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681.
The objective of this study is to examine the effect of clayminerals (illite, montmorillonite, and kaolinite) on chromate (Cr(VI)) reduction by several low molecular weightorganic compounds. Batch experiments at pH ranging from 3.0 to6.0 and 25 °C showed that 2:1 layered clays illite andsmectite catalyzed Cr(VI) reduction by oxalate. The catalyticeffect increased as pH was decreased. The 1:1 clay kaolinite hadno catalytic effect under comparable conditions. Direct Cr(VI)reduction by reactive moieties associated with illite andmontmorillonite was observed, but at a much slower rate than thecatalytic pathway. Cr(VI) reduction by glyoxylic acid, glycolicacid, lactic acid, and mandelic acid was accelerated by illite,although aqueous phase reduction might occur in parallel. Theseresults suggest that Cr(VI) reduction rates in subsurfaceenvironments rich in organic compounds may be elevated throughcatalysis of surface-bound metals and/or soluble species from theclay minerals, and as a result, higher than those expected fromaqueous phase reaction alone. Such rate enhancement for Cr(VI)reduction needs to be accounted for when developing new remedialtechniques for chromium site remediation or assessing its naturalattenuation. 相似文献
682.
Weidong Wang Jun Zheng Zhongqiong Wang Rongbin Zhang Qinghua Chen Xinfeng Yu Chengqing Yin 《环境科学学报(英文版)》2016,28(1):119-133
Shijiuyang Constructed Wetland(110 hm~2) is a drinking water source treatment wetland with primary structural units of ponds and plant-bed/ditch systems. The wetland can process about 250,000 tonnes of source water in the Xincheng River every day and supplies raw water for Shijiuyang Drinking Water Plant. Daily data for 28 months indicated that the major water quality indexes of source water had been improved by one grade. The percentage increase for dissolved oxygen and the removal rates of ammonia nitrogen, iron and manganese were 73.63%, 38.86%, 35.64%, and 22.14% respectively. The treatment performance weight of ponds and plant-bed/ditch systems was roughly equal but they treated different pollutants preferentially. Most water quality indexes had better treatment efficacy with increasing temperature and inlet concentrations. These results revealed that the pond–wetland complexes exhibited strong buffering capacity for source water quality improvement. The treatment cost of Shijiuyang Drinking Water Plant was reduced by about 30.3%. Regional rainfall significantly determined the external river water levels and adversely deteriorated the inlet water quality, thus suggesting that the "hidden" diffuse pollution in the multitudinous stream branches as well as their catchments should be the controlling emphases for river source water protection in the future. The combination of pond and plant-bed/ditch systems provides a successful paradigm for drinking water source pretreatment. Three other drinking water source treatment wetlands with ponds and plant-bed/ditch systems are in operation or construction in the stream networks of the Yangtze River Delta and more people will be benefited. 相似文献
683.
为明晰我国各海域的海滩垃圾污染状况及垃圾主要来源,在我国各海区选择24个代表性采样点,共86个调查样方,对我国各海域的海滩垃圾的种类、来源进行了详细调查和重点区域的跟踪调查.结果表明:我国海滩垃圾平均个数为1.03 m-2,其中塑料类最多(占37.37%),其次为泡沫类(占35.67%);总密度为15.91 g/m2,塑料类密度(3.62 g/m2)最大,其次为织物(布)类(2.87 g/m2)和木制品类(1.97 g/m2);主要来源是生活垃圾和旅游垃圾,分别占垃圾总量的39.26%和25.23%;对照国际国内相关调查资料,我国海洋垃圾的污染呈逐渐恶化的趋势,总体形势不容乐观.针对我国海洋垃圾的污染控制,提出应通过进一步海洋垃圾污染调查工作,从制订污染防治监督管理办法、编制污染防治专项规划等方面入手理清各部门管理权责;同时以政府为主导,联合公众、企业、NGO(非政府组织)等多方力量,建立海洋垃圾回收资源化示范点,开展海洋垃圾宣传、清理和海滩清扫活动等控制对策. 相似文献
684.
Changes in metal concentrations in the litter of Potamogeton crispus were monitored during a consecutive 40-day in situ decomposition experiment using the litterbag method.The accumulation index was calculated and used to indicate the changes in the metals in litter.The results showed that the concentrations of Al,Cd,Cr,Fe,Mn,and Pb in litter increased significantly during the decomposition,while Cu and Zn concentrations decreased dramatically.Significant positive correlations were found between the concentrations of Al,Cr,Fe,and Mn and between Cu and Zn.Moreover,Cu and Zn both negatively correlated with Al and Fe.The remaining dry mass was negatively correlated with Al and Fe concentrations but positively correlated with Cu and Zn concentrations.Generally the accumulation index values of metals other than Al were less than one,indicating that the litter of P.crispus acted as a source of metals to the surrounding water body.Al was the only metal that showed continuous net accumulation in litter.The net accumulation of Fe and Mn in litter during the last 10 days of the experiment may indicate the precipitation of Feand Mn-oxides.It was estimated that 160 g/m~2(dry weight)P.crispus was decomposed in40 days.This was equivalent to releasing the following amounts of metals:0.01 mg Cd,0.03 mg Cr,0.71 mg Cu,0.55 mg Mn,0.02 mg Pb and 13.8 mg Zn into surrounding water,and accumulating 149 mg Al and 11 mg Fe,in a 1 m~2 area. 相似文献
685.
To develop a depth filter based on the electrostatic adsorption principle, positively charged microporous ceramic membrane was prepared from a diatomaceous earth ceramic membrane.The internal surface of the highly porous ceramic membrane was coated with uniformly distributed electropositive nano-Y_2O_3 coating. The dye removal performance was evaluated through pressurized filtration tests using Titan Yellow aqueous solution. It showed that positively charged microporous ceramic membrane exhibited a flow rate of 421 L/(m~2·hr) under the trans-membrane pressure of 0.03 bar. Moreover it could effectively remove Titan Yellow with feed concentration of 10 mg/L between pH 3 to 8. The removal rate increased with the enhancement of the surface charge properties with a maximum rejection of 99.6%. This study provides a new and feasible method of removing organic dyes in wastewater. It is convinced that there will be a broad market for the application of charged ceramic membrane in the field of dye removal or recovery from industry wastewater. 相似文献
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688.
Towards Real‐Time Continental Scale Streamflow Simulation in Continuous and Discrete Space
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Fernando R. Salas Marcelo A. Somos‐Valenzuela Aubrey Dugger David R. Maidment David J. Gochis Cédric H. David Wei Yu Deng Ding Edward P. Clark Nawajish Noman 《Journal of the American Water Resources Association》2018,54(1):7-27
The National Weather Service (NWS) forecasts floods at approximately 3,600 locations across the United States (U.S.). However, the river network, as defined by the 1:100,000 scale National Hydrography Dataset‐Plus (NHDPlus) dataset, consists of 2.7 million river segments. Through the National Flood Interoperability Experiment, a continental scale streamflow simulation and forecast system was implemented and continuously operated through the summer of 2015. This system leveraged the WRF‐Hydro framework, initialized on a 3‐km grid, the Routing Application for the Parallel Computation of Discharge river routing model, operating on the NHDPlus, and real‐time atmospheric forcing to continuously forecast streamflow. Although this system produced forecasts, this paper presents a study of the three‐month nowcast to demonstrate the capacity to seamlessly predict reach scale streamflow at the continental scale. In addition, this paper evaluates the impact of reservoirs, through a case study in Texas. Validation of the uncalibrated model using observed hourly streamflow at 5,701 U.S. Geological Survey gages shows 26% demonstrate PBias ≤ |25%|, 11% demonstrate Nash‐Sutcliffe Efficiency (NSE) ≥ 0.25, and 6% demonstrate both PBias ≤ |25%| and NSE ≥ 0.25. When evaluating the impact of reservoirs, the analysis shows when reservoirs are included, NSE ≥ 0.25 for 56% of the gages downstream while NSE ≥ 0.25 for 11% when they are not. The results presented here provide a benchmark for the evolving hydrology program within the NWS and supports their efforts to develop a reach scale flood forecasting system for the country. 相似文献
689.
Lin Huiming Zhang Wei Deng Chunyan Tong Yingdong Zhang Qianggong Wang Xuejun 《Environmental science and pollution research international》2017,24(16):14190-14197
Environmental Science and Pollution Research - Atmospheric mercury monitoring is essential because of its potential human health and ecological impacts. Current automated monitoring systems include... 相似文献
690.
Regional Environmental Change - This paper estimates the impact of land use change on soil organic carbon (SOC) sequestration in China from 1985 to 2005 using a nationwide, georeferenced database... 相似文献