全文获取类型
收费全文 | 6260篇 |
免费 | 56篇 |
国内免费 | 32篇 |
专业分类
安全科学 | 145篇 |
废物处理 | 285篇 |
环保管理 | 462篇 |
综合类 | 1006篇 |
基础理论 | 1540篇 |
环境理论 | 6篇 |
污染及防治 | 2027篇 |
评价与监测 | 485篇 |
社会与环境 | 373篇 |
灾害及防治 | 19篇 |
出版年
2023年 | 64篇 |
2022年 | 151篇 |
2021年 | 173篇 |
2020年 | 81篇 |
2019年 | 103篇 |
2018年 | 255篇 |
2017年 | 266篇 |
2016年 | 337篇 |
2015年 | 224篇 |
2014年 | 329篇 |
2013年 | 486篇 |
2012年 | 352篇 |
2011年 | 413篇 |
2010年 | 273篇 |
2009年 | 250篇 |
2008年 | 372篇 |
2007年 | 336篇 |
2006年 | 281篇 |
2005年 | 220篇 |
2004年 | 213篇 |
2003年 | 163篇 |
2002年 | 141篇 |
2001年 | 94篇 |
2000年 | 55篇 |
1999年 | 52篇 |
1998年 | 31篇 |
1997年 | 26篇 |
1996年 | 27篇 |
1995年 | 37篇 |
1994年 | 34篇 |
1993年 | 20篇 |
1992年 | 23篇 |
1991年 | 24篇 |
1990年 | 22篇 |
1989年 | 20篇 |
1988年 | 18篇 |
1987年 | 12篇 |
1986年 | 26篇 |
1985年 | 15篇 |
1984年 | 14篇 |
1983年 | 13篇 |
1982年 | 22篇 |
1980年 | 13篇 |
1976年 | 12篇 |
1966年 | 19篇 |
1965年 | 12篇 |
1964年 | 11篇 |
1959年 | 10篇 |
1956年 | 11篇 |
1954年 | 11篇 |
排序方式: 共有6348条查询结果,搜索用时 14 毫秒
61.
Phylogenetic analyses of the left domain of the mitochondrial DNA control-region sequence have been used to examine the relationships
among species of the genus Merluccius (Rafinesque, 1810), and to compare these with hypotheses based on morphological, meristic and allozyme characters. Analysis
of aligned sequences revealed that transition bias was much lower than in mammalian mtDNA, and that nucleotide composition
of control-region sequences was biased toward A and T. We have roughly calibrated a molecular clock for the genus, based on
the rise of the Isthmus of Panamá, which is believed to have created a barrier to dispersal between marine species of the
Atlantic and Pacific Oceans. Our mtDNA-based phylogeny was highly congruent with allozyme-based phylogenies, but poorly so
with a previously described phylogeny based on morphology. Specifically, our phylogeny resolved two well-supported principal
clades, one of American (west Atlantic and east Pacific) species and the other of Euro–African (east Atlantic) species. This
suggests an evolutionary history during which the ancestral lineage of Merluccius was divided between two geographic regions, with subsequent dispersal and vicariant events resulting in the evolution and
distribution of extant taxa. However, the relationships between some taxa within the American clade could not be resolved.
We suggest that this is consistent with an hypothesis of a rapid origin and radiation of these taxa.
Received: 12 December 1998 / Accepted: 15 October 1999 相似文献
62.
R. Wilson G. Peters J. Regel D. Grémillet K. Pütz M. Kierspel H. Weimerskirch J. Cooper 《Marine Biology》1998,130(4):559-566
Stomach temperature loggers have proved useful for the study of feeding activity in free-living seabirds, but their usage
has been restricted because they are frequently dislodged and lost during the seabirds' regular regurgitation of indigestible
prey remains. In the present study we examine the incidence of spontaneous regurgitation (pellet production) in free-living
seabirds, consider the effect this has on the likely retrieval of stomach temperature loggers and present a structural modification
of the logger housings which leads to a much lower incidence of regurgitation. Systems were tested on albatrosses, cormorants,
gannets and penguins.
Received: 15 July 1997 / Accepted: 31 October 1997 相似文献
63.
K. Håkan Olsén J. Torbjörn Järvi Ian Mayer Erik Petersson Frederieke Kroon 《Chemoecology》1998,8(1):9-17
Summary. In the present experiment the behaviour and endocrine status of males of the brown trout, Salmo trutta L., (Salmoniformes: Salmonidae) were studied when males were kept in a stream tank with a nest digging female. Groups of
mature adult males and precocious intact or anosmic male parr were placed with the nesting female so that the group resembled
a natural spawning situation with big anadromous fish acting as dominant males and precocious parr acting as “sneakers”. A
control experiment was also run with only males without a female present. In intact parr there were significant positive correlations
between the per cent of the total observation time spent with a female, milt volume, and plasma concentration of 17α, 20β-dihydroxy-4-pregnen-3-one.
Anosmic parr had significantly lower volumes of strippable milt and gonadal steroid hormone levels compared with intact parr.
However, no differences were found in the control experiment. Significantly fewer anosmic parr attended and courted the nesting
female and those anosmic fish that attended the female had significantly lower plasma levels of gonadal hormones. Intact parr
also displayed a greater number of agonistic acts against other parr without any difference in fighting ability. No differences
in aggression occured in the control experiment. In adult males together with a female, post-experimental gonadal steroid
hormone levels were higher than pre-experimental levels. Positive correlations between aggression and androgen hormone levels
were observed in adult males. No differences in plasma hormone levels were observed between adult males and intact precocious
males. The results show that olfactory occlusion results in low steroid hormone levels and milt volumes in precocious males
placed in a spawning situation. The courting behaviour was also affected by anosmia. Odours from the nesting female may have
caused the enhanced plasma hormone levels and stimulated the males to attend the female.
Received 15 May 1997; accepted 29 June 1997. 相似文献
64.
Urban Development and Air Quality in San Luis City, Argentina 总被引:3,自引:0,他引:3
Rubén Lijteroff Virgilio Cortinez Julio Raba 《Environmental monitoring and assessment》1999,57(2):169-182
Some factors such as the high population growth, along with insufficient housing, health and sanitary services, obsolete industrial technology and the lack of environmental management programs, give rise to contamination in Latin-American cities. Owing to the urban characteristics of San Luis, a detailed analysis of air quality was planned as part of a more comprehensive study, in order to make an environmental diagnosis of the city after the demographical and economic upgrowth over the last 15 years. It has been concluded that air pollution levels in San Luis are higher than those expected for a medium-size city. The reported high levels were attributed to important industrial activity, responsible not only for the direct of polluting gases to the atmosphere but also as the principal cause of the urban expansion. The levels of CO and SO2 (ppm) found in the city can be considered as high. Some weeks during the sampling measure values were appreciably higher than the maximum tolerance levels established. The urban area under study was separated into five defined areas, which allowed to make comparisons in order to identify specific contamination problems. The slopes corresponding to the plot polluting substances concentration vs. wind speed were lower than the expected values. Because of the urban area characteristics, different micrometeorological effects facilitating a low air exchange can be generated, and consequently increasing the contamination levels. Thus, it is correct to conclude that the degradation processes are not occurring in a single environmental plane. Accordingly, air contamination rate in San Luis city could be considered as evidence of other upper-scale regional environmental degradation processes. 相似文献
65.
In field arsenic removal from natural water by zero-valent iron assisted by solar radiation 总被引:1,自引:0,他引:1
Cornejo L Lienqueo H Arenas M Acarapi J Contreras D Yáñez J Mansilla HD 《Environmental pollution (Barking, Essex : 1987)》2008,156(3):827-831
An in situ arsenic removal method applicable to highly contaminated water is presented. The method is based in the use of steel wool, lemon juice and solar radiation. The method was evaluated using water from the Camarones River, Atacama Desert in northern Chile, in which the arsenic concentration ranges between 1000 and 1300 μg L−1. Response surface method analysis was used to optimize the amount of zero-valent iron (steel wool) and the citrate concentration (lemon juice) to be used. The optimal conditions when using solar radiation to remove arsenic from natural water from the Camarones river are: 1.3 g L−1 of steel wool and one drop (ca. 0.04 mL) of lemon juice. Under these conditions, removal percentages are higher than 99.5% and the final arsenic concentration is below 10 μg L−1. This highly effective arsenic removal method is easy to use and inexpensive to implement. 相似文献
66.
Romero-Ruiz A Alhama J Blasco J Gómez-Ariza JL López-Barea J 《Environmental pollution (Barking, Essex : 1987)》2008,156(3):1340-1347
Metallothionein (MT) and other biomarker levels were measured in Scrobicularia plana clams to assess pollution of the Guadalquivir Estuary possibly affected by metals released from Aznalcóllar pyrite mine in 1998. After optimizing reagent concentrations for monobromobimane derivatization, MT levels were quantified by reversed-phase high-performance liquid chromatography coupled to fluorescence detection (RP-HPLC-FD) in heated or unheated digestive gland extracts and compared to those obtained by differential pulse polarography (DPP). MT content assayed by RP-HPLC-FD in unheated samples was higher than that obtained by DPP and correlated better with metals and anti-oxidant activities. MT assay by RP-HPLC-FD in unheated extracts would be preferable for assessing metal pollution, due to its greater sensitivity and specificity. In addition to MT induction, glyoxalase II inhibition was well correlated with metal contents. Our results suggest that metals at the estuary do not originate from Aznalcóllar spill, but from those carried along by the river and deposited at its concave bank. 相似文献
67.
In multiphase systems capillary pressures play a significant role on fluid movement and retention. The facility to predict
the effect of different thermal remediation strategies requires the knowledge of the effect of temperature on capillary pressure-saturation
relationships in the soils.
The objective of recent study was (a) to develop a technique for routinely measuring the pressure-saturation curves of soil
samples saturated with a nonpolar liquid at different regulated temperatures (b) to build a database using the measured pressure-saturation
curves and the physical, chemical properties of the model soils (c) to establish the dependence of nonaqueous phase liquid
retention on the soil properties and the temperature.
The retention curves (extraction isotherms) with nonaqueous phase liquid were determined using a modified
pressure plate extractor. The wetting phase was a non-aromatic hydrocarbon distillation product. Pressure plates were designed and constructed in
the laboratory of our department. The temperature was held constant at 20, 40 and 60 ∘C.
Statistical analysis was performed involving selected soil parameters and the measured nonaqueous phase liquid retention data.
The results show that knowing some easily measurable soil parameters (bulk density, particle size distribution, humus and
lime content) we can estimate the nonaqueous phase liquid retention of the soils. The measured “extraction isotherms” provide
essential information about the temperature-dependency of pressure-saturation curves. 相似文献
68.
Performance of a low cost MBT prior to landfilling: study of the biological treatment of size reduced MSW without mechanical sorting 总被引:3,自引:0,他引:3
In France, the interest in Mechanical Biological Treatment (MBT) prior to landfilling is actually growing. In the absence of acceptance criteria for the waste to be landfilled, an alternative to the intensive, high-technology MBT can only find its place in the French context if it shows substantial benefits from an environmental, economic or operational point of view. This paper presents an experiment of low-cost MBT of size reduced MSW without material splitting. The performance of an experimental, pilot-scale mechanical and biological treatment process has been studied on 37.5 Mg of raw municipal solid waste. The mechanical process has been kept simple with only coarse shredding and no material recovery. The biological treatment, which was a low-cost forced aeration process, was monitored for 25 weeks. The biogas production potential of the waste was reduced by 90% to 19 NL kgDM(-1). The initial AT4 index of 82.9 mg O2 gDM(-1) decreased to 16.0 mg O2 gDM(-1). After 25 weeks of aerobic treatment, the dry mass loss reached 37%, while the mass of waste going to landfill was reduced by 28%. The average performances of the process were explained by the biological process itself, which was not optimal, and also by the characteristics of the input waste. The high particle size of the treated waste and the high content of slowly biodegradable matter (such as paper and cardboard) may both be significant drawbacks for the biological stabilisation of waste. 相似文献
69.
Sulfate removal from waste chemicals by precipitation 总被引:3,自引:0,他引:3
Chemical oxidation using Fenton's reagent has proven to be a viable alternative to the oxidative destruction of organic pollutants in mixed waste chemicals, but the sulfate concentration in the treated liquor was still above the acceptable limits for effluent discharge. In this paper, the feasibility of sulfate removal from complex laboratory wastewaters using barium and calcium precipitation was investigated. The process was applied to different wastewater cases (two composite samples generated in different periods) in order to study the effect of the wastewater composition on the sulfate precipitation. The experiments were performed with raw and oxidized wastewater samples, and carried out according to the following steps: (1) evaluate the pH effect upon sulfate precipitation on raw wastewaters at pH range of 2-8; (2) conduct sulfate precipitation experiments on raw and oxidized wastewaters; and (3) characterize the precipitate yielded. At a concentration of 80 g L(-1), barium precipitation achieved a sulfate removal up to 61.4% while calcium precipitation provided over 99% sulfate removal in raw and oxidized wastewaters and for both samples. Calcium precipitation was chosen to be performed after Fenton's oxidation; hence this process configuration favors the production of higher quality precipitates. The results showed that, when dried at 105 degrees C, the precipitate is composed of hemidrate and anhydrous calcium sulfate ( approximately 99.8%) and trace metals ( approximately 0.2%: Fe, Cr, Mn, Co, Ag, Mg, K, Na), what makes it suitable for reuse in innumerous processes. 相似文献
70.
This paper performs a cost-effectiveness analysis of some of the best available technologies (BAT) that can contribute to decreasing the energy consumption and CO2 emissions in the European Union’s (EU27) cement industry. Several capital budgeting decision criteria have been used (the payback period, the net present value and the internal rate of return) to study whether or not an investment should be considered worthwhile. The results show that, independent of the capital budgeting decision criteria used, the number of cost-effective retrofitting possibilities available is large compared to the rate of improvements that the industry undertakes annually. This shows the insensitivity of the industry to financial criteria when it comes to making their investment decisions. The possible thermal energy improvement in the clinker production, if all these BATs were implemented, has been quantified to be around 10%. This achievement would place the cement industry in the upper bound of the benchmark range for clinker manufacture. However considering the delays observed nowadays in terms of diffusion of BATs in the cement industry, it requires a conducive policy environment that combines support for both technology development and to their deployment. 相似文献