全文获取类型
收费全文 | 634篇 |
免费 | 4篇 |
国内免费 | 5篇 |
专业分类
安全科学 | 8篇 |
废物处理 | 13篇 |
环保管理 | 47篇 |
综合类 | 324篇 |
基础理论 | 102篇 |
污染及防治 | 113篇 |
评价与监测 | 21篇 |
社会与环境 | 13篇 |
灾害及防治 | 2篇 |
出版年
2018年 | 6篇 |
2017年 | 9篇 |
2016年 | 13篇 |
2015年 | 9篇 |
2013年 | 23篇 |
2012年 | 12篇 |
2011年 | 22篇 |
2010年 | 16篇 |
2009年 | 16篇 |
2008年 | 25篇 |
2007年 | 21篇 |
2006年 | 9篇 |
2005年 | 17篇 |
2004年 | 15篇 |
2003年 | 16篇 |
2002年 | 21篇 |
2001年 | 8篇 |
2000年 | 8篇 |
1999年 | 14篇 |
1998年 | 15篇 |
1997年 | 7篇 |
1996年 | 6篇 |
1995年 | 9篇 |
1994年 | 7篇 |
1993年 | 6篇 |
1985年 | 5篇 |
1977年 | 5篇 |
1975年 | 6篇 |
1973年 | 7篇 |
1972年 | 5篇 |
1970年 | 8篇 |
1969年 | 6篇 |
1967年 | 8篇 |
1965年 | 11篇 |
1963年 | 13篇 |
1962年 | 10篇 |
1961年 | 9篇 |
1960年 | 12篇 |
1959年 | 17篇 |
1958年 | 11篇 |
1957年 | 8篇 |
1956年 | 9篇 |
1955年 | 8篇 |
1954年 | 8篇 |
1953年 | 6篇 |
1952年 | 6篇 |
1930年 | 4篇 |
1926年 | 6篇 |
1914年 | 6篇 |
1913年 | 10篇 |
排序方式: 共有643条查询结果,搜索用时 46 毫秒
31.
32.
Evacuation mapping: the utility of guidelines 总被引:2,自引:0,他引:2
33.
Werner E. G. Müller 《Die Naturwissenschaften》1998,85(1):11-25
Geodia cydonium , which code for proteins. The analyses of their deduced amino acid sequences allowed a molecular biological approach to solve
the problem of monophyly of Metazoa. Molecules of the extracellular matrix/basal lamina, with the integrin receptor, fibronectin,
and galectin as prominent examples, cell-surface receptors (tyrosine kinase receptor), elements of sensory systems (crystallin,
metabotropic glutamate receptor), and homologs/modules of an immune system (immunoglobulin like molecules, scavenger receptor
cysteine-rich, and short consensus repeats, rhesus system) classify the Porifera as true Metazoa. As living fossils, provided
with simple, primordial molecules allowing cell-cell and cell-matrix adhesion as well as processes of signal transduction
as known in a more complex manner from higher Metazoa, they also show peculiarities not known in other metazoan phyla. Tissues
of sponges are rich in telomerase activity, suggesting a high plasticity in the determination of cell lineages. It is concluded
that molecular biological studies with sponges as model will not only help to understand the evolution of Protoctista to Metazoa
but also the complex, hierarchial regulatory network of cells in higher Metazoa. 相似文献
34.
Sperm competition is thought to be an important selective pressure shaping sperm form and function. However, few studies have
moved beyond gross examinations of sperm morphology. Sperm length is subject to sexual selection via sperm competition in
the scarab beetle Onthophagus taurus. Here, the structure and ultrastructure of spermatozoa in this species were investigated using light and electron microscopy.
Spermatozoa were found to be filiform, measuring about 1,200 mm in length. The sperm head consists of a three-layered acrosome
and a nuclear region bearing the anterior extension of the centriole adjunct. Acrosome and nuclear regions are bilaterally
symmetric, with their axes of symmetry being orthogonal to each other. Head and flagellar structures are connected by a well-developed
centriole adjunct. The sperm heads are asymmetrically surrounded by accessory material and embedded into the cytoplasm of
the spermatocyst cell. The accessory material is produced inside the spermatids and then transferred to the outside due to
a new membrane formed around the sperm’s organelles. The old spermatid membrane separates the accessory material from the
cyst cell. The flagellum contains a 9+9+2 axoneme, two accessory bodies, and two mitochondrial derivatives of unequal size.
The major mitochondrial derivative is significantly larger than the minor one. The axoneme is arranged in a sinusoidal manner
parallel along the major mitochondrial derivative. The spermatozoa show no progressive motility when released in buffer solution
which is likely to be the result of the flagellar arrangement and the structure of the major mitochondrial derivative. The
cross-sectional area of the minor and the major mitochondrial derivatives show different patterns of genetic variation. The
data provide the first estimates of genetic variation in sperm ultrastructure for any species, and give evidence for the persistence
of genetic variation in ultrastructure required for the rapid and divergent evolution that characterizes spermatozoa generally. 相似文献
35.
de Souza Pereira M Heitmann D Reifenhäuser W Meire RO Santos LS Torres JP Malm O Körner W 《Chemosphere》2007,67(9):1736-1745
Monitoring of immission of persistent organic pollutants in the industrialized area of Volta Redonda (V.R.) and in the National Park of Itatiaia (PNI) in southeast Brazil was performed using an endemic bromeliad species as biomonitor and measuring bulk deposition rates of polychlorinated biphenyls (PCB) and polycyclic aromatic hydrocarbons (PAH). For the sum of PCB, overall deposition rates were between 17 and 314 ng/(m2 day) in winter and between 43 and 81 ng/(m2 day) in summer, respectively. Deposition rates of dioxin-like PCBs ranged from 0.14 to 2.8 pg WHO-TEQ/(m2 day) in winter and from 0.90 to 4.3 pg WHO-TEQ/(m2 day) in summer. PCB deposition rates (total PCB and WHO-TEQ) were in the same range in winter in V.R. and PNI. In summer, contamination levels in V.R. were 6-10-folds higher than in PNI. PCB concentrations in biomonitor samples from V.R. and PNI were in the same range in summer and in winter. Concentrations of total PCB ranged from 14 to 95 microg/kg dry matter (d.m.) in winter and from 18 to 27 microg/kg d.m. in summer, respectively. The TEQ values were between 1.7 and 4.1 ng WHO-TEQ/kg d.m. in winter and between 1.9 and 2.9 ng WHO-TEQ/kg d.m. in summer. PCB concentrations of di-ortho PCB but not of non-ortho PCB were a factor of 2-4 lower in summer in both areas. PCB congener profiles resembled those from technical formulations. The profiles shifted to the higher chlorinated congeners in summer, probable due to revolatilisation of the lighter components at higher temperatures. PCB profiles in biomonitor resembled those from deposition samples and the shift to the heavier congeners in summer was even more pronounced. PAH deposition rates were in a similar range in both areas (131-2415 ng/(m2 day)). PAH levels in biomonitor samples from V.R. were about one order of magnitude higher than in samples from PNI indicating the impact of local sources. PAH profiles revealed stationary thermal processes as main source of contamination in V.R. whereas in PNI, biomass burning seems to be the main contamination source. 相似文献
36.
Urbatzka R van Cauwenberge A Maggioni S Viganò L Mandich A Benfenati E Lutz I Kloas W 《Chemosphere》2007,67(6):1080-1087
The river Lambro is the most polluted tributary of the river Po in North Italy and was chosen as a representative water course discharging industrialized areas. Water and sediment samples of the river Lambro were investigated regarding the presence of endocrine disrupting compounds. A combined procedure was used consisting of solid-phase extraction and HPLC based fractionation of samples, of screening for (anti)androgenic activity using the yeast androgen screen (YAS) and of chemical analysis using HPLC-MS/MS and GC-MS. Androgenic and antiandrogenic activities were found in specific fractions of the water and sediment while the total extracts showed antiandrogenic activity only. The chemical analysis of the fractions and total extracts with antiandrogenic activities revealed the presence of compounds with suspected antiandrogenic potency such as bisphenol A, iprodione, nonylphenol, p,p'-DDE and tert-octylphenol but other unknown compounds contributed mainly to the observed antiandrogenic activities. The antiandrogenic load of the river Lambro ranged between 1.34 and 17.1 microM flutamide-equivalents and may pose a risk to aquatic environments. Future screenings for EDC in the environment that have the potential to interfere with reproduction of aquatic organisms should be extended to different modes of actions including (anti)androgenic ones. 相似文献
37.
Organic pollutants in compost and digestate. Part 1. Polychlorinated biphenyls, polycyclic aromatic hydrocarbons and molecular markers 总被引:1,自引:0,他引:1
Brändli RC Bucheli TD Kupper T Furrer R Stahel WA Stadelmann FX Tarradellas J 《Journal of environmental monitoring : JEM》2007,9(5):456-464
In Europe, 9.3 x 10(6) t(dry weight (dw)) of compost and digestate are produced per year. Most of this is applied to agricultural land, which can lead to considerable inputs of organic pollutants, such as polychlorinated biphenyls (PCB) and polycyclic aromatic hydrocarbons (PAH) to soil. This paper presents an inventory of the pollutant situation in source-separated composts, digestates and presswater in Switzerland by a detailed analysis of over 70 samples. PCB concentrations ( summation PCB 28, 52, 101, 118, 138, 153, 180) were significantly higher in urban (median: 30 microg kg(-1)dw, n = 52) than in rural samples (median: 14 microg kg(-1)dw, n = 16). Together with low concentrations in general, this points to aerial deposition on compost input material as the major contamination pathway. Enantiomeric fractions of atropisometric PCB were close to racemic. Median PAH concentration was 3010 microg kg(-1)dw( summation 15PAH, n = 69), and one quarter of the samples exhibited concentrations above the relevant Swiss guide value for compost (4000 microg kg(-1)dw). The levels were influenced by the treatment process (digestate > compost), the season of input material collection (spring-summer > winter > autumn), the particle size (coarse-grained > fine-grained), and maturity (mature > less mature). The main source of PAH in compost was pyrogenic, probably influenced mainly by liquid fossil fuel combustion and some asphalt abrasion, as suggested by multiple linear regression. This study, together with a companion paper reporting on other organic contaminates including emerging compound classes, provides a starting point for a better risk-benefit estimation of the application of compost and digestate to agricultural soil in Switzerland. 相似文献
38.
Investigations of the dandelion, Taraxacum officinale Web. in Poland, Romania and Germany showed that the species concentrates various elements dependent on the intensity of the pollutants. In this study, we followed up the question of whether T. officinale enriches pollutants by the atmospheric deposition on the leaves or via the soil. Therefore, samples from at least 10 plants and a soil sample at 57 sample sites were collected from a grid of 500 m × 500 m. In addition to the analysis of the total soil sample, the (mobile) ion pool of the soil (DIN V 19739) was analysed. The elements Al, As, Ba, Ca, Cd, Ce, Co, Cr, Cu, Fe, Ga, K, Mg, Mn, Mo, Na, Ni, Rb, Sr, Ti, Tl, V, and Zn were determined through the use of spectrometry with inductive coupled plasma (ICP-MS and ICP-OES). The results are compared with the element concentrations of washed and unwashed leaf samples in T. officinale. We could only find two direct correlations (Ti and Zn) between the element content, of the entire soil samples, but 14 correlations (As, Ba, Cd, Cu, Ga, K, Mn, Mo, Na, Ni, Rb, Ti, Tl und Zn) between the ion pool of the soil and the washed samples. The grid point data interpolation by ArcInfo showed a similar distribution pattern for the unwashed leaf elements Al, Ce, Fe, Ti and V (r≥0.75). The elements Al, Ce, Fe, Ti, and V are washed out at the same ratio. Thus, although the concentration of these elements were significantly reduced by the washing procedure, the correlations were not influenced. The admissibility of the grid point data interpolation for a distribution map of the town area was investigated, as well. It is shown that the element content varies with the land use (meadow, field, rural areas), the sampling point and the local pollutants. However, none of the discussed elements, Al, Ce, Fe, Ti, and V, is significantly influenced by the land use. The data allows one to make the conclusion that the elements of Al, Ce, Fe, Ti and V are dependent on the dry and wet deposition on the leaves of T. officinale. These elements are taken up not only by the roots, but also by the surface of the leaves. This is evident because there is no correlation between one of these elements in the leaves and the ion pool of the soil. 相似文献
39.
Daniel P. Connell Jeffrey A. Withum Stephen E. Winter Robert M. Statnick Richard A. Bilonick 《Journal of the Air & Waste Management Association (1995)》2013,63(4):467-480
Abstract Average concentrations of particulate matter with an aerodynamic diameter less than or equal to 2.5 μm (PM2.5) in Steubenville, OH, have decreased by more than 10 μg/m3 since the landmark Harvard Six Cities Study1 associated the city’s elevated PM2.5 concentrations with adverse health effects in the 1980s. Given the promulgation of a new National Ambient Air Quality Standard (NAAQS) for PM2.5 in 1997, a current assessment of PM2.5 in the Steubenville region is warranted. The Steubenville Comprehensive Air Monitoring Program (SCAMP) was conducted from 2000 through 2002 to provide such an assessment. The program included both an outdoor ambient air monitoring component and an indoor and personal air sampling component. This paper, which is the first in a series of four that will present results from the outdoor portion of SCAMP, provides an overview of the outdoor ambient air monitoring program and addresses statistical issues, most notably autocorrelation, that have been overlooked by many PM2.5 data analyses. The average PM2.5 concentration measured in Steubenville during SCAMP (18.4 μg/m3) was 3.4g/m3 above the annual PM2.5 NAAQS. On average, sulfate and organic material accounted for ~31% and 25%, respectively, of the total PM2.5 mass. Local sources contributed an estimated 4.6 μg/m3 to Steubenville’s mean PM2.5 concentration. PM2.5 and each of its major ionic components were significantly correlated in space across all pairs of monitoring sites in the region, suggesting the influence of meteorology and long-range transport on regional PM2.5 concentrations. Statistically significant autocorrelation was observed among time series of PM2.5 and component data collected at daily and 1-in-4-day frequencies during SCAMP. Results of spatial analyses that accounted for autocorrelation were generally consistent with findings from previous studies that did not consider autocorrelation; however, these analyses also indicated that failure to account for autocorrelation can lead to incorrect conclusions about statistical significance. 相似文献
40.
Friedrich U von Oheimb G Dziedek C Kriebitzsch WU Selbmann K Härdtle W 《Environmental pollution (Barking, Essex : 1987)》2011,159(12):3553-3559
We analysed growth strategies (biomass allocation, nutrient sequestration and allocation) of heather (Calluna vulgaris) and purple moor-grass (Molinia caerulea) seedlings in monocultures and mixtures in relation to N, P, and N + P fertilisation in a greenhouse experiment in order to simulate a heath’s pioneer phase under high airborne nitrogen (N) loads. N fertilisation increased the total biomass of both species in monocultures. In mixtures, M. caerulea sequestered about 65% of the N applied, while C. vulgaris suffered from N shortage (halving of the total biomass). Thus, in mixtures only M. caerulea will benefit from airborne N loads, and competition will become increasingly asymmetric with increasing N availability. Our results demonstrate that the heath’s pioneer phase is the crucial tipping point at which the competitive vigour of M. caerulea (high belowground allocation, efficient use of belowground resources, shortened reproductive cycles) induces a shift to dominance of grasses under increased N availability. 相似文献