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261.
Characterizing dissolved organic matter and evaluating associated nanofiltration membrane fouling 总被引:1,自引:0,他引:1
Natural organic matter (NOM) characteristics were determined for three ground waters exhibiting different water quality conditions. The water quality of the three feed waters collected at various water table depths was characterized by XAD-8/-4 resin adsorption, high performance size exclusion chromatography with ultraviolet and dissolved organic carbon (DOC) detections, and Fourier transform infrared spectroscopy (FTIR) to determine NOM fractionation, molecular weight, and NOM functional groups, respectively. Systematic studies were conducted to identify potential NOM foulants in ground water for nanofiltration (NF) membrane fouling. The results show that the hydrophobic fraction of NOM in all of the samples was significantly high (71-93%) compared to the hydrophilic (1.7-22.6%) and transphilic (5.3-6.6%) fractions. However, insignificant flux-decline (less than 5%) was observed for the highest DOC (36.9 mg l(-1)) and hydrophobic NOM (93%) containing groundwater compared to the other lesser DOC and hydrophobic NOM containing ground waters. This is presumably due to either higher fractions of hydrophilic and transphilic NOM or inorganic interactions that may be major foulants. Based on FTIR, aromatic foulants were observed at 1662 cm(-1) (CO-NH2 or CO conjugated with aromatic rings) for the fouled NF membrane with the relatively low DOC source waters. The contact angle of the clean membrane (52 degrees ) decreased with fouling up to 42-47 degrees for fouled membranes with the various samples. 相似文献
262.
This study strives to estimate the emission of dioxin and furthermore attempts to find the best technological control methods available for waste incinerators by investigating the emission status thereof. In order to incorporate the Stockholm Convention, a particular stringent law was promulgated in Korea and in recent years incinerators were forced to utilize better technological control. After the enforcement of special dioxin emission regulation in 2003, the average concentration of dioxin emitted from municipal and industrial waste incinerators decreased from 15.25 and 12.86 ng TEQ Nm(-3) to 5.53 and 4.96 ng TEQ Nm(-3) in 2001 and 2004, respectively. Based on test results at commercial plants, several best arranged sets of air pollution control devices (APCDs) were suggested in order to provide guidelines to help operators. These sets included combinations of spray dry absorbers, bag type filters, wet scrubbers, selective catalytic reductions and electrostatic precipitators. Different suggestions and real installations of APCD arrangement were investigated during the years around the regulation in effective. The results were presented depending on the capacity of the incinerators and different waste streams to observe the efforts to reduce dioxin emission by operators of incineration plants. The annual amount of dioxin emission from the incinerators is expected to be 212.5 g-TEQ in 2011 and 234.3g-TEQ in 2015, respectively, compared to 891.6g-TEQ recorded in 2001. The enforcement of new regulation and the installation of better APCDs showed the significant effect on such reduction. This reduction in dioxin emission from incinerators confirmed the nation's commitment to the regulatory requirement set by the Stockholm Convention. 相似文献
263.
In the Ag(II)/Ag(I) based mediated electrochemical oxidation (MEO) process, the spent waste from the electrochemical cell, which is integrated with the scrubber columns, contains high concentrations of precious silver as dissolved ions in both the anolyte and the catholyte. This work presents an electrochemical developmental study for the recovery of silver from simulated waste water from Ag(II)/Ag(I) based MEO process. Galvanostatic method of silver deposition on Ti cathode in an undivided cell was used, and the silver recovery rate kinetics of silver deposition was followed. Various experimental parameters, which have a direct bearing on the metal recovery efficiency, were optimized. These included studies with the nitric acid concentration (0.75-6M), the solution stirring rate (0-1400 rpm), the inter-electrode distance between the anode and the cathode (2-8 cm), the applied current density (29.4-88.2 mA cm(-2)), and the initial Ag(I) ion concentration (0.01-0.2M). The silver recovered by the present electrodeposition method was re-dissolved in 6M nitric acid and subjected to electrooxidation of Ag(I) to Ag(II) to ascertain its activity towards Ag(II) electrogeneration from Ag(I), which is a key factor for the efficient working of MEO process. Our studies showed that the silver metal recovered by the present electrochemical deposition method could be reused repeatedly for MEO process with no loss in its electrochemical activity. Some work on silver deposition from sulfuric acid solution of different concentrations was also done because of its promising features as the catholyte in the Ag(II) generating electrochemical cell used in MEO process, which include: (i) complete elimination of poisonous NO(x) gas liberation in the cathode compartment, (ii) reduced Ag(+) ion migration across Nafion membrane from anolyte to catholyte thereby diminished catholyte contamination, and (iii) lower cell voltage and hence lesser power consumption. 相似文献
264.
Chung KW Chandler AR Key PB 《Journal of environmental science and health. Part. B》2008,43(4):293-299
This study examined the toxicity of two pesticides (carbaryl and diquat dibromide) and one polycyclic aromatic hydrocarbon (fluoranthene), both singly and in mixture, to grass shrimp larvae (Palaemonetes pugio). These three chemicals are all present in coastal environments and can easily enter estuarine ecosystems. Fluoranthene was the most toxic chemical with a 96-h LC50 value of 32.45 microg/L, followed by carbaryl (43.02 microg/L) and diquat dibromide (1624 microg/L). In the chemical mixture tests, the binary carbaryl/diquat dibromide mixture and the ternary carbaryl/diquat dibromide/fluoranthene mixture had additive results. 相似文献
265.
Ke‐Sheng Cheng Hui‐Chung Yeh Ching‐Yuan Liou 《Journal of the American Water Resources Association》2000,36(3):511-521
ABSTRACT: Predicting the likelihood of a drought markedly enhances the efficiency of reservoir operations. This study applies the kriging method and time series analysis to predict inflows to Shihmen Reservoir in northern Taiwan. A subsequent reservoir operation simulation is employed to determine the drought lead time (DLT), the time before the onset of a drought. A more efficient reservoir operational strategy can be established with the aid of DLT and the probability of successful drought prediction (P s). Simulation results of reservoir operation over a period of three decades demonstrate that, at one month DLT, the kriging approach achieves 0.86 of P s for moderate droughts and 0.94 of P s for severe droughts. The kriging approach generally outperformed the time series approach in terms of DLT, P s of drought prediction, and the number of correctly predicted drought events. 相似文献
266.
Chung Yong-Seung Kim Hak-Sung Park Kie-Hyon Dulam Jugder Gao Tao 《Water, Air, & Soil Pollution: Focus》2005,5(3-6):15-35
A joint monitoring of dust-storms that occurred in East Asia from March until May 2003 has been carried. Our discussions include
dust-storm observations in the source areas of China and Mongolia, and measurements with satellites and ground monitors in
central Korea. Differences were found in the definition and measurement of dust-storms. Over the source area of Mongolia there
were 6 dusty days in March, 18 days in April, and 10 dusty days in May. In Inner Mongolia of northern China there were 4 dust-storms
with 14 dusty days observed over the three months. In central Korea, a sink area, there were 4 cases of weak dust-storm and
17 dusty days in the spring of 2003. The highest PM10 value was 607 μgm−3 and PM 2.3 was 149 μgm−3, respectively. These observations identify the growing need for further universal observation practices and dust-storm reporting
in future.
Observations indicated that snow covered the central part of the Gobi Desert, near the boundary of China and Mongolia, from
December until mid-March. This is in contrast to other years when the Gobi was relatively wet, producing unfavourable conditions
for the formation of intense dust-storms. In addition, the very strong winds associated with intense cyclones and anticyclones
were not apparent and the systems shifted northward during the spring. As a result, the frequency and intensity of observed
dust-storms in 2003 in this region were very low. This confirms that there is variability in the frequency of dust-storm formation
due to the current process of desertification and climate change. 相似文献
267.
Wu Qingli Chung Yong-Seung Zheng Yongguang Tao Zuyu 《Water, Air, & Soil Pollution: Focus》2003,3(2):81-92
To investigate the large-scale environmental conditions of duststorms occurring in Northern China, a synoptic situation of tendust events in Northern China during 2000–2001 was composed andits dynamic features were identified. The composite synoptic situation showed that the occurrence of the ten dust events was associated with the eastward movement of a strong cold high fromMongolia, and the development of a cyclone in Northeast China, which caused the pressure gradient to intensify considerably in Northern China. The upper level circulation revealed that a 500 hPa trough developed rapidly above Northern China, and diagnosis showed that composite ascending motion was pronouncedabove the Siberian district. The change of vertical motion in themiddle and low troposphere above Mongolia was also related to theoccurrence of the ten dust events. When the descendingcurrent, 12 hr before the occurrence, was completely replacedby the ascending current, the instable atmospheric stratificationof the lower troposphere enabled dry dust to be transported from the surface to high altitudes toward Northern China. 相似文献
268.
269.
270.
Chiou-Shuang Yan An-Min Chung Edward C Koziara Andrew G Verzilli 《Journal of Environmental Economics and Management》1975,2(1):60-68
The purpose of this study was to ascertain, through the use of an input-output model, the impact of air pollution control costs on income groups in the Philadelphia Region. The range of increases in consumption expenditure was found to be fairly narrow, with the middle-income group bearing the largest increase (2.9%) and the highest and lowest groups slightly lower increases (about 2%). This finding lends support to the proposition that all income groups would probably share the costs of control equally, which leads to a slightly regressive effect on income distribution. The sharing of the region's air quality costs by other areas was also analyzed. 相似文献