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71.
Higher concentrations of Hg can be emitted from coal pyrolysis or gasification than from coal combustion, especially elemental Hg. Highly efficient Hg removal technology from coal-derived fuel gas is thus of great importance. Based on the very excellent Hg removal ability of Pd and the high adsorption abilities of activated carbon(AC) for H2 S and Hg, a series of Pd/AC sorbents was prepared by using pore volume impregnation, and their performance in capturing Hg and H2 S from coal-derived fuel gas was investigated using a laboratory-scale fixed-bed reactor. The effects of loading amount, reaction temperature and reaction atmosphere on Hg removal from coal-derived fuel gas were studied. The sorbents were characterized by N2 adsorption, X-ray diffraction(XRD) and X-ray photoelectron spectroscopy(XPS). The results indicated that the efficiency of Hg removal increased with the increasing of Pd loading amount, but the effective utilization rate of the active component Pd decreased significantly at the same time. High temperature had a negative influence on the Hg removal. The efficiency of Hg removal in the N2-H2S-H2-CO-Hg atmosphere(simulated coal gas) was higher than that in N2-H2S-Hg and N2-Hg atmospheres, which showed that H2 and CO, with their reducing capacity, could benefit promote the removal of Hg. The XPS results suggested that there were two different ways of capturing Hg over sorbents in N2-H2S-Hg and N2-Hg atmospheres. 相似文献
72.
采用微波消解法对固体废物浸出液样品进行前处理,采用乙炔-空气火焰原子吸收法测定钡的含量,检出限为2.04mg/L,加标回收率为94.5%,精密度为4.85%-6.81%。 相似文献
73.
74.
基于本地污染源调查的杭州市大气污染物排放清单研究 总被引:4,自引:0,他引:4
基于实地调查数据并辅以统计数据,采用物料衡算法和排放因子法,估算了杭州市2015年大气污染物排放清单,并选取经纬度坐标、路网、航道、土地类型和人口等数据作为权重因子,研究了该地区各类排放源污染物排放空间分布特征.结果表明,杭州市2015年SO_2、NO_x、CO、VOCs、PM_(10)、PM_(2.5)和NH_3年排放总量分别为22.20×10~3、108.17×10~3、192.10×10~3、134.94×10~3、78.12×10~3、27.65×10~3和59.75×10~3t.工业源是杭州市SO_2排放的主要来源,移动源对NO_x和CO的排放贡献最为显著,扬尘源是杭州市PM_(10)和PM_(2.5)排放的最主要来源,其次为工业源;VOCs排放的主要来源依次为工业源、天然源和移动源;NH_3排放主要来自农业源.从空间分布来看,排放主要集中在中心城区及其周边的萧山、下沙、大江东、余杭和富阳等工业企业相对密集的区域.本研究建立的排放清单在污染源覆盖范围和排放因子方面仍然存在一定的不确定性,建议在后续研究中重点开展低、小、散企业及本地化排放因子调查研究工作,进一步提升大气污染物排放清单的准确度. 相似文献
75.
为研究地铁网络化运营枢纽车站火灾烟气扩散特征和防排烟技术,根据工程资料和标准规范对典型多线换乘车站进行1∶10火灾实验模型设计,并依据设计方案完成车站模型主体结构和通风排烟系统的搭建,同时在各个防烟分区设计安装温度、流速、烟气浓度和热辐射测量装置,可实现对“T”形、“十”形和“L”形换乘等不同换乘形式车站的火灾场景模拟和危险参数测量。研究结果表明:该模型装置能够开展一系列针对不同换乘形式和通风模式的火灾实验,对于全面揭示大型换乘车站火灾烟气运动规律、验证并优化火灾防排烟设计方法、支撑复杂结构枢纽车站火灾烟气控制技术具有重要意义。 相似文献
76.
工业内窥镜是电站锅炉内部检验中不可或缺的设备,主要用来对集箱、减温器、受热面管等内部人眼无法观察到的地方进行检验,从而确定承压部件内部是否存在严重影响锅炉安全运行的缺陷.本文通过对锅炉内窥实例进行分析和总结,阐述内窥镜检查在锅炉内检中的重要性并给相关工作人员提供借鉴与参考. 相似文献
77.
Zihao Li Yang Geng Lei Ma Xiaoyin Chen Junhua Li Huazhen Chang Johannes W. Schwank 《Frontiers of Environmental Science & Engineering》2020,14(4):65
78.
Yapeng Song Hui Gong Jianbing Wang Fengmin Chang Kaijun Wang 《Frontiers of Environmental Science & Engineering》2020,14(4):64
79.
Yiming Chang Liangang Mao Lan Zhang Yanning Zhang Hongyun Jiang 《Environmental science and pollution research international》2020,27(10):10286-10295
Compound pollution refers to two or more kinds of pollutants with different properties, a pollutant from different sources, or the simultaneous existence of two or more different types of pollutants in the same environment. In this study, we aimed to investigate the individual and combined toxicity of the insecticide imidacloprid (IMI), the herbicide acetochlor (ACT), and the fungicide tebuconazole (TBZ) to zebrafish. The acute toxicity test results showed that the 96-h LC50 values of IMI, ACT, and TBZ were 276.84 (259.62–294.35) mg active ingredient (a.i.) L−1, 1.52 (1.34–1.74) mg a.i. L−1, and 8.16 (7.7–8.6) mg a.i. L−1, respectively. The combinations of IMI, ACT, and TBZ with toxicity ratios of 1:2:2, 1:4:4, 2:4:1, and 4:1:4 displayed synergistic toxic effects on zebrafish, while the toxicity ratios of 1:1:1, 1:1:2, 2:1:2, 2:2:1, and 4:2:1 of IMI, ACT, and TBZ, respectively, exhibited antagonistic toxic effects on zebrafish. The following experiments were performed with a toxicity ratio of 1:4:4 (IMI:ACT:TBZ). The activities of four enzyme biomarkers related to oxidative stress in the liver, catalase (CAT), superoxide dismutase (SOD), glutathione S-transferase (GST), and malondialdehyde (MDA) content were evaluated in each exposure group on days 7, 14, 21, and 28. Compared with those of the control group, the activities of CAT, SOD, and GST and the MDA content were significantly altered at different time points in the individual and combined exposure groups. Additionally, the activities of CAT, SOD, and GST and the MDA content were significantly altered in the combined group compared with those of the individual group after 14 days or 21 days of exposure. Therefore, it was confirmed that combined toxicity studies are indispensable in risk assessment. 相似文献
80.
Song Yao Wang Liancheng Lv Baoliang Chang Guozhang Jiao Weizhou Liu Youzhi 《Environmental science and pollution research international》2020,27(7):7015-7024
Environmental Science and Pollution Research - In this study, porous activated carbon balls supported by nanoscale zero-valent iron composites (Fe@PACB-700) were used for the first time for the... 相似文献