首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   95篇
  免费   2篇
  国内免费   4篇
安全科学   6篇
废物处理   2篇
环保管理   8篇
综合类   19篇
基础理论   22篇
污染及防治   35篇
评价与监测   6篇
社会与环境   3篇
  2022年   2篇
  2021年   2篇
  2018年   2篇
  2017年   1篇
  2016年   1篇
  2015年   1篇
  2014年   3篇
  2013年   5篇
  2012年   2篇
  2011年   2篇
  2010年   1篇
  2009年   1篇
  2008年   2篇
  2007年   8篇
  2006年   8篇
  2005年   6篇
  2004年   10篇
  2003年   2篇
  2002年   9篇
  2001年   1篇
  2000年   2篇
  1999年   2篇
  1998年   2篇
  1996年   2篇
  1995年   1篇
  1994年   2篇
  1993年   1篇
  1992年   1篇
  1988年   3篇
  1987年   1篇
  1984年   1篇
  1983年   3篇
  1982年   2篇
  1981年   1篇
  1978年   1篇
  1975年   2篇
  1973年   2篇
  1972年   1篇
  1969年   1篇
  1954年   1篇
排序方式: 共有101条查询结果,搜索用时 15 毫秒
21.
This research examines the degradation of atrazine by photocatalytic oxidation (PCO) under different experimental conditions. Deisopropylatrazine, deethylatrazine and deethyldeisopropylatrazine were formed as major intermediates based on gas chromatography-mass spectrometry. The reaction mixture was found to be toxic towards two bioassays, i.e. the Microtox and amphipods survival tests even when atrazine was completely degraded by PCO within 2 h under optimized conditions. The results indicate that adding H2O2 could significantly enhance the degradation of atrazine by PCO. Ammeline, ammelide and cyanuric acid (CA) became the major intermediates/products as detected by high performance liquid chromatography from 6th to the 40th h of PCO treatment. After 72 h PCO treatment, only CA was detectable in the reaction mixture. Further degradation of CA was carried out by a newly isolated CA-degrading bacterium, Sphingomonas capsulata. The photochemical pretreatment integrated with microbial degradation lead to the complete degradation and detoxification of atrazine.  相似文献   
22.
A membrane enhanced biological phosphorus removal (MEBPR) process was studied to determine the impact of hydraulic retention time (HRT) and solids retention time (SRT) on the removal of chemical oxygen demand (COD), nitrogen, and phosphorus from municipal wastewater. The MEBPR process was capable of delivering complete nitrification independent of the prevailing operating conditions, whereas a significant improvement in COD removal efficiency was observed at longer SRTs. In the absence of carbon-limiting conditions, the MEBPR process was able to achieve low phosphorus concentrations in the effluent at increasingly higher hydraulic loads, with the lowest HRT being 5 hours. The MEBPR process was also able to maintain optimal phosphorus removal when the SRT was increased from 12 to 20 days. However, at higher suspended solids concentrations, a substantial increase was observed in carbon utilization per unit mass of phosphorus removed from the influent. These results offer critical insights to the application of membrane technology for biological nutrient removal systems.  相似文献   
23.
Wang XL  Tao S  Dawson RW  Wang XJ 《Chemosphere》2004,55(4):525-531
A Monte Carlo simulation for uncertainty analysis of three key parameters (local coal consumption rate Q(1L), dry deposition velocity of aerosol particulate Kp and biodegradation rate of benzo(a)pyrene in soil and sediment K(R3)) was conducted in this study. Results of the simulation indicate that the three parameters were influenced by uncertainty and that all equilibrium concentrations in the four bulk compartments and various sub-compartments were log-normally distributed. However, the results also indicated that among the six primary transfer fluxes, erosion associated with solids in soil and deposition associated with solids in water, along with output from sewers were also log-normally distributed, while deposition from air to soil and biodegradation in soil and sediment followed normal distributions. The effect of uncertainty on the model results of the three key parameters was derived using a comparison of upper and lower of confidence interval boundaries at the 95% level of confidence. The results reveal that uncertainty in the key parameters had a more significant influence on equilibrium concentrations of the chemical in the bulk compartments of soil and sediment than on concentrations in the other two bulk compartments, various sub-compartments and the six predominant transfer fluxes.  相似文献   
24.
Xu FL  Dawson RW  Tao S  Li BG  Cao J 《Chemosphere》2002,46(2):173-185
This paper presents the system-level responses of experimental lake ecosystems to three chemical stresses (acidification, copper and pesticide contamination) using exergy and structural exergy as ecological indicators. The results indicate that the doses or toxicity of the three chemical stressors contributed to changes in both exergy and structural exergy. Remarkable changes in exergy and structural exergy occurred under acidic conditions and in the presence of Dursban, 24D-DMA, permethrin, bifenthrin, Carbaryl, TCP, PCP, trichlorethylene, benzene, and high doses of Cu, oil, and hexazinone. This seemed to indicate that the subject ecosystems were seriously contaminated by these chemical stressors. For low doses of Cu, oil, atrazine, HCBP, and hexazinone, exergy and structural exergy were either unchanged or only slightly changed, suggesting that the lake ecosystems were not significantly impacted by these chemical stressors. Discussion of the relationships between ecosystem-level changes and structural and functional changes in stressed lake ecosystems indicates that the above-mentioned ecosystem-level changes were in accordance with the changes in structure and function. The observed changes in exergy and structural exergy were also consistent with Odum's predictions of shortened food chains, reduced resource use efficiency, poor stability, low information, and high entropy in stressed aquatic ecosystems. The findings lead the authors to conclude that it is feasible for exergy and structural exergy to serve as ecological indicators when characterizing the system-level responses of experimental lake ecosystems to chemical stress. These results for experimental lake ecosystems would be extrapolated to actual lakes.  相似文献   
25.
An amniocentesis was performed on a gravida 1, para 0 23-year-old female because of high maternal serum alpha-fetoprotein and nuchal thickening/cystic mass apparent on the fetal ultrasound. Detailed ultrasound examination revealed multiple anomalies including brain abnormalities. The fetus was found to have a mosaic female karyotype: 45,XX, - 6/46,XX,r(6) (p25q27) (62 per cent:38 per cent). This is the first report of a prenatally diagnosed case of ring chromosome 6.  相似文献   
26.
Considerable attention has focused on inter- and intraspecific variation in trophic niches of marine predators. Although this has revealed evidence for sexual segregation in distribution in some species, few studies have been able to address sex-related dietary specialisation. Stable isotope analysis of blood cells collected from albatrosses and petrels at South Georgia during chick-rearing indicated a difference in δ13C, suggesting that females fed to the north of males, only in two species with male-biased sexual size dimorphism; in no species did sexes differ in trophic level (δ15N). Based on a wider review, significant differences between sexes in isotope signatures were much more common in seabirds during the pre-laying or breeding than the nonbreeding period, presumably reflecting greater between-sex partitioning of resources when foraging ranges are more constrained and competition is greater. Sex differences, or their absence, were usually consistent across successive stages during the pre-laying and breeding periods, but not necessarily year-round nor between populations. Significant differences in isotope signatures between males and females were extremely rare in monomorphic species, suggesting a link between sexual size dimorphism and segregation in diet or distribution. Among the Southern Ocean albatrosses, sex differences in δ13C suggested the underlying mechanism was related to habitat specialisation, whereas in other size-dimorphic taxa (both male- and female-biased), sex differences were more common in δ15N than δ13C and therefore more consistent with size-mediated competitive exclusion or dietary specialisation.  相似文献   
27.
Topsoil samples from 56 sites around the Guanting Reservoir, China, were measured for HCH and DDT concentrations. The total soil HCH content (including alpha-, beta-, gamma-, and delta-isomers) in these soil samples ranged from 0 to 7.33 ng x g(-1), with a mean of 0.69 ng x g(-1). These levels were considerably lower than those of the total DDT soil contents (including pp'-DDE, pp'-DDD, op'-DDT, and pp'-DDT), which ranged from 0 to 76.01 ng x g(-1), with a mean of 9.46 ng x g(-1). DDT was also found to be the major pollutant in the soil samples, accounting for approximately 93% of the total organochlorine pesticide (OCP) contents. Several environmental factors including land use, soil texture, soil taxonomy, and microbial biomass were considered to be responsible for the OCP levels observed. The data provide some insight into the effects of environmental conditions such as soil formation, agricultural cultivation, nutrient enrichment, and other anthropogenic activities on the degradation of OCPs in soils. Although the OCP residues currently are below the maximum limits set for use on agricultural land in China, and only rarely would such levels pose significant ecological concern, OCPs are highly persistent in soil and bioaccumulative. The data provided in this study are considered crucial for reservoir remediation, especially since the Guanting Reservoir will serve as one of the main drinking water sources for Beijing in the foreseeable future.  相似文献   
28.
Tripathi  Rahul  Dhal  B.  Shahid  Md  Barik  S. K.  Nayak  A. D.  Mondal  B.  Mohapatra  S. D.  Chatterjee  D.  Lal  B.  Gautam  Priyanka  Jambhulkar  N. N.  Fitton  Nuala  Smith  Pete  Dawson  T. P.  Shukla  A. K.  Nayak  A. K. 《Environment, Development and Sustainability》2021,23(8):11563-11582

A study was conducted to examine the interrelationships among socioeconomic factors, household consumption patterns, calorie intake and greenhouse gas emissions factors in rural eastern India based on household survey data. Findings indicated that higher monthly per capita incomes (12.1–80.1$) were associated with greater average calorie intakes (2021–2525 kcal d?1). As estimated by the FEEDME model, in total 17.2% of the population was calorie malnourished with a regional disparity of 29.4–18.2% malnourishment. Greenhouse gas (GHG) emissions were calculated only on the basis of crop and livestock production and consumption. Rice accounted for the highest share of total GHG emissions, on average 82.6% on a production basis, which varied from 58.1% to 94.9% in regional basis. Rice contributed the greatest share (~?65% and 66.2%) in terms of both calories and GHG emissions (CO2 eq y?1), respectively, on a consumption basis. We conclude that extensive rice farming and increasing animal product consumption are dominant factors in the higher carbon footprint in this region and are likely to further increase with increase in per capita income. This study provides useful information to help for better crop planning and for fine-tuning food access policy, to reduce carbon footprint and calorie malnutrition.

  相似文献   
29.
The Arctic Ocean is undergoing rapid change: sea ice is being lost, waters are warming, coastlines are eroding, species are moving into new areas, and more. This paper explores the many ways that a changing Arctic Ocean affects societies in the Arctic and around the world. In the Arctic, Indigenous Peoples are again seeing their food security threatened and cultural continuity in danger of disruption. Resource development is increasing as is interest in tourism and possibilities for trans-Arctic maritime trade, creating new opportunities and also new stresses. Beyond the Arctic, changes in sea ice affect mid-latitude weather, and Arctic economic opportunities may re-shape commodities and transportation markets. Rising interest in the Arctic is also raising geopolitical tensions about the region. What happens next depends in large part on the choices made within and beyond the Arctic concerning global climate change and industrial policies and Arctic ecosystems and cultures.  相似文献   
30.
Densely populated coastal urban areas are often exposed to multiple hazards, in particular floods and storms. Flood defenses and other engineering measures contribute to the mitigation of flood hazards, but a holistic approach to flood risk management should consider other interventions from the human side, including warning information, adaptive behavior, people/property evacuation, and the multilateral relief in local communities. There are few simulation approaches to consider these factors, and these typically focus on collective human actions. This paper presents an agent-based model that simulates flood response preferences and actions taken within individual households to reduce flood losses. The model implements a human response framework in which agents assess different flood scenarios according to warning information and decide whether and how much they invest in response measures to reduce potential inundation damages. A case study has been carried out in the Ng Tung River basin, an urbanized watershed in northern Hong Kong. Adopting a digital elevation model (DEM) as the modeling environment and a building map of household locations in the case area, the model considers the characteristics of households and the flood response behavior of their occupants. We found that property value, warning information, and storm conditions all influence household losses, with downstream and high density areas being particularly vulnerable. Results further indicate (i) that a flood warning system, which provides timely, accurate, and broad coverage rainstorm warning, can reduce flood losses by 30–40%; and (ii) to reduce losses, it is more effective and cheaper to invest early in response measures than late actions. This dynamic agent-based modeling approach is an innovative attempt to quantify and model the role of human responses in flood loss assessments. The model is demonstrated being useful for analyzing household scale flood losses and responses and it has the potential to contribute to flood emergency planning resource allocation in pluvial flood incidents.  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号