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71.
In the investigation of arsenic warfare agents in ammunitions scrap, a differentiation of inorganic and organic arsenic compounds is necessary. This study describes a method that allows this differential determination. By GC/MS CLARK I, some stabilizers and several phenylarsenic compounds could be identified in chemical warfare pellets. 相似文献
72.
Die wechselseitige Beeinflussung der PAK- und Schwermetall-Aufnahme (Cu, Zn, Cd, Pb) durch Weizen und Gerste von einer durch
Munitionsrückst?nde belasteten Nutzfl?che wird beschrieben. Die nachgewiesenen PAK in der Pflanze k?nnten auf Membranver?nderungen
der Wurzeln durch Schwermetalle zurückzuführen sein. 相似文献
73.
For the time being, simple and reliable methods which permit the imaging of the complex topography of contaminant plumes in groundwater are missing. The conventional methods for the punctual determination of contaminant concentrations cannot fulfill this demand. To successfully implement and utilize. Natural Attenuation, these deficits have to be overwhelmed. The detectors described in the following represent only part of the probing device system the authors have developed; it shall enable their user to image different aspects of plume topography and its time dependent change by monitoring within the undisturbed groundwater aquifer in groundwater measuring levels: ? relative freights of contaminants and trace contaminants by passive samplers [4] and ? redox milieu parameters by detectors. The detectors offer multi-purpose, tape-like probing devices of unlimited length. They are charged with a defined reserve of reactive substances. During monitoring actions, the derector tape hangs vertically stretched by a weight preferably covering from the top to the bottom of the whole water column. During the reaction period, the detector may be relaunched for repeated visual inspection. The colour changes of the detectors enable the identification of a row of parameters in the vertically (depth-) oriented profile by unbroken optical/visually perceivable imaging: ? Position of Redox potential thresholds for Mn-IV-Mn-II, Fe-III-Fe-II, Sulfate-Sulfide ? Position of ochre precipitation and iron-sulfide precipitation horizons ? Relative freights of the sum of substances effecting reduction (period until defined oxidant reserve has been reduced) ? Relative freights of the sum of substances effecting iron-sulfide oxidation (period until defined reductant reserve has been reduced) ? Position of dissolved iron-II ions containing horizons ? Position of dissolved hydrogen-sulfide ions/hydrogen-sulfide containing horizons ? Relative freights of iron-II ions (period until defined oxidant reserve has been reduced) ? Relative freights of hydrogen-sulfide ions/hydrogen-sulfide (period until defined oxidant reserve has been reduced). Furthermore, the detectors are also suitable for the examination of waters even of great depth, as for example artificial or natural lakes, sea and ocean basins. 相似文献
74.
The efficacy of disinfection processes in water purification systems is governed by several key factors, including reactor hydraulics, disinfectant chemistry, and microbial inactivation kinetics. The objective of this work was to develop a computational fluid dynamics (CFD) model to predict velocity fields, mass transport, chlorine decay, and microbial inactivation in a continuous flow reactor. The CFD model was also used to evaluate disinfection efficiency in alternative reactor designs. The CFD reactor analysis demonstrates that disinfection efficiency is affected by both kinetics and mixing state (i.e., degree of micromixing or segregation). Residence time distributions (RTDs) derived from tracer analysis do not describe intrinsic mixing conditions. The CFD-based disinfection models account for reactor mixing patterns by resolution of the reactor velocity field and thus provide a better prediction of microbial inactivation than models that use an RTD. 相似文献
75.
de Haas EM Léon Paumen M Koelmans AA Kraak MH 《Environmental pollution (Barking, Essex : 1987)》2004,127(1):99-107
Effects observed in whole-sediment bioassays must be seen as the joint effect of all sediment characteristics. In whole-sediment bioassays, however, adverse effects on test organisms are usually attributed to the presence of contaminants and effects of food are often ignored. The aim of this study was to analyze the response of the midge Chironomus riparius to sediment spiked with different combinations of food and copper. The responses of C. riparius to these spiked sediments were assessed in 10-day whole-sediment bioassays. Decreases in survival, dry weight, and length of C. riparius were observed with increasing copper concentrations. However, an increase in the amount of food resulted in an increase of larval dry weight and length until copper concentrations reached a critical threshold of 200 mg/kg. In addition, an increase in the amount of food resulted in a decrease of accumulated copper in the larvae. The present study demonstrated that the combination of copper and food in the sediment determines the performance of C. riparius in whole-sediment bioassays. The dependency of C. riparius on high feeding levels, which mask toxic effects, questions its suitability as a test organism for whole-sediment bioassays. Because benthic communities in polluted ecosystems are often exposed to varying levels of both food and toxicants it is concluded that the trophic state of the ecosystem may alter the ecological risk of sediment-bound toxicants to opportunistic benthic invertebrates such as C. riparius. 相似文献
76.
For the first time we are able to report the identification and quantification of several unexpected alkylated tin compounds such as dimethyldiethyltin, trimethylethyltin and propyltrimethyltin in European municipal waste deposits, by using GC-ICP-MS. Future studies will reveal whether their origin is from the degradation of butyl-, or octyltin compounds or simply products of de novo synthesis within the landfill environment. 相似文献
77.
78.
79.
Ethylarsine dichloride was used during WW I as a chemical warfare agent. Residues of this chemical warfare agent and its metabolites
are still present today and continue to contaminate soil and water.
A gas Chromatographic method for the detection and determination of ethylarsine dichloride is shown. Six dithiols were tested
as possible derivatization reagents for ethylarsine dichloride. With selection of the dithiol, matrix interferences can be
eliminated because of the different retention times of the derivatives. 相似文献
80.
Rainer W. Sieke Günter Lippke Alfred Krippendorf Rainer Haas Sven Lüdtke 《Environmental science and pollution research international》1998,5(4):199-201
The new technology of Plasmazon® uses the extremely strong oxidation of radicals to break up the compocunds of organic connections, e.g. chemical warfare agents like Clark I. In making a comparison of oxidation to normal ozone, the factor of the Plasmazon® -technology is available up to 103. The investigation in an experimental test shows that it is possible to destroy the warfare agent character of Clark I. As the possibility of a large-lot application this technology is the method of choice for other chemical or biological warfare agents. 相似文献