全文获取类型
收费全文 | 289篇 |
免费 | 1篇 |
国内免费 | 9篇 |
专业分类
安全科学 | 6篇 |
废物处理 | 65篇 |
环保管理 | 11篇 |
综合类 | 43篇 |
基础理论 | 60篇 |
污染及防治 | 88篇 |
评价与监测 | 12篇 |
社会与环境 | 12篇 |
灾害及防治 | 2篇 |
出版年
2023年 | 2篇 |
2022年 | 4篇 |
2021年 | 4篇 |
2020年 | 2篇 |
2019年 | 1篇 |
2018年 | 10篇 |
2017年 | 5篇 |
2016年 | 7篇 |
2015年 | 8篇 |
2014年 | 10篇 |
2013年 | 20篇 |
2012年 | 7篇 |
2011年 | 19篇 |
2010年 | 7篇 |
2009年 | 27篇 |
2008年 | 17篇 |
2007年 | 21篇 |
2006年 | 21篇 |
2005年 | 18篇 |
2004年 | 19篇 |
2003年 | 18篇 |
2002年 | 5篇 |
2001年 | 7篇 |
2000年 | 3篇 |
1999年 | 4篇 |
1998年 | 1篇 |
1997年 | 6篇 |
1996年 | 2篇 |
1995年 | 4篇 |
1994年 | 3篇 |
1993年 | 2篇 |
1989年 | 2篇 |
1987年 | 1篇 |
1984年 | 3篇 |
1982年 | 1篇 |
1977年 | 1篇 |
1976年 | 1篇 |
1973年 | 1篇 |
1972年 | 1篇 |
1969年 | 1篇 |
1968年 | 1篇 |
1965年 | 1篇 |
1961年 | 1篇 |
排序方式: 共有299条查询结果,搜索用时 15 毫秒
171.
Cell growth of a coastal marine diatom, Chaetoceros sociale, in the presence of different premixed organic-Fe(III) complexes [EDTA-Fe(III) (100:1 and 2:1), citric-Fe(III) (100:1) and
fulvic-Fe(III) (0.1, 0.2 and 1 ppm C)] and solid amorphous hydrous ferric oxide [am-Fe(III) or Fe(III) hydroxide] were experimentally
measured in culture experiments at 10 °C under 3000 lux fluorescent light. Fulvic-Fe(III) (0.1 and 0.2 ppm C) and citric-Fe(III)
(100:1) induced maximal cell yields of C. sociale. The order of cell yields was: fulvic-Fe(III) (0.1 and 0.2 ppm C) ≥ citric-Fe(III) (100:1) > EDTA-Fe(III) (2:1) ≫ solid am-Fe(III) > EDTA-Fe(III)
(100:1) ≫ fulvic-Fe(III) (1 ppm C). The short-term iron uptake rates by C. sociale in fulvic-Fe(III) (0.1 and 0.2 ppm C) and citric-Fe(III) (100:1) media were about five to six times faster than those in
EDTA-Fe(III) (100:1) and solid am-Fe(III) media. The dissociative precipitation rates of premixed organic-Fe(III) complexes
in seawater at 10 °C were determined by simple filtration (0.025 μm) involving γ-activity measurements of 59Fe. The order of estimated initial Fe(III) dissociative precipitation rates of these organic-Fe(III) complexes in seawater
were nearly consistent with those of cell yields in the culture experiments and short-term iron uptake rates by C. sociale [except for fulvic-Fe(III) (1 ppm C) medium]. In fulvic-Fe(III) (0.1 and 0.2 ppm C), citric-Fe(III) (100:1) and EDTA-Fe(III)
(2:1) media, the concentrations of dissolved organic-Fe(III) complexes in initial culture experiments are prone to supersaturate
under the culture conditions. The supersaturated dissolved organic-Fe(III) complex in seawater supplies biologically available
inorganic Fe(III) species in culture media through its dissociation at high pH and high levels of seawater cations. Therefore,
the natural dissolved organic-Fe(III) complexes supplied by riverine input may play an important role in supplying bioavailable
iron in estuarine mixing system and coastal waters.
Received: 6 September 1998 / Accepted: 8 April 1999 相似文献
172.
Tsunamis and storm surges have killed more than one million people and some three billion people currently live with a high risk of these disasters, which are becoming more frequent and devastating worldwide. Effective mitigation of such disasters is possible via healthy coastal forests, which can reduce the energy of tsunamis. In recent years, these natural barriers have declined due to adverse human and natural activities. In the past 20 years, the world has lost almost 50 per cent of its mangrove forests, making them one of the most endangered landscapes. It is essential to recover them and to use them as a shield against a tsunami and as a resource to secure optimal socio-economic, ecological and environmental benefits. This paper examines the emerging scenario facing mangrove forests, discusses protection from tsunamis, and proposes a way to improve the current situation. We hope that practical tips will help communities and agencies to work collectively to achieve a common goal. 相似文献
173.
Nigussie Haregeweyn Atsushi Tsunekawa Mitsuru Tsubo Derege Meshesha Enew Adgo Jean Poesen Brigitta Schütt 《Regional Environmental Change》2016,16(4):951-966
In the drylands of the Upper Blue Nile basin, high climate variability and land degradation are rampant. To enhance adaptive capacity in the region, various soil and water conservation interventions have been implemented. Moreover, water resources development schemes such as the Grand Ethiopian Renaissance Dam should be implemented by 2025. We modeled the effects of these interventions on surface runoff in the basin for both current and future (2025) basin conditions, using the runoff coefficient method in a spatially explicit approach. Under current conditions, we observed high spatial variability of mean annual runoff. The northeastern Blue Nile-1 sub-basin produces the highest mean annual runoff (391 mm or 10 × 109 m3), whereas the northwestern Blue Nile-2 sub-basin produces the lowest mean annual runoff (178 mm or 0.2 × 109 m3). The basin generates a total annual runoff volume of 47.7 × 109 m3, of which about 54 % comes from cultivated land. The strong association between land use and topography masked the direct effect of rainfall on runoff. By 2025, total annual runoff yield could decrease by up to 38 % if appropriate basin-wide soil and water conservation interventions and the Grand Ethiopian Renaissance Dam are implemented. However, the full effects of most physical structures will only last for 1 or 2 years without regular maintenance. The improved understanding of the dynamics of the Upper Blue Nile basin’s hydrology provided by the present study will help planners to design appropriate management scenarios. Developing the basin’s database remains important for a holistic understanding of the impacts of future development interventions. 相似文献
174.
We developed a novel polymer type sulfoxide-modified solid phase enabling to achieve selective separation of polychlorinated biphenyls (PCBs) from insulation oil. In this study, firstly we prepared base-polymer based on the concept of the molecular imprinting to capture PCBs in selectively, then, the sulfoxide groups were modified on the pore surface of base-polymers by changing preparation methods. As results of liquid chromatographic analyses for the polymers as columns, the base-polymer prepared by xylene as a porogenic solvent showed selective retention ability for chlorinated aromatic compounds by the porogen imprinting effect. Additionally, the polymer-type sulfoxide solid phases showed highly retention ability for PCBs by increasing amount of introduced sulfoxide groups. Consequently, the results of separation of PCBs comparing to insulation oil suggested that the prepared solid phase can be used for the selective separation of PCBs at the same level as a commercially available media utilized for the regulated method. 相似文献
175.
TiO2 powder-containing paper composites, called TiO2 paper, were prepared by a papermaking technique, and their photocatalytic efficiency was investigated. The TiO2 paper has a porous structure originating from the layered pulp fiber network, with TiO2 powders scattered on the fiber matrix. Under UV irradiation, the TiO2 paper decomposed gaseous acetaldehyde more effectively than powdery TiO2 and a pulp/TiO2 mixture not in paper form. Scanning electron microscopy and mercury intrusion analysis revealed that the TiO2 paper had characteristic unique voids ca. 10 μm in diameter, which might have contributed to the improved photocatalytic performance. TiO2 paper composites having different void structures were prepared by using beaten pulp fibers with different degrees of freeness and/or ceramic fibers. The photodecomposition efficiency was affected by the void structure of the photocatalyst paper, and the initial degradation rate of acetaldehyde increased with an increase in the total pore volume of TiO2 paper. The paper voids presumably provided suitable conditions for TiO2 catalysis, resulting in higher photocatalytic performance by TiO2 paper than by TiO2 powder and a pulp/TiO2 mixture not in paper form. 相似文献
176.
Perfluorooctanesulfonate and perfluorooctanoate in raw and treated tap water from Osaka, Japan 总被引:7,自引:0,他引:7
Takagi S Adachi F Miyano K Koizumi Y Tanaka H Mimura M Watanabe I Tanabe S Kannan K 《Chemosphere》2008,72(10):1409-1412
Perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA) have been recognized as emerging environmental pollutants because of their ubiquitous occurrence in the environment, biota, and humans. PFOS and PFOA have been detected in water in Japan. Nevertheless, occurrence of PFOS and PFOA in potable water from municipal water treatment plants is not clearly known. We analyzed PFOS and PFOA in raw and tap water samples collected from 14 drinking water treatment plants in winter and summer seasons in Osaka to determine the concentrations of PFOS and PFOA in raw and potable tap water samples. PFOS and PFOA were detected in all raw water samples. Concentration ranges of PFOS and PFOA in raw water were 0.26-22 ng/l and 5.2-92 ng/l, respectively. Whereas the concentrations PFOS in raw water from Osaka were similar to those in other areas in Japan, the concentrations of PFOA were higher than in other areas. Concentration ranges of PFOS and PFOA in potable tap water were 0.16-22 ng/l and 2.3-84 ng/l, respectively. There were positive correlations between PFC concentrations in raw water and tap water samples. Therefore, the removal efficiency of PFCs by the present water treatment may be low. Based on the current action value reported by U.S. Environmental Protection Agency, PFOA concentrations found in tap water in Osaka is not expected to pose health risks. 相似文献
177.
Distribution of pesticides and bisphenol A in sediments collected from rivers adjacent to coral reefs 总被引:1,自引:0,他引:1
To investigate the deteriorating health of coral reefs in Okinawa, Japan, natural sediment samples were analyzed for diuron, Irgarol 1051, chlorpyrifos, and bisphenol A (BPA) which are hazardous to corals. Samples were analyzed by solid-phase extraction (SPE) followed by high-performance liquid chromatography with tandem mass spectrometry (LC–MS–MS). Although diuron and chlorpyrifos usage is only well recorded for farms and not for cities, these chemicals were detected in both rural and urban areas. Additionally, diuron concentration in urban areas was in some cases higher than in rural areas, which might be caused by greater consumption of these chemicals in home gardens in city areas. Irgarol 1051 was detected in downstream river areas, which are situated far from the source sites such as pier or fishery harbor (0.6–3.2 km). This result suggested that Irgarol 1051 could be transported from the river mouths to the sampling sites during flood tides. High BPA concentrations were associated with urban areas (<1.2–22.0 μg kg−1), while low concentrations were associated with rural areas (nd–6.8 μg kg−1). The river sediments under study are delivered to coral reefs in large quantity through runoff caused by typhoons and other heavy rains. The highly hazardous chemicals are carried into coral reefs on these sediments. Therefore, these hazardous chemical substances may already be influencing the coral reefs. 相似文献
178.
Kuzuhara Shunsuke Akimoto Yuta Shibata Kazu Oguchi Masahiro Terazono Atsushi 《Journal of Material Cycles and Waste Management》2018,20(1):431-438
Journal of Material Cycles and Waste Management - Our objective was to provide the information necessary to efficiently recover metals from end-of-life lithium-ion secondary batteries by assessing... 相似文献
179.
Stef Bokhorst Stine Højlund Pedersen Ludovic Brucker Oleg Anisimov Jarle W. Bjerke Ross D. Brown Dorothee Ehrich Richard L. H. Essery Achim Heilig Susanne Ingvander Cecilia Johansson Margareta Johansson Ingibjörg Svala Jónsdóttir Niila Inga Kari Luojus Giovanni Macelloni Heather Mariash Donald McLennan Gunhild Ninis Rosqvist Atsushi Sato Hannele Savela Martin Schneebeli Aleksandr Sokolov Sergey A. Sokratov Silvia Terzago Dagrun Vikhamar-Schuler Scott Williamson Yubao Qiu Terry V. Callaghan 《Ambio》2016,45(5):516-537
180.
Sonoko Dorothea Bellingrath-Kimura Ayaka Wenhong Kishimoto-Mo Noriko Oura Seiko Sekikawa Seichiro Yonemura Shigeto Sudo Atsushi Hayakawa Kazunori Minamikawa Yusuke Takata Hiroshi Hara 《Ambio》2015,44(1):55-66
The spatial variability of carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O) fluxes from forest soil with high nitrogen (N) deposition was investigated at a rolling hill region in Japan. Gas fluxes were measured on July 25th and December 5th, 2008 at 100 points within a 100 × 100 m grid. Slope direction and position influenced soil characteristics and site-specific emissions were found. The CO2 flux showed no topological difference in July, but was significantly lower in December for north-slope with coniferous trees. Spatial dependency of CH4 fluxes was stronger than that of CO2 or N2O and showed a significantly higher uptake in hill top, and emissions in the valley indicating strong influence of water status. N2O fluxes showed no spatial dependency and exhibited high hot spots at different topology in July and December. The high N deposition led to high N2O fluxes and emphasized the spatial variability. 相似文献