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131.
In China, volatile organic compound(VOC) control directives have been continuously released and implemented for important sources and regions to tackle air pollution. The corresponding control requirements were based on VOC emission amounts(EA), but never considered the significant differentiation of VOC species in terms of atmospheric chemical reactivity. This will adversely influence the effect of VOC reduction on air quality improvement. Therefore,this study attempted to develop a comprehensive classification method for typical VOC sources in the Beijing–Tianjin–Hebei region(BTH), by combining the VOC emission amounts with the chemical reactivities of VOC species. Firstly, we obtained the VOC chemical profiles by measuring 5 key sources in the BTH region and referencing another 10 key sources, and estimated the ozone formation potential(OFP) per ton VOC emission for these sources by using the maximum incremental reactivity(MIR) index as the characteristic of source reactivity(SR). Then, we applied the data normalization method to respectively convert EA and SR to normalized EA(NEA) and normalized SR(NSR) for various sources in the BTH region.Finally, the control index(CI) was calculated, and these sources were further classified into four grades based on the normalized CI(NCI). The study results showed that in the BTH region,furniture coating, automobile coating, and road vehicles are characterized by high NCI and need to be given more attention; however, the petro-chemical industry, which was designated as an important control source by air quality managers, has a lower NCI. 相似文献
132.
双酚A和邻苯二甲酸二正丁酯在纸类上的吸附特性研究 总被引:5,自引:1,他引:4
采用序批式实验,考察了报纸对双酚A(BPA)和邻苯二甲酸二正丁酯(DnBP)的吸附能力,用Freundlich、Langmuir、Dubinin-Radushkevich(D-R)、Flory-Huggins(F-H)、BET、Temkin 6种吸附等温线模型对实验数据进行了拟合.并选择了回归系数(R2)、均方根差(RMSE)和卡方检验(X2检验)3种非线性回归方法评价了模型拟合度.结果表明,Freundlich和Temkin吸附等温线模型能很好地描述BPA和DnBP在纸类表面的吸附,BPA和DnBP的R2均大于0.95(P<0.01),RMSE和X2分别小于0.05和0.02;吸附能力与吸附质的疏水性呈正相关.由D-R和F-H吸附等温线模型拟合结果可知,BPA和DnBP的吸附平均自由能分别为1.484和1.609 kJ/mol;Gibbs自由能分别为-6.559和-7.021 kJ/mol.说明BPA和DnBP在纸类上的吸附为自发的物理吸附.BPA和DnBP在纸类上的Freundlich吸附常数k分别为0.147和0.502 mg(1-n)·L"·g-1,均高于文献报道的底泥等的吸附常数,说明生活垃圾填埋场中纸类会阻碍BPA和DnBP的迁移和生物可利用性. 相似文献
133.
Pinjing He Min Li Suyun Xu Liming Shao 《Frontiers of Environmental Science & Engineering in China》2009,3(4):404-411
This paper describes the feasibility of fresh leachate treatment by an upflow blanket filter (UBF). Through dilution and partial
effluent recycling, the organic loading rates increased from 0.51 to 14.56 kg COD/(m3·d), meanwhile the corresponding hydraulic retention time decreased from 9.0 to 3.6 d. The reactor was able to achieve steady-state
within 80 d. Based on the distribution of COD fluxes in the process, it was concluded that anabolism was the main pathway
of COD removal in the initial phase (1–33 d), accounting for 57%–85% of total COD removed. As the anaerobic consortium of
bacteria reached steady-state (after 70–86 d), the majority of COD removed was transformed into methane, because the specific
methane yield was close to the theoretical value (0.36 L CH4/(g CODdeg)). 相似文献
134.
阴霾天气PM_(10)的微观特征及生物活性研究 总被引:2,自引:0,他引:2
利用高分辨率场发射扫描电镜(FESEM)、图像分析技术(IA),对北京市2004年12月一次严重的阴霾天气条件下采集的PM10(指空气动力学直径小于10μm的颗粒物)的微观形貌、粒度分布、主要颗粒物类型进行了分析,并运用质粒DNA评价法对阴霾和非阴霾天气条件下的PM10样品的生物活性进行了对比研究。结果表明,阴霾天气时PM10样品中以粒度较小的烟尘及其集合体为主,且多呈湿状,含有较多的二次颗粒物,并发现了残余的有机液滴颗粒。质粒DNA实验的结果显示,阴霾天气PM10样品的水溶和全样样品的TD20值(造成20%DNA破坏时所需要的样品剂量)分别为93μg.ml-1和50μg.ml-1,而同一月份非阴霾天气条件下PM10样品的水溶和全样样品的TD20值分别为200μg.ml-1和160μg.ml-1,表明阴霾天气PM10样品比非阴霾天气样品具较强的生物活性,即对人体健康存在着潜在的危害。且无论是阴霾还是非阴霾天气条件下的PM10的全样样品均较水溶样品具更大的生物活性。 相似文献
135.
136.
Pinjing He Na Yang Wenjuan Fang Fan Lü Liming Shao 《Frontiers of Environmental Science & Engineering in China》2011,5(2):175-185
To understand the influence patterns and interactions of three important environmental factors, i.e. soil water content, oxygen
concentration, and ammonium addition, on methane oxidation, the soils from landfill cover layers were incubated under full
factorial parameter settings. In addition to the methane oxidation rate, the quantities and community structures of methanotrophs
were analyzed to determine the methane oxidation capacity of the soils. Canonical correspondence analysis was utilized to
distinguish the important impact factors. Water content was found to be the most important factor influencing the methane
oxidation rate and Type II methanotrophs, and the optimum value was 15% (w/w), which induced methane oxidation rates 10- and
6- times greater than those observed at 5% (w/w) and 20% (w/w), respectively. Ambient oxygen conditions were more suitable
for methane oxidation than 3% oxygen. The addition of 100 mg-N·kgdrysoil−1 of ammonium induced different effects on methane oxidation capacity when conducted at low or high water content. With regard
to the methanotrophs, Type II was sensitive to the changes of water content, while Type I was influenced by oxygen content.
Furthermore, the methanotrophic acidophile, Verrucomicrobia, was detected in soils with a pH of 4.9, which extended their known living environments. 相似文献
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