全文获取类型
收费全文 | 2637篇 |
免费 | 30篇 |
国内免费 | 18篇 |
专业分类
安全科学 | 68篇 |
废物处理 | 82篇 |
环保管理 | 427篇 |
综合类 | 567篇 |
基础理论 | 575篇 |
环境理论 | 4篇 |
污染及防治 | 661篇 |
评价与监测 | 181篇 |
社会与环境 | 108篇 |
灾害及防治 | 12篇 |
出版年
2023年 | 19篇 |
2022年 | 23篇 |
2021年 | 30篇 |
2020年 | 31篇 |
2019年 | 27篇 |
2018年 | 55篇 |
2017年 | 56篇 |
2016年 | 58篇 |
2015年 | 59篇 |
2014年 | 70篇 |
2013年 | 195篇 |
2012年 | 95篇 |
2011年 | 139篇 |
2010年 | 100篇 |
2009年 | 114篇 |
2008年 | 127篇 |
2007年 | 147篇 |
2006年 | 101篇 |
2005年 | 93篇 |
2004年 | 106篇 |
2003年 | 84篇 |
2002年 | 99篇 |
2001年 | 44篇 |
2000年 | 38篇 |
1999年 | 36篇 |
1998年 | 27篇 |
1997年 | 33篇 |
1996年 | 33篇 |
1995年 | 35篇 |
1994年 | 50篇 |
1993年 | 20篇 |
1992年 | 21篇 |
1991年 | 22篇 |
1990年 | 20篇 |
1989年 | 15篇 |
1988年 | 23篇 |
1987年 | 16篇 |
1986年 | 20篇 |
1984年 | 13篇 |
1983年 | 16篇 |
1982年 | 17篇 |
1981年 | 17篇 |
1980年 | 16篇 |
1979年 | 17篇 |
1978年 | 14篇 |
1977年 | 12篇 |
1960年 | 11篇 |
1959年 | 12篇 |
1956年 | 12篇 |
1954年 | 17篇 |
排序方式: 共有2685条查询结果,搜索用时 15 毫秒
981.
Monitoring of the microbial community composition in saline aquifers during CO2 storage by fluorescence in situ hybridisation 总被引:1,自引:0,他引:1
Daria Morozova Maren Wandrey Mashal Alawi Martin Zimmer Andrea Vieth Michael Zettlitzer Hilke Würdemann the COSINK Group 《International Journal of Greenhouse Gas Control》2010,4(6):981-989
This study reveals the first analyses of the composition and activity of the microbial community of a saline CO2 storage aquifer. Microbial monitoring during CO2 injection has been reported. By using fluorescence in situ hybridisation (FISH), we have shown that the microbial community was strongly influenced by the CO2 injection. Before CO2 arrival, up to 6 × 106 cells ml−1 were detected by DAPI staining at a depth of 647 m below the surface. The microbial community was dominated by the domain Bacteria that represented approximately 60% to 90% of the total cell number, with Proteobacteria and Firmicutes as the most abundant phyla comprising up to 47% and 45% of the entire population, respectively. Both the total cell counts as well as the counts of the specific physiological groups revealed quantitative and qualitative changes after CO2 arrival. Our study revealed temporal outcompetition of sulphate-reducing bacteria by methanogenic archaea. In addition, an enhanced activity of the microbial population after five months CO2 storage indicated that the bacterial community was able to adapt to the extreme conditions of the deep biosphere and to the extreme changes of these atypical conditions. 相似文献
982.
Patrick J. Dugan Chris Barlow Angelo A. Agostinho Eric Baran Glenn F. Cada Daqing Chen Ian G. Cowx John W. Ferguson Tuantong Jutagate Martin Mallen-Cooper Gerd Marmulla John Nestler Miguel Petrere Robin L. Welcomme Kirk O. Winemiller 《Ambio》2010,39(4):344-348
The past decade has seen increased international recognition of the importance of the services provided by natural ecosystems. It is unclear however whether such international awareness will lead to improved environmental management in many regions. We explore this issue by examining the specific case of fish migration and dams on the Mekong river. We determine that dams on the Mekong mainstem and major tributaries will have a major impact on the basin’s fisheries and the people who depend upon them for food and income. We find no evidence that current moves towards dam construction will stop, and consider two scenarios for the future of the fisheries and other ecosystems of the basin. We conclude that major investment is required in innovative technology to reduce the loss of ecosystem services, and alternative livelihood strategies to cope with the losses that do occur. 相似文献
983.
Martin Forsius Maximilian Posch Julian Aherne Gert Jan Reinds Jesper Christensen Lars Hole 《Ambio》2010,39(2):136-147
For more than a decade, anthropogenic sulfur (S) and nitrogen (N) deposition has been identified as a key pollutant in the
Arctic. In this study new critical loads of acidity (S and N) were estimated for terrestrial ecosystems north of 60° latitude
by applying the Simple Mass Balance (SMB) model using two critical chemical criteria (Al/Bc = 1 and ANCle = 0). Critical loads were exceeded in large areas of northern Europe and the Norilsk region in western Siberia during the
1990s, with the more stringent criterion (ANCle = 0) showing the larger area of exceedance. However, modeled deposition estimates indicate that mean concentrations of sulfur
oxides and total S deposition within the Arctic almost halved between 1990 and 2000. The modeled exceeded area is much reduced
when currently agreed emission reductions are applied, and almost disappears under the implementation of maximum technically
feasible reductions by 2020. In northern North America there was no exceedance under any of the deposition scenarios applied.
Modeled N deposition was less than 5 kg ha−1 y−1 almost across the entire study area for all scenarios; and therefore empirical critical loads for the eutrophying impact
of nitrogen are unlikely to be exceeded. The reduction in critical load exceedances is supported by observed improvements
in surface water quality, whereas the observed extensive damage of terrestrial vegetation around the mining and smelter complexes
in the area is mainly caused by direct impacts of air pollution and metals. 相似文献
984.
Martin D. King Adrian R. Rennie Christian Pfrang Arwel V. Hughes Katherine C. Thompson 《Atmospheric environment (Oxford, England : 1994)》2010,44(14):1822-1825
The reactions between atmospheric oxidants and organic amphiphiles at the air–water interface of an aerosol droplet may affect the size and critical supersaturation required for cloud droplet formation. We demonstrate that no reaction occurs between gaseous nitrogen dioxide (1000 ppm in air) and a monolayer of an insoluble amphiphile, oleic acid (cis-9-octadecenoic acid), at the air–water interface which removes material from the air–water interface. We present evidence that the NO2 isomerises the cis-9-octadecenoic (oleic) acid to trans-9-octadecenoic (elaidic) acid. The study presented here is important for future and previous studies of (1) the reaction between the nitrate radical, NO3, and thin organic films as NO2 is usually present in high concentrations in these experimental systems and (2) the effect of NO2 air pollution on the unsaturated fatty acids and lipids found at the air–liquid surface of human lung lining fluid. 相似文献
985.
James F. Fox Charles M. Davis Darren K. Martin 《Journal of the American Water Resources Association》2010,46(6):1192-1204
Fox, James F., Charles M. Davis, and Darren K. Martin, 2010. Sediment Source Assessment in a Lowland Watershed Using Nitrogen Stable Isotopes. Journal of the American Water Resources Association (JAWRA) 46(6):1192–1204. DOI: 10.1111/j.1752-1688.2010.00485.x Abstract: Sediment sources and transported sediments were sampled in a lowland watershed with pronounced fine sediment storage in the streambed. Sediments were analyzed for carbon and nitrogen content and stable nitrogen isotopic composition. Analysis of the data shows that temporarily stored streambed sediments dominate the sediment load during moderate- and low-flow hydrologic events. Modeling of sediment transport and nitrogen elemental and isotopic mass balance was performed for the watershed for a 12-month time period using a continuous, conceptual-based model. The model results show that during moderate- and low-flow hydrologic events, the streambed is slowly downcutting. During very high-flow hydrologic events, deposition is pronounced in the streambed and sediment is replenished to the bed. Nitrogen model results show that elemental and isotopic nitrogen of streambed sediments vary substantially over the simulation period. In this manner, the streambed in a lowland watershed functions as a temporary storage zone that, in turn, can impact the nitrogen elemental and isotopic signature of sediments. The variation could significantly impact estimates of sediment provenance using nitrogen tracer-based methods. Future work should consider both hydrologic and biogeochemical control on the nitrogen isotopic signature of sediments in small lowland watersheds and streams where a significant portion of deposited fines are temporarily stored. 相似文献
986.
Occurrence and sources of selected phenolic endocrine disruptors in Ria de Aveiro,Portugal 总被引:2,自引:0,他引:2
Niels Jonkers Ana Sousa Susana Galante-Oliveira Carlos M. Barroso Hans-Peter E. Kohler Walter Giger 《Environmental science and pollution research international》2010,17(4):834-843
Background, aim and scope
Ria de Aveiro (Portugal) is a shallow coastal lagoon of high economic and ecological importance. Hardly any data on its chemical pollution by polar organic pollutants are available in literature. This study focused on the presence and sources of a series of phenolic endocrine-disrupting compounds (EDCs) in this area, including parabens, alkylphenolic compounds and bisphenol-A (BPA). A number of possible sources of pollution are present in the area, including the large harbours present in the lagoon, the city of Aveiro and the rivers discharging into the area. A recently constructed submarine wastewater outfall, located a few kilometres from the lagoon inlet has also been suggested as a possible source of pollution to Ria de Aveiro in several publications. The aim of the current field study was to investigate the occurrence and main sources of phenolic endocrine disruptors in Ria de Aveiro. 相似文献987.
Pimp Your Landscape: A Tool for Qualitative Evaluation of the Effects of Regional Planning Measures on Ecosystem Services 总被引:1,自引:0,他引:1
The article presents the platform “Pimp your landscape” (PYL), which aims firstly at the support of planners by simulating
alternative land-use scenarios and by an evaluation of benefits or risks for regionally important ecosystem services. Second,
PYL supports an integration of information on environmental and landscape conditions into impact assessment. Third, PYL supports
the integration of impacts of planning measures on ecosystem services. PYL is a modified 2-D cellular automaton with GIS features.
The cells have the major attribute “land-use type” and can be supplemented with additional information, such as specifics
regarding geology, topography and climate. The GIS features support the delineation of non-cellular infrastructural elements,
such as roads or water bodies. An evaluation matrix represents the core element of the system. In this matrix, values in a
relative scale from 0 (lowest value) to 100 (highest value) are assigned to the land-use types and infrastructural elements
depending on their effect on ecosystem services. The option to configure rules for describing the impact of environmental
attributes and proximity effects on cell values and land-use transition probabilities is of particular importance. User interface
and usage of the platform are demonstrated by an application case. Constraints and limits of the recent version are discussed,
including the need to consider in the evaluation, landscape-structure aspects such as patch size, fragmentation and spatial
connectivity. Regarding the further development, it is planned to include the impact of land management practices to support
climate change adaptation and mitigation strategies in regional planning. 相似文献
988.
Tung V. Nguyen Martin Reinhard Huiting Chen Karina Y.-H. Gin 《Environmental science and pollution research international》2016,23(11):10382-10392
Transport and fate of perfluoro- and polyfluoroalkyl substances (PFASs) in an urban water body that receives mainly urban runoff was investigated. Water, suspended solids, and sediment samples were collected during the monsoon (wet) and inter-monsoon (dry) season at different sites and depths. Samples were analyzed for C7 to C12 perfluoroalkyl carboxylate homologues (PFCAs) (PFHpA, PFOA, PFNA, PFDA, PFUnA, PFDoA), perfluorohexane, perfluorooctane, and 6:2-fluorotelomer sulfonate (PFHxS, PFOS, and 6:2FtS, respectively), perfluorooctane sulfonamide (FOSA), N-ethyl FOSA (sulfluramid), N-ethyl sulfonamidoethanol (N-EtFOSE), and N-methyl and N-ethyl sulfonamidoacetic acid (N-EtFOSAA and N-MeFOSAA, respectively). Concentrations in wet samples were only slightly higher. The sum total PFAS (ΣPFAS) concentrations dissolved in the aqueous phase and sorbed to suspended solids (SS) ranged from 107 to 253 ng/L and 11 to 158 ng/L, respectively. PFOA, PFOS, PFNA, PFHxS, and PFDA contributed most (approximately 90 %) to the dissolved ΣPFASs. N-EtFOSA dominated the particulate PFAS burden in wet samples. K D values of PFOA and PFOS calculated from paired SS and water concentrations varied widely (1.4 to 13.7 and 1.9 to 98.9 for PFOA and PFOS, respectively). Field derived K D was significantly higher than laboratory K D suggesting hydrophobic PFASs sorbed to SS resist desorption. The ΣPFAS concentrations in the top sedimentary layer ranged from 8 to 42 μg/kg and indicated preferential accumulation of the strongly sorbing long-chain PFASs. The occurrence of the metabolites N-MeFOSAA, N-EtFOSAA and FOSA in the water column and sediments may have resulted from biological or photochemical transformations of perfluorooctane sulfonamide precursors while the absence of FOSA, N-EtFOSA and 6:2FtS in sediments was consistent with biotransformation. 相似文献
989.
Blood mercury levels among fish consumers residing in areas with high environmental burden 总被引:1,自引:0,他引:1
Mercury is a ubiquitous, persistent toxicant found in the environment. In water, mercury bioaccumulates up the food chain and leads to high concentrations in fish. Consumption of contaminated fish is the major source of exposure to mercury in the US. The objective of this study was to enroll persons living in areas selected by the Environmental Protection Agency (EPA) to have high mercury concentrations and who consume at least 6 oz of locally caught fish per week to determine the feasibility of monitoring future trends among a population identified as highly exposed. Blood samples were collected at time of interview and analyzed for mercury. Participants (n = 287) were enrolled from North Carolina, Maryland, and South Dakota. Participants reported eating an average of five servings of fish per week. The overall geometric mean for total mercury was 0.75 μg L−1, with North Carolina having the highest mean level (2.02 μg L−1). Overall, 42% of the study population had levels greater than the US geometric mean 0.83 μg L−1. The number of servings of fish consumed was not found to be associated with blood mercury levels. We were able to identify some persons with elevated mercury concentrations living in areas identified by EPA; however, identifying and monitoring a highly exposed population over time would be challenging. 相似文献
990.
Controls on coarse wood decay in temperate tree species: birth of the LOGLIFE experiment 总被引:1,自引:0,他引:1
Cornelissen JH Sass-Klaassen U Poorter L van Geffen K van Logtestijn RS van Hal J Goudzwaard L Sterck FJ Klaassen RK Freschet GT van der Wal A Eshuis H Zuo J de Boer W Lamers T Weemstra M Cretin V Martin R Ouden Jd Berg MP Aerts R Mohren GM Hefting MM 《Ambio》2012,41(Z3):231-245
Dead wood provides a huge terrestrial carbon stock and a habitat to wide-ranging organisms during its decay. Our brief review highlights that, in order to understand environmental change impacts on these functions, we need to quantify the contributions of different interacting biotic and abiotic drivers to wood decomposition. LOGLIFE is a new long-term 'common-garden' experiment to disentangle the effects of species' wood traits and site-related environmental drivers on wood decomposition dynamics and its associated diversity of microbial and invertebrate communities. This experiment is firmly rooted in pioneering experiments under the directorship of Terry Callaghan at Abisko Research Station, Sweden. LOGLIFE features two contrasting forest sites in the Netherlands, each hosting a similar set of coarse logs and branches of 10 tree species. LOGLIFE welcomes other researchers to test further questions concerning coarse wood decay that will also help to optimise forest management in view of carbon sequestration and biodiversity conservation. 相似文献