.Recommendations and perspectives
The application of screening assays such as the YES to complex mixtures should be accompanied by measures that safeguard against false negative results which may be caused by non-estrogenic but toxic confounders. Simultaneous assessments of estrogenicity and toxicity are generally advisable. 相似文献184.
Richard Bindler Ingemar Renberg Thomas Andrén 《Environmental pollution (Barking, Essex : 1987)》2009,157(7):2132-2141
Metal pollution is viewed as a modern problem that began in the 19th century and accelerated through the 20th century; however, in many parts of the globe this view is wrong. Here, we studied past waterborne metal pollution in lake sediments from the Bergslagen region in central Sweden, one of many historically important mining regions in Europe. With a focus on lead (including isotopes), we trace mining impacts from a local scale, through a 120-km-long river system draining into Mälaren - Sweden's third largest lake, and finally also the Baltic Sea. Comparison of sediment and peat records shows that pollution from Swedish mining was largely waterborne and that atmospheric deposition was dominated by long-range transport from other regions. Swedish ore lead is detectable from the 10th century, but the greatest impact occurred during the 16th-18th centuries with improvements occurring over recent centuries, i.e., historical pollution > modern industrial pollution. 相似文献
185.
Mechanistic effect models for ecological risk assessment of chemicals (MEMoRisk)—a new SETAC-Europe Advisory Group 总被引:1,自引:1,他引:0
186.
Claire L. Martin Ian D. Longley James R. Dorsey Rick M. Thomas Martin W. Gallagher Eiko Nemitz 《Atmospheric environment (Oxford, England : 1994)》2009,43(31):4714-4721
Little information is known about the behaviour of ultrafine particles (UFP) on a citywide scale. Total particle number flux, dominated by UFP, and other meteorological parameters were collected from tower sites in Manchester, London, Edinburgh and Gothenburg between 1999 and 2006 using the eddy covariance technique. Averaged diurnal cycles were produced for particle number flux, concentration, sensible heat flux, emission velocity, friction velocity, wind speed and temperature. UFP flux cycles showed clear diurnal trends which were linked to traffic activity and local sources. Wind sector analysis showed contributions to flux from local heavily urbanised areas. A simple parameterised model linking UFP flux to traffic activity, sensible heat and friction velocity above the city was produced. 相似文献
187.
Anna Rabinovich Thomas A. Morton Tom Postmes Bas Verplanken 《Journal of environmental psychology》2009
This paper investigated the effect of goal and mindset specificity on goal-related behavior in the environmental domain. Two studies demonstrated that goal-related behavior was maximized when participants focused on an abstract goal in combination with a specific mindset, or when they focused on a specific goal in combination with an abstract mindset. When goals and mindsets instead matched in terms of abstractness, goal-related behavior was reduced. Study 2 demonstrated that the effect of goal specificity on behavior was mediated by different processes in each of the mindset conditions. When mindsets were abstract, self-efficacy mediated the positive effect of specific goals on behavior; when mindsets were specific, the value of collective environmental action mediated the positive effect of abstract goals on behavior. The results are discussed in the framework of a complementarity approach. It is argued that complementarity of levels of specificity of goals and mindsets may affect behavior particularly strongly in domains where the discrepancy between the abstract and the specific is large (e.g. the environmental domain). 相似文献
188.
Thomas G. Measham 《Environmental management》2009,43(6):1096-1107
Conventional approaches to evaluation of environmental programs have tended to limit themselves to restricted measures of
program effectiveness. This paper shows how a social learning approach can be incorporated into evaluating public environmental
programs. A social learning approach is particularly suited to complex environmental challenges which are inherently difficult
to understand, predict, and manage, thus complicating the evaluation process. The paper presents an Australian case study
of dryland salinity management where there are major knowledge barriers impeding conventional management techniques. The research
presented in this paper focused on evaluating a public demonstration program to track its impact through its design, implementation,
and monitoring phases. The paper shows that, by incorporating social learning principles and practices, program evaluation
can promote collective action, critical reflection, and increased knowledge to underpin improved environmental management. 相似文献
189.
Brominated flame retardants and organochlorines in the European environment using great tit eggs as a biomonitoring tool 总被引:1,自引:0,他引:1
Van den Steen E Pinxten R Jaspers VL Covaci A Barba E Carere C Cichoń M Dubiec A Eeva T Heeb P Kempenaers B Lifjeld JT Lubjuhn T Mänd R Massa B Nilsson JA Norte AC Orell M Podzemny P Sanz JJ Senar JC Soler JJ Sorace A Török J Visser ME Winkel W Eens M 《Environment international》2009,35(2):310-317
Large-scale studies are essential to assess the emission patterns and spatial distribution of organohalogenated pollutants (OHPs) in the environment. Bird eggs have several advantages compared to other environmental media which have previously been used to map the distribution of OHPs. In this study, large-scale geographical variation in the occurrence of OHPs, such as polychlorinated biphenyls (PCBs), polybrominated diphenyl ethers (PBDEs) and organochlorine pesticides (OCPs), was investigated throughout Europe using eggs of a terrestrial residential passerine species, the great tit (Parus major). Great tit eggs from 22 sampling sites, involving urban, rural and remote areas, in 14 European countries were collected and analysed (5-8 eggs per sampling site). The environmentally most important congeners/compounds of the analysed pollutants were detectable in all sampling locations. For PCBs, PBDEs and OCPs, no clear geographical contamination pattern was found. Sum PCB levels ranged from 143 ng/g lipid weight (lw) to 3660 ng/g lw. As expected, PCB concentrations were significantly higher in the sampled urban compared to the remote locations. However, the urban locations did not show significantly higher concentrations compared to the rural locations. Sum PBDEs ranged from 4.0 ng/g lw to 136 ng/g lw. PBDEs were significantly higher in the urbanized sampling locations compared to the other locations. The significant, positive correlation between PCB and PBDE concentrations suggests similar spatial exposure and/or mechanisms of accumulation. Significantly higher levels of OCPs (sum OCPs ranging from 191 ng/g lw to 7830 ng/g lw) were detected in rural sampling locations. Contamination profiles of PCBs, PBDEs and OCPs differed also among the sampling locations, which may be due to local usage and contamination sources. The higher variance among sampling locations for the PCBs and OCPs, suggests that local contamination sources are more important for the PCBs and OCPs compared to the PBDEs. To our knowledge, this is the first study in which bird eggs were used as a monitoring tool for OHPs on such a large geographical scale. 相似文献
190.
Aourell Mauffret André Rottiers Thomas Federle David C. Gillan Miriam Hampel Julian Blasco Ali Temara 《Environment international》2009,35(6):885-892
An innovative biodegradation test system was developed in order to fill the current gap for cost effective and environmentally relevant tools to assess marine biodegradability. Glass beads were colonized by a biofilm in an open flow-through system of seawater with continuous pre-exposure to Linear Alkylbenzene Sulfonate (LAS) (20 μg/L). Thereafter, such colonized beads were added as inoculum in different test systems. [14C]-LAS (5–100 μg/L) was added and primary and ultimate biodegradation were assessed. The bacterial density collected on the beads (109 bact./mL beads) was ca. 3 orders of magnitude higher than the typical seawater content. The LAS mineralization lag phase duration decreased from 55 to < 1 days and the mineralization extent increased from 53 to 90% as the colonized beads volume increased from 10 to 275 mL. This is the first demonstration of marine bacteria's ability to mineralize LAS. On the opposite, less than 13% LAS was mineralized in seawater only. The colonized beads possibly enhanced the probability to encounter the full degraders' consortium in a low volume of seawater (100 mL). 相似文献