全文获取类型
收费全文 | 16643篇 |
免费 | 148篇 |
国内免费 | 109篇 |
专业分类
安全科学 | 441篇 |
废物处理 | 672篇 |
环保管理 | 1978篇 |
综合类 | 2870篇 |
基础理论 | 4294篇 |
环境理论 | 11篇 |
污染及防治 | 4529篇 |
评价与监测 | 1114篇 |
社会与环境 | 889篇 |
灾害及防治 | 102篇 |
出版年
2023年 | 110篇 |
2022年 | 226篇 |
2021年 | 237篇 |
2020年 | 149篇 |
2019年 | 168篇 |
2018年 | 338篇 |
2017年 | 336篇 |
2016年 | 471篇 |
2015年 | 360篇 |
2014年 | 521篇 |
2013年 | 1255篇 |
2012年 | 636篇 |
2011年 | 815篇 |
2010年 | 614篇 |
2009年 | 655篇 |
2008年 | 816篇 |
2007年 | 785篇 |
2006年 | 673篇 |
2005年 | 593篇 |
2004年 | 508篇 |
2003年 | 501篇 |
2002年 | 458篇 |
2001年 | 538篇 |
2000年 | 376篇 |
1999年 | 250篇 |
1998年 | 156篇 |
1997年 | 177篇 |
1996年 | 178篇 |
1995年 | 217篇 |
1994年 | 220篇 |
1993年 | 168篇 |
1992年 | 150篇 |
1991年 | 187篇 |
1990年 | 180篇 |
1989年 | 169篇 |
1988年 | 126篇 |
1987年 | 122篇 |
1986年 | 137篇 |
1985年 | 103篇 |
1984年 | 120篇 |
1983年 | 120篇 |
1982年 | 131篇 |
1981年 | 116篇 |
1980年 | 106篇 |
1979年 | 117篇 |
1978年 | 79篇 |
1977年 | 80篇 |
1975年 | 83篇 |
1973年 | 76篇 |
1972年 | 73篇 |
排序方式: 共有10000条查询结果,搜索用时 15 毫秒
941.
John E. Hobbie Gaius R. Shaver Edward B. Rastetter Jessica E. Cherry Scott J. Goetz Kevin C. Guay William A. Gould George W. Kling 《Ambio》2017,46(1):160-173
Long-term measurements of ecological effects of warming are often not statistically significant because of annual variability or signal noise. These are reduced in indicators that filter or reduce the noise around the signal and allow effects of climate warming to emerge. In this way, certain indicators act as medium pass filters integrating the signal over years-to-decades. In the Alaskan Arctic, the 25-year record of warming of air temperature revealed no significant trend, yet environmental and ecological changes prove that warming is affecting the ecosystem. The useful indicators are deep permafrost temperatures, vegetation and shrub biomass, satellite measures of canopy reflectance (NDVI), and chemical measures of soil weathering. In contrast, the 18-year record in the Greenland Arctic revealed an extremely high summer air-warming of 1.3 °C/decade; the cover of some plant species increased while the cover of others decreased. Useful indicators of change are NDVI and the active layer thickness. 相似文献
942.
Niels M. Schmidt Bess Hardwick Olivier Gilg Toke T. Høye Paul Henning Krogh Hans Meltofte Anders Michelsen Jesper B. Mosbacher Katrine Raundrup Jeroen Reneerkens Lærke Stewart Helena Wirta Tomas Roslin 《Ambio》2017,46(1):12-25
How species interact modulate their dynamics, their response to environmental change, and ultimately the functioning and stability of entire communities. Work conducted at Zackenberg, Northeast Greenland, has changed our view on how networks of arctic biotic interactions are structured, how they vary in time, and how they are changing with current environmental change: firstly, the high arctic interaction webs are much more complex than previously envisaged, and with a structure mainly dictated by its arthropod component. Secondly, the dynamics of species within these webs reflect changes in environmental conditions. Thirdly, biotic interactions within a trophic level may affect other trophic levels, in some cases ultimately affecting land–atmosphere feedbacks. Finally, differential responses to environmental change may decouple interacting species. These insights form Zackenberg emphasize that the combination of long-term, ecosystem-based monitoring, and targeted research projects offers the most fruitful basis for understanding and predicting the future of arctic ecosystems. 相似文献
943.
Magnus Lund Katrine Raundrup Andreas Westergaard-Nielsen Efrén López-Blanco Josephine Nymand Peter Aastrup 《Ambio》2017,46(1):26-38
Insect outbreaks can have important consequences for tundra ecosystems. In this study, we synthesise available information on outbreaks of larvae of the noctuid moth Eurois occulta in Greenland. Based on an extensive dataset from a monitoring programme in Kobbefjord, West Greenland, we demonstrate effects of a larval outbreak in 2011 on vegetation productivity and CO2 exchange. We estimate a decreased carbon (C) sink strength in the order of 118–143 g C m?2, corresponding to 1210–1470 tonnes C at the Kobbefjord catchment scale. The decreased C sink was, however, counteracted the following years by increased primary production, probably facilitated by the larval outbreak increasing nutrient turnover rates. Furthermore, we demonstrate for the first time in tundra ecosystems, the potential for using remote sensing to detect and map insect outbreak events. 相似文献
944.
In the present context of global change and search for sustainability, we detected a gap between restoration and society: local communities are usually only considered as threats or disturbances when planning for restoration. To bridge this gap, we propose a landscape design framework for planning riparian rehabilitation in an urban–rural gradient. A spatial multi-criteria analysis was used to assess the priority of riversides by considering two rehabilitation objectives simultaneously—socio-environmental and ecological—and two sets of criteria were designed according to these objectives. The assessment made it possible to identify 17 priority sites for riparian rehabilitation that were associated with different conditions along the gradient. The double goal setting enabled a dual consideration of citizens, both as beneficiaries and potential impacts to rehabilitation, and the criteria selected incorporated the multi-dimensional nature of the environment. This approach can potentially be adapted and implemented in any other anthropic–natural interface throughout the world. 相似文献
945.
Jeanne Clécia Alves Esther Lima de Paiva Raquel Fernanda Milani Eduardo Bearzoti Marcelo Antonio Morgano 《Journal of environmental science and health. Part. B》2017,52(6):418-424
Although fish is a healthy alternative for meat, it can be a vehicle for mercury (Hg), including in its most toxic organic form, methylmercury (MeHg). The objective of the present study was to estimate the risk to human health caused by the consumption of sushi and sashimi as commercialized by Japanese food restaurants in the city of Campinas (SP, Brazil). The total Hg content was determined by atomic absorption spectrometry with thermal decomposition and amalgamation, and the MeHg content calculated considering that 90% of the total Hg is in the organic form. The health risk was estimated from the values for the provisional tolerable weekly ingestion (PTWI) by both adults and children. The mean concentrations for total Hg were: 147.99, 6.13, and 3.42 µg kg?1 in the tuna, kani, and salmon sushi samples, respectively, and 589.09, 85.09, and 11.38 µg kg?1 in the tuna, octopus and salmon sashimi samples, respectively. The tuna samples showed the highest Hg concentrations. One portion of tuna sashimi exceeded the PTWI value for MeHg established for children and adults. The estimate of risk for human health indicated that the level of toxicity depended on the type of fish and size of the portion consumed. 相似文献
946.
Alessandra A. Z. Rodrigues André Fernando De Oliveira Antônio Augusto Neves Fernanda F. Heleno Laércio Zambolim 《Journal of environmental science and health. Part. B》2017,52(12):850-857
This study was undertaken to evaluate the effectiveness of several household practices (washing with water or acidic, alkaline, and oxidizing solutions, and peeling) in minimizing pesticide residue contamination of tomatoes, as well as the impact on the quality of the treated fruit. Tests were performed using two systemic fungicides (azoxystrobin and difenoconazole) and one contact fungicide (chlorothalonil). Solid-liquid extraction with low temperature partition (SLE/LTP) and liquid-liquid extraction with low temperature partition (LLE/LTP) were used to prepare the samples for pesticides determination by gas chromatography. Washing the tomatoes with water removed approximately 44% of chlorothalonil, 26% of difenoconazole, and 17% of azoxystrobin. Sodium bicarbonate (5%) and acetic acid (5%) solutions were more efficient, removing between 32 and 83% of the residues, while peeling removed from 68 to 88% of the pesticides. The washing solutions altered some fruit quality parameters, including acidity and chroma, and also caused weight loss. Acetic acid (0.15 and 5%) and hypochlorite (1%) solutions had the greatest effect on these parameters. 相似文献
947.
Daniela Iannazzo Alessandro Pistone Ida Ziccarelli Claudia Espro Signorino Galvagno Salvatore V Giofré Roberto Romeo Nicola Cicero Giuseppe D Bua Giuseppe Lanza Laura Legnani Maria A Chiacchio 《Environmental science and pollution research international》2017,24(17):14735-14747
Dendrimer-functionalized multi-walled carbon nanotubes (MWCNT) for heavy metal ion removal from wastewaters were developed. Triazole dendrimers (TD) were built directly onto the carbon nanotube surface by successive click chemistry reactions affording the zero- and first-generation dendrimer-functionalized MWCNT (MWCNT-TD1 and MWCNT-TD2). The Moedritzer-Irani reaction carried out on the amino groups present on the MWCNT-TD2 sample gave the corresponding α-aminophosphonate nanosystem MWCNT-TD2P. Both MWCNT-TD2 and MWCNT-TD2P nanosystems have been characterized by physical, chemical, and morphological analyses. Their chelating abilities towards the toxic metal ions Pb2+, Hg2+, and Ni2+ and the harmless Ca2+ ion have been experimentally evaluated in the two different sets of experiments and at the salt concentrations of 1 mg/mL or 1 μg/mL by inductively coupled plasma mass spectrometry (ICP-MS). The results of these studies pointed out the interesting chelating behavior for the phosphonated nanosystem towards the Hg2+ ion. The complexation mode of the best chelating system MWCNT-TD2P with mercury was investigated through density functional theory (DFT) calculations, suggesting a chelation mechanism involving the two oxygen atoms of the phosphate group. The synthesized dendrimers, supported on the multi-walled carbon nanotubes, have shown the potential to be used for the selective toxic metal ion removal and recovery. 相似文献
948.
Suéllen Satyro Enrico Mendes Saggioro Fábio Veríssimo Daniel Forsin Buss Danielly de Paiva Magalhães Anabela Oliveira 《Environmental science and pollution research international》2017,24(19):16077-16085
Triclocarban (TCC) is an antibacterial agent found in pharmaceuticals and personal care products (PPCP). It is potentially bioaccumulative and an endocrine disruptor, being classified as a contaminant of emerging concern (CEC). In normal uses, approximately 96% of the used TCC can be washed down the drain going into the sewer system and eventually enter in the aquatic environment. UV photolysis can be used to photodegrade TCC and ecotoxicity assays could indicate the photodegradation efficiency, since the enormous structural diversity of photoproducts and their low concentrations do not always allow to identify and quantify them. In this work, the TCC was efficiently degraded by UVC direct photolysis and the ecotoxicity of the UV-treated mixtures was investigated. Bioassays indicates that Daphnia similis (48 h EC50 = 0.044 μM) was more sensitive to TCC than Pseudokirchneriella subcapitata (72 h IC50 = 1.01 μM). TCC and its photoproducts caused significant effects on Eisenia andrei biochemical responses (catalase and glutathione-S-transferase); 48 h was a critical exposure time, since GST reached the highest activity values. UVC reduced the TCC toxic effect after 120 min. Furthermore, TCC was photodegraded in domestic wastewater which was simultaneously disinfected for total coliform bacterial (TCB) (360 min) and Escherichia coli (60 min). 相似文献
949.
Félix Schmitt Khac-Uan Do 《Environmental science and pollution research international》2017,24(29):22885-22913
Membrane fouling is a major concern for the optimization of membrane bioreactor (MBR) technologies. Numerous studies have been led in the field of membrane fouling control in order to assess with precision the fouling mechanisms which affect membrane resistance to filtration, such as the wastewater characteristics, the mixed liquor constituents, or the operational conditions, for example. Worldwide applications of MBRs in wastewater treatment plants treating all kinds of influents require new methods to predict membrane fouling and thus optimize operating MBRs. That is why new models capable of simulating membrane fouling phenomenon were progressively developed, using mainly a mathematical or numerical approach. Faced with the limits of such models, artificial neural networks (ANNs) were progressively considered to predict membrane fouling in MBRs and showed great potential. This review summarizes fouling control methods used in MBRs and models built in order to predict membrane fouling. A critical study of the application of ANNs in the prediction of membrane fouling in MBRs was carried out with the aim of presenting the bottlenecks associated with this method and the possibilities for further investigation on the subject. 相似文献
950.
Design of water quality monitoring networks with two information scenarios in tropical Andean basins
Juan Carlos Bastidas Jorge Julián Vélez Jeannette Zambrano Adela Londoño 《Environmental science and pollution research international》2017,24(25):20134-20148
Design and redesign of water quality monitoring networks were evaluated for two similarly sized watersheds in the tropical Andes via optimization techniques using geographic information system technology (GIS) and a matter-element analysis of 5-day biological oxygen demand (BOD5) and total suspended solids (TSS). This resulted in a flexible, objectively based design for a 1128-km2 watershed without prior water quality data (La Miel River), and a network redesign of a 1052-km2 watershed with historical water quality monitoring (Chinchiná River). Monitoring design for the undocumented basin incorporated mathematical expressions for physical, anthropological, and historical factors—and was based on clear objectives for diagnosis and intervention of water pollution. Network redesign identified network redundancy, which resulted in a 64% reduction in the number of water quality monitoring stations along the channel, and a 78% reduction of stations throughout the basin. Most tropical drainage basins throughout the world have little to no prior water quality data. But even in well-studied drainage basins like the Chinchiná River, which is among the most thoroughly studied basins in Colombia, redesign of historical and existing monitoring networks will become a standard tool to advance the restoration of polluted surface waters, not only in Colombia, but also throughout the world. 相似文献