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271.
Huan Feng Yu Qian Frank J. Gallagher Meiyin Wu Weiguo Zhang Lizhong Yu Qingzhi Zhu Kewei Zhang Chang-Jun Liu Ryan Tappero 《Environmental science and pollution research international》2013,20(6):3743-3750
Synchrotron X-ray microfluorescence and X-ray absorption near-edge microstructure spectroscopy techniques were applied to Typha latifolia (cattail) root sections and rhizosphere soils collected from a brownfield site in New Jersey to investigate lead (Pb) accumulation in T. latifolia roots and the role of iron (Fe) plaque in controlling Pb uptake. We found that Pb and Fe spatial distribution patterns in the root tissues are similar with both metals present at high concentrations mainly in the epidermis and at low concentrations in the vascular tissue (xylem and phloem), and the major Pb and Fe species in T. latifolia root are Pb(II) and Fe(III) regardless of concentration levels. The sequestration of Pb by T. latifolia roots suggests a potential low-cost remediation method (phytostabilization) to manage Pb-contaminated sediments for brownfield remediation while performing wetland rehabilitation. 相似文献
272.
273.
Harold C. Hodge Frank A. Smith 《Journal of the Air & Waste Management Association (1995)》2013,63(4):226-232
Minute traces of fluoride are found in the air of rural communities and of cities, having been contributed perhaps from volcanic effluvia, perhaps from burning coal, and perhaps from industrial sources. Atmospheres of urban areas of the U. S. have been found to contain from less than 0.2 μg F/m3 to as much as 1.9/μg F/m3. Fluorides released from industrial processes may release elemental fluorine, soluble gaseous fluorides, and soluble or insoluble fluoride dusts. At least in some instances inhaled fluoride from fluoride containing dusts has proven to be as biologically available as that from similar concentrations of inhaled HF. Measurement of the amount of fluoride excreted in the urine has proven to be a valuable index of exposure and a means of preventing cumulative injury. Average urinary F concentrations not exceeding 5 mg/liter, which corresponds approximately to a daily intake of 5 mg, are not associated with osteosclerosis in such workmen, and such changes are unlikely at daily intakes of 5 – 8 mg F. The amount of fluoride which is retained by an individual inhaling air containing 2.5 mg of fluoride dusts per m3 (the current TLV) is approximately 5-6 mg. A review of the literature describing the exposure of work forces to fluorides in industrial atmospheres indicates that concentrations have ranged from a fraction of a milligram/m3 to values mostly less than 10 mg/ml Surveys of populations living near installations emitting fluoride fumes or dusts indicate that, with few exceptions, the health of these persons has not been adversely affected. Many species of vegetation are far more susceptible to the effects of fluoride than is man, hence an air quality standard to protect vegetation will be far lower than those encountered in the factory, and can be expected to be of the order of 10 ppb or less. The probable daily intake of F at this level of exposure is 0.16 mg, an intake far below that required for the production of clear-cut effects in the human. Thus, air quality standards set to protect vegetation would contribute negligible quantities of F in terms of any possible adverse effect on human health, and would give a wide margin of protection for man. 相似文献
274.
Joseph F. Walling Gary Evans Thomas A. Hinners Joseph P. Lambert Sharon J. Long Frank W. Wilshire 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1134-1136
A comparison was made of over 300 pairs of arsenic results from instrumental neutron activation and flameless atomic absorption analyses of atmospheric particulates collected on glass fiber filters. Atomic absorption analyses involved low temperature ashing of filters at high power levels. No matrix modification chemicals were added to the acid extract which was analyzed. Neutron activation results are on the average 9% higher than those obtained by atomic absorption and the difference is statistically significant. This small difference is probably due to the analytical techniques or acid extraction and not in any important way to losses during low temperature ashing. This conclusion is in sharp contrast to other recently reported situations where low temperature ashing losses in analyzing atmospheric particulate were sizable. Although the atmospheres sampled differed somewhat between these situations the most obvious difference was in the combustibility of the filters used in sampling. 相似文献
275.
Noel de Nevers Kin Wan Lee Neil H. Frank 《Journal of the Air & Waste Management Association (1995)》2013,63(10):995-1000
The highest values in annual TSP distributions fall below the best-fit, log-normal straight line more than one would expect from ordinary sampling statistics but not dramatically so. The lowest values in annual TSP distributions overwhelmingly fall below the best-fit, log-normal straight line. The most highly improbable high values above the best-fit line in such distributions are very questionable and probably do not represent true air quality values. The most improbable cases of highest values falling below the best-fit, log-normal line are the result of data artifacts at the opposite end of the data distribution. They do not represent low probabilities and probably do represent true air quality values. The most improbable low values are all of highly doubtful validity. 相似文献
276.
Peter A. Gabele James O. Baugh Frank Black Richard Snow 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1168-1175
Exhaust and evaporative emissions were examined from vehicles fueled with methanol or a gasoline-methanol blend. Regulated automobile pollutants, as well as detailed hydrocarbons, methanol, and aldehydes were measured, and exhaust emission trends were obtained for vehicle operation over five different driving cycles. Results indicated that use of the blended fuel does not generally have any significant effect on base-line exhaust emission rates of regulated pollutants; however, emission rates of aldehydes increased during the Federal Test Procedure. Aldehyde emissions from the methanol-fueled car were roughly an order of magnitude higher than those resulting from blended fuel usage. The hydrocarbon composition of evaporative emissions with the blended fuel was similar to that with the base-line fuel except when canister breakthrough occurred. Evaporative emissions during breakthrough were comprised chiefly of N-butane. 相似文献
277.
Chun W. Lee Ravi K. Srivastava S. Behrooz Ghorishi Thomas W. Hastings Frank M. Stevens 《Journal of the Air & Waste Management Association (1995)》2013,63(12):1560-1566
Abstract Selective catalytic reduction (SCR) technology increasingly is being applied for controlling emissions of nitrogen oxides (NOx) from coal-fired boilers. Some recent field and pilot studies suggest that the operation of SCR could affect the chemical form of mercury (Hg) in coal combustion flue gases. The speciation of Hg is an important factor influencing the control and environmental fate of Hg emissions from coal combustion. The vanadium and titanium oxides, used commonly in the vanadia-titania SCR catalyst for catalytic NOx reduction, promote the formation of oxidized mercury (Hg2+). The work reported in this paper focuses on the impact of SCR on elemental mercury (Hg0) oxidation. Bench-scale experiments were conducted to investigate Hg0 oxidation in the presence of simulated coal combustion flue gases and under SCR reaction conditions. Flue gas mixtures with different concentrations of hydrogen chloride (HCl) and sulfur dioxide (SO2) for simulating the combustion of bituminous coals and subbituminous coals were tested in these experiments. The effects of HCl and SO2 in the flue gases on Hg0 oxidation under SCR reaction conditions were studied. It was observed that HCl is the most critical flue gas component that causes conversion of Hg0 to Hg2+ under SCR reaction conditions. The importance of HCl for Hg0 oxidation found in the present study provides the scientific basis for the apparent coal-type dependence observed for Hg0 oxidation occurring across the SCR reactors in the field. 相似文献
278.
Anders Galatius Rossana Bossi Christian Sonne Frank Farsø Rigét Carl Christian Kinze Christina Lockyer Jonas Teilmann Rune Dietz 《Environmental science and pollution research international》2013,20(11):8013-8020
Profiles of seven compounds of perfluoro-alkyl substances (PFASs) were compared among three species of top predators from the Danish North Sea: the white-beaked dolphin (Lagenorhynchus albirostris), the harbor porpoise (Phocoena phocoena), and the harbor seal (Phoca vitulina). The seals had higher total burdens (757.8 ng g?1 ww) than the dolphins (439.9 ng g?1 ww) and the porpoises (355.8 ng g?1 ww), probably a reflection of feeding closer to the shore and thus contamination sources. The most striking difference among the species was the relative contribution of perfluorooctanesulfonamide (PFOSA) to the profiles; the seals (0.1 %) had much lower levels than porpoises (8.3 %) and dolphins (26.0 %). In combination with the values obtained from the literature, this result indicates that Carnivora species including Pinnipedia have a much higher capacity of transforming PFOSA to perfluorooctane sulfonic acid (PFOS) than cetacean species. Another notable difference among the species was that the two smaller species (seals and porpoises) with supposedly higher metabolic rates had lower concentrations of the perfluorinated carboxylic acids, which are generally more easily excreted than perfluorinated sulfonamides. Species-specific characteristics should be recognized when PFAS contamination in marine mammals is investigated, for example, several previous studies of PFASs in cetaceans have not quantified PFOSA. 相似文献
279.
Alfred Marzocchi Ph.D. Frank Lachut William H. Willis JR. 《Journal of the Air & Waste Management Association (1995)》2013,63(1):38-42
Typical air quality effect levels of photochemical oxidants on specific plant substrates are illustrated. These include ambient oxidant exposure data measured as “total oxidant” as well as laboratory exposures to individual pure oxidants, ozone, or PAN compounds, since these oxidants are identified in photochemical smog. New terms, “PaNs” and “PAN-type” oxidant, have been proffered for purposes of clarification of the terminology. PAN-type oxidant more precisely defines the phytotoxicant complex causing silvering or bronzing of the lower leaf surfaces in lieu of the older term “oxidant.” Due to the recognition of several oxidizing phytotoxicants in recent years, it is recommended that the term oxidant be reserved for use as a generic term. A tabular classification of the oxidizing phytotoxicants found in community photochemical smog and the specific syndromes produced is provided. 相似文献
280.