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371.
Sakan S Grzetić I Dordević D 《Environmental science and pollution research international》2007,14(4):229-236
Introduction In this work, sediments of the River Tisa (Tisza) are studied to assess their environmental pollution levels for some major
heavy metals, as well as to predict the investigated elements’ mobility on the basis of their association type with the substrate.
The Tisa River catchments area is a subbasin of the River Danube. Part of this river, 166 km long, belongs to the Serbian
province of Vojvodina, before it flows into the Danube. It has been chosen for our investigation, because it has been exposed
to intense pollution in the last decades.
Materials and Methods The river sediment samples were collected at 32 locations. The proportions of sand, silt and clay fractions were determined.
The sequential extraction procedure following a modified Tessier method was applied for speciation of the metal forms in the
collected samples. The metal concentrations of Zn, Cd, Pb, Ni, Cu, Cr, Fe and Mn in extracts were determined by atomic absorption
spectroscopy.
Results and Discussion Granulometric analysis showed that some 50% of the Tisa River sediments were silt and clay, while the rest was sand with quartz,
as the main constituent. The average metal content of the surface river sediment samples for every fraction of sequential
extraction was presented and discussed in relation to pH, Eh and metal fractionation. The average metal content from the Tisa
River sediments, obtained as an average of the metal’s concentration released in all five sequential extraction fractions
was compared with: average metal contents of the Tisa River sediments in Hungary, metal content in soils formed on the Tisa
River alluvium of Vojvodina, average metal content in soils of Vojvodina, and average metal content in soils of Hungary. An
assessment of metal pollution levels in Tisa River sediments was made by comparing mean values for obtained results for the
Tisa River sediments with the freshwater sediment’s Quality Guidelines as published by US EPA, Environment Canada and soil
standards for Serbia.
Conclusion According to US EPA and Canadian Quality Guidelines for freshwater sediments, the concentration of heavy metals in Tisa sediments
were: (a) much higher than defined concentrations below which harmful effects on river biota are unlikely to be observed,
(b) below defined concentrations above which harmful effects on river biota are likely to be observed. The concentration levels
of Pb, Ni, Cu and Cr in Tisa River sediments are safe when compared with Serbian MAQ (Maximum Allowed Quantity) standards
for soils, but they are unsafe in the case of Zn and Cd.
Recommendations and Outlook The quality of sediments in the Tisa River was on the border line between potentially polluted and polluted. This line could
very easily be exceeded since the quality of sediments in the Tisa River in Hungary was already worse than in Serbia. These
results indicated the need for further monitoring of heavy metals in that locality. 相似文献
372.
Crnković D Ristić M Jovanović A Antonović D 《Environmental monitoring and assessment》2007,125(1-3):75-83
Polycyclic aromatic hydrocarbons (PAHs) were analysed in 39 soil samples (0–10 cm upper layer) collected in Belgrade, the
capital of Serbia. The sampling sites were randomly selected from urban, urban/recreational and rural areas; the samples were
collected in April and December 2003 and July and October 2004.
The sum of the 16 PAHs corresponding to the recreational zone (298 μg/kg) was close to the urban zone (375 μg/kg). Mean soil
ΣPAH concentration from rural areas was 18 μg/kg dry weight. Comparing to values observed in the urbanized locations around
the world, the overall levels of PAHs in this study are low. The PAH ratios obtained pointed to a domination of pyrogenically
formed PAHs in the examined soils. The dominant PAHs in soil samples in urban zones were fluoranthene, benz[a]anthracene, phenanthrene and pyrene, mostly emitted from noncatalyst vehicles which are still in use in Serbia. The total
carcinogenic potency for each sampling site was calculated. Regardless of the used carcinogenic activity factors, carcinogenic
potency of 7 sites were 3–9 times higher than the reference ones indicating the increased carcinogenic burden of soils from
these sites. 相似文献
373.
The study was aimed at determining the levels of metals in water samples and muscles of the fish caught in the Una River basin,
located in the northwestern part of Bosnia and Herzegovina. For that purpose, three fish species: Brown Trout (Salmo trutta m. fario), Grayling (Thymallus thymallus) and Californian Trout (Salmo gairdneri), together with stem water samples, were analyzed for metal concentrations (Pb, Hg, Cd, As, Mn, Ni, Cu, Cr, Se, Co, Sn, Zn,
Fe, Ca, P) during a 2-year period. The fish was captured using electric fishing, nets or fishing equipment. The capture was
undertaken on three sites (the river source, the middle flow and the river mouth) of each of the five biggest rivers belonging
to the Una River basin (Unac, Krušnica, Sana, Klokot, and Una). The concentrations of metals in each sample were determined
via atomic absorption spectrophotometry. In the tested waters, the presence of Mn in concentrations higher than permitted
(0.07 mg/l) had been detected. In the tested meat, the following average concentrations of metals (mg/kg) had been found:
Pb (0.67), Cd (0.06), Mn (0.65), Ni (0.15), Cu (0.79), Cr (1.05), Se (0.03), Zn (8.92), Fe (5.40), Ca (14.68), and P (10.85).
The correlation between Mn concentrations identified in the tested waters and those identified in the meat of Brown Trout
was revealed to be statistically significant, which confirms that, over time, bioaccumulation of metals took place. Even though
the results were not indicative of contamination, they strongly suggest that constant monitoring of the ecosystems in reference
should be implemented. 相似文献