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41.
Thomas J. Fredette Joseph D. Germano Drew A. Carey Peggy M. Murray Paula G. Kullberg 《Chemistry and Ecology》2013,29(1-4):173-194
Geochemical analysis and visual inspection of cores collected from capped dredged material mounds revealed that in many cores, cap material was clearly distinguishable, both visually and chemically, from mound material. Contaminated dredged sediments were disposed in Long Island Sound eleven and seven years prior to sampling, and capped with uncontaminated dredged sediments. Core data provided no conclusive evidence of physical disturbance of, or chemical migration from, the contaminated mound sediments. Obvious chemical gradients of contaminant concentrations, which we propose are indicators of chemical migration, were not detected in the cores. Heterogeneity of the cap and mound sediments in some cores made the interface less distinct. We postulate that the preservation of spatial variability of sediment texture and associated contaminants observed within dredged material mounds is a result of the dredging process. Preservation of the textural and contaminant history of dredged sediments within finegrained cohesive cap materials provides evidence of the absence of physical or chemical disturbance. 相似文献
42.
Contribution of Wastewater Treatment Plant Effluents to Nutrient Dynamics in Aquatic Systems: A Review 总被引:1,自引:0,他引:1
Excessive nutrient loading (considering nitrogen and phosphorus) is a major ongoing threat to water quality and here we review
the impact of nutrient discharges from wastewater treatment plants (WWTPs) to United States (U.S.) freshwater systems. While
urban and agricultural land uses are significant nonpoint nutrient contributors, effluent from point sources such as WWTPs
can overwhelm receiving waters, effectively dominating hydrological characteristics and regulating instream nutrient processes.
Population growth, increased wastewater volumes, and sustainability of critical water resources have all been key factors
influencing the extent of wastewater treatment. Reducing nutrient concentrations in wastewater is an important aspect of water
quality management because excessive nutrient concentrations often prevent water bodies from meeting designated uses. WWTPs
employ numerous physical, chemical, and biological methods to improve effluent water quality but nutrient removal requires
advanced treatment and infrastructure that may be economically prohibitive. Therefore, effluent nutrient concentrations vary
depending on the particular processes used to treat influent wastewater. Increasingly stringent regulations regarding nutrient
concentrations in discharged effluent, along with greater freshwater demand in populous areas, have led to the development
of extensive water recycling programs within many U.S. regions. Reuse programs provide an opportunity to reduce or eliminate
direct nutrient discharges to receiving waters while allowing for the beneficial use of reclaimed water. However, nutrients
in reclaimed water can still be a concern for reuse applications, such as agricultural and landscape irrigation. 相似文献
43.
Given the relatively rapid rate of dense nonaqueous‐phase liquid (DNAPL) ganglia depletion, source zones are generally dominated by horizontal layers of DNAPL after a release to the saturated zone. Estimating the time required to attain specific source strength reduction targets resulting from partial DNAPL source depletion is challenging due to a lack of available screening models, and because little has been done to synthesize available empirical data. Analytical and semi‐analytical models are used to study general DNAPL pool dissolution dynamics. The half‐life for the decline in DNAPL source strength (i.e., aqueous mass discharge) is demonstrated as proportional to the square root of the pool length, the thickness of the pool, and the solubility for single component DNAPLs. The through‐pool discharge is shown to be potentially significant for thin pools or in upper regions of thicker pools. An empirical analysis is used to evaluate average concentration decline rates for 13 in situ chemical oxidation (ISCO) and 16 enhanced in situ bioremediation (EISB) sites. Mean apparent decline rates, based on the time required to achieve the observed source strength reduction, are calculated for the ISCO and EISB sites (half‐lives of 0.39 year and 0.29 year, respectively). The empirical study sites are shown to have faster decline rates than for a large, complex study site where ISCO was implemented (half‐life of 2.5 years), and for a conceptual pool‐dominated trichloroethene source zone where EISB was simulated (half‐life of 2.5 years). Guidance is provided on using these findings in estimating timeframes for partial DNAPL depletion goals. © 2014 Wiley Periodicals, Inc. 相似文献
44.
Henry H. Carey 《Environmental management》1983,7(2):161-170
Harvest calculations determine sawtimber flows from public lands and are closely scruntinized by a wide spectrum of forest users. This study examines the reliability of harvest calculations on a single national forest in New Mexico Forest Service determinations of an array of variables were reviewed and evaluated. The study revealed a lack of precision in Forest Service adherence to self-imposed procedural standards governing the calculation process. Timber sales have taken place on lands where such standards prohibit harvesting and these lands have been included in annual harvest calculations. Assumptions required by a mathematical model used by the Forest Service in calculating the harvest were not followed in the subsequent implementation of the harvest level. These factors suggest that the Forest Service could have significantly over-stated annual harvest rate for the first decade. Opportunities exist to improve the calculation, and benefits realized may greatly exceed additional costs of implementation 相似文献
45.
应用Models-3/CMAQ研究长三角区域大气污染及输送 总被引:3,自引:0,他引:3
选用美国国家环保局第3代空气质量模式(Models-3,/CMAQ),配合中尺度气象模式(MM5)进行研究,模拟了2001年1、7月份长江三角洲区域冬夏季典型天气条件下大气层二次污染物臭氧及颗粒物的浓度分布及输送状况。采用2001年冬.夏季各10d的小时监测数据对模式验证。结果表明,Models-3/CMAQ对O3、PM10的模拟相关系数分别为0.77和052;一致性指数分别达到081和0.99。模型对于O3略微低估,标准偏差为-31%,而对于PM10则有所高估,标准偏差为46%。对长三角7月份O3浓度及1月份PM10的模拟结果显示,7月份长三角区域16个主要城市O3日均浓度集中在0.043~0.086mg/m^3之间,其中,泰州、扬州.湖州、镇江O3月日均浓度相对较高,均超过0.064mg/m3o模拟时段内O3最高小时浓度达0.276mg/m^3。1月份整个模拟区域PM10月日均浓度为O056mg/m^3,其中,南京市PM10日均浓度最高,达0.080mg/m^3模拟时段内PM10最高小时浓度达0.432mg/m^3研究表明,长三角地区存在明显的污染物输送现象,大气污染已经从局地污染转化为区域污染。 相似文献
46.
长江三角洲地区大气O3和PM10的区域污染特征模拟 总被引:6,自引:1,他引:5
以TRACE-P污染源资料及上海市地方排放清单为基础,采用Models-3/CMAQ环境空气质量模型和中尺度气象模式MM5,模拟研究了2001-01和2001-07长三角近地面二次污染物O3及PM 10的浓度分布及输送状况,并以上海市国控点2001年冬、夏季各10 d的小时监测数据对模型进行了验证.验证结果显示,Models-3/CMAQ对O3和PM10的模拟结果与监测值的相关系数分别为0.77和0.52;一致性指数分别达到0.81和0.99.模型对O3小时最高浓度的估算偏低27%,标准偏差为-3.1%;对PM10小时平均浓度的估算偏低10%,标准偏差为46%.模型已具备再现和模拟长三角大气污染输送过程的能力,且误差落在可接受的范围之内.模拟结果显示,2001-07长三角区域16个主要城市中,有14个城市O3小时最大浓度超过国家二级标准,高浓度O3可覆盖苏南和浙北广大区域.2001-01泰州、扬州、南京、镇江、常州等城市受本地排放源和北部大气污染输送的影响显著,大气PM10日均浓度超过PM10国家二级标准.长三角地区环境空气质量与污染类型受大气污染传输与化学转化的影响十分明显.夏季太阳辐射较强时,南部城市排放的污染物常以二次污染物的形式影响下风向城市;太阳辐射较弱的情况下,则以一次污染物输送为主的形式影响周边地区.冬季长三角区域颗粒物污染总体水平较高,这与我国北方地区排放的颗粒物在西北风作用下向长三角输送造成的影响密切相关.长三角地区的大气污染已逐渐从局地转为区域问题. 相似文献
47.
Hypothesis Concerning the Causes of the Disappearance of Boreal Toads from the Mountains of Colorado 总被引:1,自引:0,他引:1
Cynthia Carey 《Conservation biology》1993,7(2):355-362
Recent reports of world-wide declines and extinctions of amphibian populations have raised questions about the relation of environmental change to the demise of certain amphibian species. Between 1974 and 1982, 11 populations of boreal toads ( Bufo boreas boreas ) in the West Elk Mountains of Colorado totally disappeared. The apparent cause of extinction of these toads was infection with the bacteria Aeromonas hydrophila . In this paper, the presence of disease in declining populations of these toads is used in conjunction with a variety of data from the literature to formulate a working hypothesis for explaining the cause of the decline of this species, and perhaps others:
48.
Litao Wang Carey Jang Yang Zhang Kai Wang Qiang Zhang David Streets Joshua Fu Yu Lei Jeremy Schreifels Kebin He Jiming Hao Yun-Fat Lam Jerry Lin Nicholas Meskhidze Scott Voorhees Dale Evarts Sharon Phillips 《Atmospheric environment (Oxford, England : 1994)》2010,44(28):3442-3448
Under the 11th Five Year Plan (FYP, 2006–2010) for national environmental protection by the Chinese government, the overarching goal for sulfur dioxide (SO2) controls is to achieve a total national emissions level of SO2 in 2010 10% lower than the level in 2005. A similar nitrogen oxides (NOx) emissions control plan is currently under development and could be enforced during the 12th FYP (2011–2015). In this study, the U.S. Environmental Protection Agency (U.S.EPA)’s Community Multi-Scale Air Quality (Models-3/CMAQ) modeling system was applied to assess the air quality improvement that would result from the targeted SO2 and NOx emission controls in China. Four emission scenarios — the base year 2005, the 2010 Business-As-Usual (BAU) scenario, the 2010 SO2 control scenario, and the 2010 NOx control scenario—were constructed and simulated to assess the air quality change from the national control plan. The Fifth-Generation NCAR/Penn State Mesoscale Model (MM5) was applied to generate the meteorological fields for the CMAQ simulations. In this Part I paper, the model performance for the simulated meteorology was evaluated against observations for the base case in terms of temperature, wind speed, wind direction, and precipitation. It is shown that MM5 model gives an overall good performance for these meteorological variables. The generated meteorological fields are acceptable for using in the CMAQ modeling. 相似文献
49.
Peter J. Gunning Colin D. Hills Paula J. Carey 《Waste management (New York, N.Y.)》2010,30(6):1081-1090
The disposal of industrial waste presents major logistical, financial and environmental issues. Technologies that can reduce the hazardous properties of wastes are urgently required. In the present work, a number of industrial wastes arising from the cement, metallurgical, paper, waste disposal and energy industries were treated with accelerated carbonation. In this process carbonation was effected by exposing the waste to pure carbon dioxide gas. The paper and cement wastes chemically combined with up to 25% by weight of gas. The reactivity of the wastes to carbon dioxide was controlled by their constituent minerals, and not by their elemental composition, as previously postulated. Similarly, microstructural alteration upon carbonation was primarily influenced by mineralogy. Many of the thermal wastes tested were classified as hazardous, based upon regulated metal content and pH. Treatment by accelerated carbonation reduced the leaching of certain metals, aiding the disposal of many as stable non-reactive wastes. Significant volumes of carbon dioxide were sequestrated into the accelerated carbonated treated wastes. 相似文献
50.
东莞是珠三角O_3污染最严重的城市,使用RSM/CMAQ(曲面响应模型)法分析了珠三角区域人为排放的NO_x和VOCs对东莞市O_3浓度变化源贡献.2014基准年分析结果表明,扣除模型域外区域传输及天然源排放对O_3本底浓度贡献(41.00%)后,东莞本地VOCs排放对O_3贡献最大(18.50%),珠三角区域NO_x减排率13%时可持续降低东莞市O_3浓度.进一步使用ABa CAS-SE(空气污染控制成本效益与达标评估系统)对2017、2020、2025东莞市3个未来年O_3污染控制情景进行了费效评估.评估结果显示,NO_x和VOCs控制比例相对较低的2017年控制情景人体健康效益/区域控制成本比约为1.1;而控制比例相对较高的2025年东莞O_3达标情景效益成本比仅为0.1.这说明,在高减排率情景下,以末端治理为主的控制措施经济可行性较差,需综合采取产业/能源结构调整、清洁生产等措施实现NO_x和VOCs的大比例减排,实现东莞O_3的稳定达标.今后将进一步研究NO_x和VOCs减排对PM_(2.5)环境浓度及健康效益影响,开展多目标污染物协同控制费效评估. 相似文献