全文获取类型
收费全文 | 2349篇 |
免费 | 18篇 |
国内免费 | 20篇 |
专业分类
安全科学 | 64篇 |
废物处理 | 100篇 |
环保管理 | 253篇 |
综合类 | 890篇 |
基础理论 | 370篇 |
环境理论 | 2篇 |
污染及防治 | 473篇 |
评价与监测 | 136篇 |
社会与环境 | 92篇 |
灾害及防治 | 7篇 |
出版年
2022年 | 27篇 |
2021年 | 32篇 |
2020年 | 21篇 |
2019年 | 23篇 |
2018年 | 41篇 |
2017年 | 42篇 |
2016年 | 35篇 |
2015年 | 39篇 |
2014年 | 52篇 |
2013年 | 98篇 |
2012年 | 93篇 |
2011年 | 104篇 |
2010年 | 70篇 |
2009年 | 91篇 |
2008年 | 79篇 |
2007年 | 102篇 |
2006年 | 76篇 |
2005年 | 83篇 |
2004年 | 90篇 |
2003年 | 73篇 |
2002年 | 69篇 |
2001年 | 42篇 |
2000年 | 28篇 |
1999年 | 21篇 |
1998年 | 33篇 |
1997年 | 17篇 |
1996年 | 22篇 |
1995年 | 32篇 |
1994年 | 24篇 |
1993年 | 16篇 |
1992年 | 20篇 |
1990年 | 21篇 |
1989年 | 15篇 |
1984年 | 15篇 |
1983年 | 14篇 |
1965年 | 17篇 |
1964年 | 15篇 |
1963年 | 25篇 |
1962年 | 18篇 |
1961年 | 14篇 |
1960年 | 23篇 |
1959年 | 24篇 |
1958年 | 16篇 |
1957年 | 16篇 |
1956年 | 14篇 |
1955年 | 28篇 |
1954年 | 33篇 |
1953年 | 19篇 |
1952年 | 14篇 |
1951年 | 24篇 |
排序方式: 共有2387条查询结果,搜索用时 31 毫秒
131.
De Laender F Van den Brink PJ Janssen CR 《Environmental pollution (Barking, Essex : 1987)》2011,159(10):3009-3017
An extensive data set describing effects of the herbicide linuron on macrophyte-dominated microcosms was analysed with a food web model to assess effects on ecosystem functioning. We showed that sensitive phytoplankton and periphyton groups in the diets of heterotrophs were gradually replaced by more tolerant phytoplankton species as linuron concentrations increased. This diet shift--showing redundancy among phytoplankton species--allowed heterotrophs to maintain their functions in the contaminated microcosms. On an ecosystem level, total gross primary production was up to hundred times lower in the treated microcosms but the uptake of dissolved organic carbon by bacteria and mixotrophs was less sensitive. Food web efficiency was not consistently lower in the treated microcosms. We conclude that linuron predominantly affected the macrophytes but did not alter the overall functioning of the surrounding planktonic food web. Therefore, a risk assessment that protects macrophyte growth also protects the functioning of macrophyte-dominated microcosms. 相似文献
132.
Muchitsch N Van Nooten T Bastiaens L Kjeldsen P 《Journal of contaminant hydrology》2011,126(3-4):258-270
An important issue of concern for permeable reactive iron barriers is the long-term efficiency of the barriers due to the long operational periods required. Mineral precipitation resulting from the anaerobic corrosion of the iron filings and bacteria present in the barrier may play an important role in the long-term performance. An integrated study was performed on the Vapokon permeable reactive barrier (PRB) in Denmark by groundwater and iron core sample characterization. The detailed field groundwater sampling carried out from more than 75 well screens up and downstream the barrier showed a very efficient removal (>99%) for the most important CAHs (PCE, TCE and 1,1,1-TCA). However, significant formation of cis-DCE within the PRB resulted in an overall insufficient efficiency for cis-DCE removal. The detailed analysis of the upstream groundwater revealed a very heterogeneous spatial distribution of contaminant loading into the PRB, which resulted in that only about a quarter of the barrier system is treating significant loads of CAHs. Laboratory batch experiments using contaminated groundwater from the site and iron material from the core samples revealed that the aged iron material performed equally well as virgin granular iron of the same type based on determined degradation rates despite that parts of the cored iron material were covered by mineral precipitates (especially iron sulfides, carbonate green rust and aragonite). The PCR analysis performed on the iron core samples indicated the presence of a microbial consortium in the barrier. A wide range of species were identified including sulfate and iron reducing bacteria, together with Dehalococcoides and Desulfuromonas species indicating microbial reductive dehalogenation potential. The microbes had a profound effect on the performance of the barrier, as indicated by significant degradation of dichloromethane (which is typically unaffected by zero valent iron) within the barrier. 相似文献
133.
Plant communities in relation to flooding and soil contamination in a lowland Rhine River floodplain
Schipper AM Lotterman K Leuven RS Ragas AM de Kroon H Hendriks AJ 《Environmental pollution (Barking, Essex : 1987)》2011,159(1):182-189
Using canonical correspondence analysis (CCA), relationships were investigated between plant species composition and flooding characteristics, heavy metal contamination and soil properties in a lowland floodplain of the Rhine River. Floodplain elevation and yearly average flooding duration turned out to be more important for explaining variation in plant species composition than soil heavy metal contamination. Nevertheless, plant species richness and diversity showed a significant decrease with the level of contamination. As single heavy metal concentrations seemed mostly too low for causing phytotoxic effects in plants, this trend is possibly explained by additive effects of multiple contaminants or by the concomitant influences of contamination and non-chemical stressors like flooding. These results suggest that impacts of soil contamination on plants in floodplains could be larger than expected from mere soil concentrations. In general, these findings emphasize the relevance of analyzing effects of toxic substances in concert with the effects of other relevant stressors. 相似文献
134.
Contaminants in the coastal karst aquifer system along the Caribbean coast of the Yucatan Peninsula, Mexico 总被引:1,自引:0,他引:1
Metcalfe CD Beddows PA Bouchot GG Metcalfe TL Li H Van Lavieren H 《Environmental pollution (Barking, Essex : 1987)》2011,159(4):991-997
Intensive land development as a result of the rapidly growing tourism industry in the “Riviera Maya” region of the Yucatan Peninsula, Mexico may result in contamination of groundwater resources that eventually discharge into Caribbean coastal ecosystems. We deployed two types of passive sampling devices into groundwater flowing through cave systems below two communities to evaluate concentrations of contaminants and to indicate the possible sources. Pharmaceuticals and personal care products accumulated in the samplers could only have originated from domestic sewage. PAHs indicated contamination by runoff from highways and other impermeable surfaces and chlorophenoxy herbicides accumulated in samplers deployed near a golf course indicated that pesticide applications to turf are a source of contamination. Prevention and mitigation measures are needed to ensure that expanding development does not impact the marine environment and human health, thus damaging the tourism-based economy of the region. 相似文献
135.
136.
Van der Eerden LJ Lekkerkerk LJ Smeulders SM Jansen AE 《Environmental pollution (Barking, Essex : 1987)》1992,76(1):1-9
Three-year-old Douglas firs (Pseudotsuga menziesii) were fumigated with 180 microg m(-3) NH3 or clean (charcoal-filtered) air. During these fumigations the plants received 15 mm artificial rain weekly, supplemented with 20, 500 or 2500 micromol litre(-1) (NH4)2SO4. Exposure to NH3 and NH4+ for 14 weeks resulted in a change of the nutrient status of the needles. The most remarkable effect was the increase in the N/K ratio, due to both uptake of N and leaching of K. The action of NH3 was stronger than that of NH4+. Both NH3 and (NH4)2SO4 affected the epicuticular wax layer and decreased mycorhiza frequency. Following fumigation and artificial rain treatments, needles were incubated for 8 h in a medium containing 0, 50, 250, 500 and 2500 micromol litre(-1) (NH4)2SO4. Almost no exchange of Ca, Mg and K for NH4+ was found. Therefore this ion exchange probably explains only a minor part of the changes in nutrient status of the whole trees. 相似文献
137.
John I. “Hans” Gilderbloom Gregory D. Squires William Riggs Stella Čapek 《Local Environment》2017,22(7):894-899
Each year governments and industry around the globe spend billions of dollars in search of treatments and cures for diseases that shorten lives, which often means gadgets, implants, radiation and pills. These “cures”, do not get to the root of the problem. Perhaps it is time for us to adjust our thinking to be more proactive instead of reactive in public health. Perhaps we need to consider confronting environmental pollution of air, soil and water at a local level. As the Physicians for Social Responsibility point out, we should be “preventing what we cannot cure”. One such preventive measure is ensuring that our communities, including our poor inner-city neighbourhoods, enjoy a clean environment. We challenge local and national policy-makers to respond to the global call and to take action to address environmental toxins; to take local action to ameliorate the pollution of the air, water and soil in so many of our nation’s neighbourhoods. A person’s neighbourhood, and the proximity of dangerous environmental contaminants within it, is a powerful predictor of how long s/he will live. While situations like the poisoning of the water in Flint, Michigan have gotten some attention, they are generally treated as the exception rather than a reflection of real environmental hazards that exist in the west. Moreover we wonder why more endemic issues of neighbourhood environmental contamination that shorten human lives are not a priority for local action or that it is not linked to disproportionate production of greenhouse gases that cause climate change/warming/chaos. 相似文献
138.
Alexandre Caseiro Heidi Bauer Christoph Schmidl Casimiro A. Pio Hans Puxbaum 《Atmospheric environment (Oxford, England : 1994)》2009,43(13):2186-2195
Anhydrosugars (levoglucosan, mannosan and galactosan) were investigated during one year in three Austrian regions at three types of sites (city-heavy traffic-impacted, city-residential and background) in order to assess the magnitude of the contribution of wood smoke to the particulate matter load and its organic fraction. The annually averaged concentrations of levoglucosan ranged from 0.12 to 0.48 μg m?3. The levoglucosan concentration exhibited a strong annual cycle with higher concentrations in the cold season. The minor anhydrosugars had a similar annual trend, but their concentrations were lower by a factor of about 5 and about 25 in the cold season for mannosan and galactosan, respectively. Levoglucosan concentrations were higher at the inner-urban as compared to rural sites. The contribution of wood smoke to organic carbon and PM10 levels was calculated using a constant ratio of levoglucosan and OC, respectively PM10 as derived for fire wood typical for Alpine European regions [Schmidl, C., Marr, I.L., Caseiro, A.e, Kotianová, P., Berner, A., Bauer, H., Kasper-Giebl, A., Puxbaum, H., 2008a. Chemical characterisation of fine particle emissions from wood stove combustion of common woods growing in mid-European Alpine regions. Atmospheric Environment 42, 126–141]. The estimated contribution of wood smoke-OC to the OC of PM10 ranged from one third to more than half in the cold season with higher contributions up to 70% in winter (December, January and February) in the smaller cities and the rural background. This indicates, that wood smoke is the predominant source of organic material at rural and small urban sites in central Europe. Consistently, wood smoke was an important contributor to PM10 during the cold season, with contributions of around 10% in the Vienna larger region and around 20% at rural sites in the densely forested regions of Salzburg and Styria during the winter months. In those regions residential sites exhibited highest relative wood smoke contents in PM10 during autumn (September till November), indicating the use of wood stoves for auxiliary heating in the transition of warm to cold season. Using the relationships between the different anhydrosugars the combustion of softwood was found to be dominant for the wood smoke occurrence in ambient air at the investigated sites. Potassium, a commonly used tracer for biomass burning, correlated well to levoglucosan, with a mass ratio of around 0.80 in the cold season. 相似文献
139.
Sachin D. Ghude R.J. Van der A S. Fadnavis 《Environmental pollution (Barking, Essex : 1987)》2009,157(6):1873-1878
We assessed satellite derived tropospheric NO2 distribution on a global scale and identified the major NO2 hotspot regions. Combined GOME and SCIAMACHY measurements for the period 1996-2006 have been used to compute the trends over these regions. Our analysis shows that tropospheric NO2 column amounts have increased over the newly and rapidly developing regions like China (11 ± 2.6%/year), south Asia (1.76 ± 1.1%/year), Middle East (2.3 ± 1%/year) and South Africa (2.4 ± 2.2%/year). Tropospheric NO2 column amounts show some decrease over the eastern US (−2 ± 1.5%/year) and Europe (0.9 ± 2.1%/year). We found that although tropospheric NO2 column amounts decreased over the major developed regions in the past decade, the present tropospheric NO2 column amounts over these regions are still significantly higher than those observed over newly and rapidly developing regions (except China). Tropospheric NO2 column amounts show some decrease over South America and Central Africa, which are major biomass burning regions in the Southern Hemisphere. 相似文献
140.
An indispensable asset at risk: merits and needs of chemicals-related environmental sciences 总被引:1,自引:1,他引:0