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661.
S. Hellsten U. Dragosits C. J. Place T. H. Misselbrook Y. S. Tang M. A. Sutton 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):3-13
Most ammonia (NH3) emission inventories have been calculated on an annual basis and do not take into account the seasonal variability of emissions
that occur as a consequence of climate and agricultural practices that change throughout the year. When used as input to atmospheric
transport models to simulate concentration fields, these models therefore fail to capture seasonal variations in ammonia concentration
and dry and wet deposition. In this study, seasonal NH3 emissions from agriculture were modelled on a monthly basis for the year 2000, by incorporating temporal aspects of farming
practice. These monthly emissions were then spatially distributed using the AENEID model (Atmospheric Emissions for National
Environmental Impacts Determination). The monthly model took the temporal variation in the magnitude of the ammonia emissions,
as well as the fine scale (1-km) spatial variation of those temporal changes into account to provide improved outputs at 5-km
resolution. The resulting NH3 emission maps showed a strong seasonal emission pattern, with the highest emissions during springtime (March and April) and
the lowest emissions during summer (May to July). This emission pattern was mainly influenced by whether cattle were outside
grazing or housed and by the application of manures and fertilizers to the land. When the modelled emissions were compared
with measured NH3 concentrations, the comparison suggested that the modelled emission trend corresponds fairly well with the seasonal trend
in the measurements. The remaining discrepancies point to the need to develop functional parametrisations of the interactions
with climatic seasonal variation. 相似文献
662.
663.
Ian D. Leith Lucy J. Sheppard David Fowler J. Neil Cape Matt Jones Alan Crossley Ken J. Hargreaves Y. Sim Tang Mark Theobald Mark R. Sutton 《Water, Air, & Soil Pollution: Focus》2004,4(6):207-218
Providing an accurate estimate of the dry component of N deposition to low N background, semi-natural habitats, such as bogs and upland moors dominated by Calluna vulgaris is difficult, but essential to relate nitrogen deposition to effects in these communities. To quantify the effects of NH3 inputs to moorland vegetation growing on a bog at a field scale, a field release NH3 fumigation system was established at Whim Moss (Scottish Borders) in 2002. Gaseous NH3 from a line source was released along of a 60 m transect, when meteorological conditions (wind speed >2.5 m s–1 and wind direction in the sector 180–215°) were met, thereby providing a profile of decreasing NH3 concentration with distance from the source. In a complementary study, using a NH3 flux chamber system, the relationships between NH3 concentrations and cuticular resistances were quantified for a range of NH3 concentrations and micrometeorological conditions for moorland vegetation. Cuticular resistances increased with NH3 concentration from 11 s m–1 at 3.0 g m–3 to 30 s m–1 at 30 g m–3. The NH3 concentration data and the concentration-dependent canopy resistance are used to calculate NH3 deposition taking into account leaf surface wetness. The implications of using an NH3 concentration-dependent cuticular resistance and the importance for refining critical loads are discussed. 相似文献
664.
665.
666.
土体的导热系数是能源岩土工程设计与研究中重要的热物理参数。工程中土体常处于非饱和状态。非饱和土体的导热系数会影响地下结构物的力学性能、热交换效率以及整个热工结构的工作效率。为给能源岩土工程设计与研究提供可靠的热物理参数,通过室内单元试验测量了不同含水率和温度下砾砂、粉土和黏土的导热系数,研究这三种非饱和土体的导热系数与含水率、基质吸力和温度的关系。研究结果表明,三种非饱和土体的导热系数都随含水率的增加而增加,最后趋于稳定。砾砂导热系数增加的速率最快,粉土次之,黏土最小。相同含水率下,砾砂导热系数最大,粉土次之,黏土最小。粉土的导热系数与基质吸力密切相关,其关系曲线趋势近似土 水特征曲线。三种土体的导热系数均随温度的增加近似线性增加,但增加幅度仅为10-3级别,可忽略其影响。 相似文献
667.
利用TaPL3(Version3.00)模型计算了天津地区p,p'-DDT通过大气和水体的长距离传输潜力(LRTP).通过灵敏度分析,确定了模型的关键参数.利用蒙特卡罗方法对模型结果进行了不确定性分析.结果表明,天津地区p,p'-DDT通过大气的LRTP为473~762km,均值为579km;通过水体的LRTP为940~10958km,均值为2254km.通过大气的LRTP的结果分布比通过水体的LRTP更集中.与国外同类结果比较,通过大气的LRTP略低,而通过水体的LRTP则明显偏低. 相似文献
668.
2010年本实验室开始生物质对柴油的吸附实验,和前人的结论一致,生物质热改性后其吸油和漂浮性能提高,但成本增加很多。受到前人复合吸油材料的启发,2012年开展了蒲绒-芦苇机械混合复合材料吸油和漂浮性能的研究,并采用正交实验对影响除油效果的因素进行优化。结果表明,蒲绒-芦苇复合材料较之芦苇吸油性能提高,且比各组分的叠加饱和吸油量还高。震荡使芦苇的漂浮率明显降低,但对蒲绒及复合材料的影响较小。正交实验结果显示,投加量0.7g,油膜厚度0.55 mm,不震荡时,蒲绒除油最佳;在相同条件下,粒径为380~500μm的芦苇除油最佳,蒲绒和该粒径的芦苇按质量比为1∶4混合成的复合材料的除油效果最佳。 相似文献
669.
Zhuo Guan Xiang-Yu Tang Jae E. Yang Yong Sik Ok Zhihong Xu Taku Nishimura Brian J. Reid 《Environmental geochemistry and health》2017,39(6):1221-1243
Excessive transport of fine sediment, and its associated pollutants, can cause detrimental impacts in aquatic environments. It is therefore important to perform accurate sediment source apportionment to identify hot spots of soil erosion. Various tracers have been adopted, often in combination, to identify sediment source type and its spatial origin; these include fallout radionuclides, geochemical tracers, mineral magnetic properties and bulk and compound-specific stable isotopes. In this review, the applicability of these techniques to particular settings and their advantages and limitations are reviewed. By synthesizing existing approaches, that make use of multiple tracers in combination with measured changes of channel geomorphological attributes, an integrated analysis of tracer profiles in deposited sediments in lakes and reservoirs can be made. Through a multi-scale approach for fine sediment tracking, temporal changes in soil erosion and sediment load can be reconstructed and the consequences of changing catchment practices evaluated. We recommend that long-term, as well as short-term, monitoring of riverine fine sediment and corresponding surface and subsurface sources at nested sites within a catchment are essential. Such monitoring will inform the development and validation of models for predicting dynamics of fine sediment transport as a function of hydro-climatic and geomorphological controls. We highlight that the need for monitoring is particularly important for hilly catchments with complex and changing land use. We recommend that research should be prioritized for sloping farmland-dominated catchments. 相似文献
670.
Xianqiang Tang Min Wu Rui Li Zhenhua Wang 《Environmental science and pollution research international》2017,24(29):22808-22815
Phosphorus recovery from wastewater not only reduces the unbearable impacts of excessive nutrient discharge on environmental systems but also favor the reuse of phosphorus resource. Based on the mechanism as well as technical analysis for major phosphorus recovery techniques including struvite precipitation and wetland substrate adsorption, a novel magnesium slag-packed wetland filter and corresponding operational procedures are proposed, which aim to reduce the dependence of using magnesium-containing chemical reagent as magnesium sources for struvite precipitation, and improve the accumulation and recovery performance for struvite precipitation within porous wetland substrate. Results from preliminary experiments indicated that magnesium slag particles with approximately 2 mm in diameter can recover 43.20–72.39% phosphorus from 1–25 mol/L PO4 3? solution, and the presence of 5–50 mol/L NH4 + contributed to 11.71–29.11% enhancement of phosphorus recovery mainly due to struvite precipitation. The detected generation of struvite via XRD spectrum analysis partly demonstrated the potential of phosphorus recovery in magnesium slag-packed wetland filter. The proposed phosphorus recovery technology is free of secondary pollution and solid waste generation; phosphorus-saturated (mainly due to struvite precipitation and adsorption) magnesium slag particles can be potentially used as phosphorus fertilizer and thus partly solved the traditional shortages of disposing phosphorus-saturated substrate due to low phosphorus contents. 相似文献