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201.
Hongxing Dai Hongxia Lin Jinmo Wu Fan Zhou Xiaolong Zhao Pengfei Lu Guanghui Sun Yuhan Song Yayun Li Xiaoyong Liu 《环境科学学报(英文版)》2023,35(2):570-590
Semiconductor photocatalytic technology has shown great prospects in converting solar energy into chemical energy to mitigate energy crisis and solve environmental pollution problems. The key issue is the development of high-efficiency photocatalysts. Various strategies in the state-of-the-art advancements, such as heterostructure construction, heteroatom doping, metal/single atom loading, and defect engineering, have been presented for the graphitic carbon nitride (g-C3N4)-based nanocomposite catalysts to design their surface chemical environments and internal electronic structures to make them more suitable for different photocatalytic applications. In this review, nanoarchitecture design, synthesis methods, photochemical properties, potential photocatalytic applications, and related reaction mechanisms of the modified high-efficiency carbon nitride-based photocatalysts were briefly summarized. The superior photocatalytic performance was identified to be associated with the enhanced visible-light response, fast photoinduced electron-hole separation, efficient charge migration, and increased unsaturated active sites. Moreover, the further advance of the visible-light harvesting and solar-to-energy conversions are proposed. 相似文献
202.
Evaluationonabundanceordeficiencyofavai-labletraceelementsinsoilofmiddleareainChinaandtheeffectofapplyingtraceelementfertiliz... 相似文献
203.
The air-dust samples collected from petro-chemical industrial region in the suburb of Lanzhou and from a certain rural region 64 km away from the city were extracted, with a mixed solvent (benzene: hexane: isopropanol=7:2:1) for 8 hours. A strong free radical signal at g= 2.00 of air-dust itself and a hyperfine splitting EPR signal of extract from air-dust have been detected. The sister chromatid exchange frequency (SCE) was increased by extracts of both dusts from the industrial region and from the rural region. If a chemical is able to increase SCE up to twice as high as the control, this chemical is considered to be mutagenic and/or carcinogenic. The double SCE frequency concentration is 23 μg/ml for the dust extract obtained from the industrial region and 47μg/ml for that from the rural region. Extracts were able to damage to DNA template. Results indicated that the mutagenicity and/or carcinogenicity of the extracts obtained from the petro-chemical industrial region were stronger than that of the 相似文献
204.
Fan Cheng xin 《环境科学学报(英文版)》1998,10(1):49-55
EfectsofmainrangeandstrengthfactorsonchangeofCODinashalowlakeFanChengxinNanjingInstituteofGeographyandLimnology,ChineseAcad... 相似文献
205.
This paper presents a model that can aid planners in defining the total allowable pollutant discharge in the planning region,accounting for the dynamic and stochastic character of meteorological conditions.This is accomplished by integrating Monte Carlo simulation and using genetic algorithm to solve the model.The model is demonstrated by using a realistic air urban-scale SO2 control problem in the Yuxi City of China.To evaluate effectiveness of the model,results of the approach are shown to compare with those of the linear deterministic procedures. This paper also provides a valuable insight into how air quality targets should be made when the air pollutant will not threat the residents‘ health.Finally,a discussion of the areas for further research are briefly delineated. 相似文献
206.
Three columns each with 770 cm2 of surface area and 60-105 cm effective depth were set up for this study. These columns were filled with compacted, stabilized refuse. High-strength brewery wastewaters were uniformly trickled down the medium. Overall, 16 runs with various organic loadings were tested and the results demonstrated that the stabilized refuse had excellent capability in removing chemical oxygen demand (COD). The COD removal efficiency reached 95% at a depth of 60 cm at Q = 8 L/day for the initial COD of approximately 6000 mg/L and the efficiency increased to >99% at a depth of 90 cm (organic loading of 0.69 kg/m3/day). As would be expected, the filter performance is a function of flow rate, influent COD concentration, and bed depth. The Schulze equation is able to predict the COD removal performance well. The variations of pH, oxidation reduction potential, and volatile fatty acids indicated that the acidogenesis reaction occurred in the upper layers. 相似文献
207.
Dan Xiao Zhaofeng Lyu Shiheng Chen Yang Huo Wei Fan Mingxin Huo 《Frontiers of Environmental Science & Engineering》2022,16(9):112
208.
The purpose of this work is to remove Pb(II) from the aqueous solution using a type of hydrogel composite. A hydrogel composite consisting of waste linear low density polyethylene, acrylic acid, starch, and organo-montmorillonite was prepared through emulsion polymerization method. Fourier transform infrared spectroscopy(FTIR), Solid carbon nuclear magnetic resonance spectroscopy(CNMR)), silicon-29 nuclear magnetic resonance spectroscopy(Si NMR)), and X-ray diffraction spectroscope((XRD) were applied to characterize the hydrogel composite. The hydrogel composite was then employed as an adsorbent for the removal of Pb(II) from the aqueous solution. The Pb(II)-loaded hydrogel composite was characterized using Fourier transform infrared spectroscopy(FTIR)),scanning electron microscopy(SEM)), and X-ray photoelectron spectroscopy((XPS)). From XPS results, it was found that the carboxyl and hydroxyl groups of the hydrogel composite participated in the removal of Pb(II). Kinetic studies indicated that the adsorption of Pb(II)followed the pseudo-second-order equation. It was also found that the Langmuir model described the adsorption isotherm better than the Freundlich isotherm. The maximum removal capacity of the hydrogel composite for Pb(II) ions was 430 mg/g. Thus, the waste linear low-density polyethylene-g-poly(acrylic acid)-co-starch/organo-montmorillonite hydrogel composite could be a promising Pb(II) adsorbent. 相似文献
209.
CO2 is the main greenhouse gas which causes global climatic changes on larger scale. Many techniques have been utilised to capture CO2. Membrane gas separation is a fast growing CO2 capture technique, particularly gas separation by composite membranes. The separation of CO2 by a membrane is not just a process to physically sieve out of CO2 through the controlled membrane pore size. It mainly depends upon diffusion and solubility of gases, particularly for composite dense membranes. The blended components in composite membranes have a high capability to adsorb CO2. The adsorption kinetics of the gases may directly affect diffusion and solubility. In this study, we have investigated the adsorption behaviour of CO2 in pure and composite membranes to explore the complete understanding of diffusion and solubility of CO2 through membranes. Pure cellulose acetate (CA) and cellulose acetate-titania nanoparticle (CA-TiO2) composite membranes were fabricated and characterised using SEM and FTIR analysis. The results indicated that the blended CA-TiO2 membrane adsorbed more quantity of CO2 gas as compared to pure CA membrane. The high CO2 adsorption capacity may enhance the diffusion and solubility of CO2 in the CA-TiO2 composite membrane, which results in a better CO2 separation. The experimental data was modelled by Pseudo first-order, pseudo second order and intra particle diffusion models. According to correlation factor R2, the Pseudo second order model was fitted well with experimental data. The intra particle diffusion model revealed that adsorption in dense membranes was not solely consisting of intra particle diffusion. 相似文献
210.
Removal of tetracycline from water by Fe-Mn binary oxide 总被引:2,自引:0,他引:2
Significant concerns have been raised over the presence of antibiotics including tetracyclines in aquatic environments. A series of Fe-Mn binary oxide with different Fe:Mn molar ratios was synthesized by a simultaneous oxidation and coprecipitation process for TC removal. Results showed that Fe-Mn binary oxide had higher removal efficiency than that of hydrous iron oxide and hydrous manganese oxide, and that the oxide with a Fe:Mn molar ratio of 5:1 was the best in removal than other molar ratios. The tetracycline removal was highly pH dependent. The removal of tetracycline decreased with the increase of initial concentration, but the absolute removal quantity was more at high concentration. The presence of cations and anions such as Ca2+, Mg2+, CO32- and SO42- had no significant effect on the tetracycline removal in our experimental conditions, while SiO32- and PO43- had hindered the adsorption of tetracycline. The mechanism investigation found that tetracycline removal was mainly achieved by the replacement of surface hydroxyl groups by the tetracycline species and formation of surface complexes at the water/oxide interface. This primary study suggests that Fe-Mn binary oxide with a proper Fe:Mn molar ratio will be a very promising material for the removal of tetracycline from aqueous solutions. 相似文献