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Gal F Joublin F Haas H Jean-Prost V Ruffier V 《Journal of environmental radioactivity》2011,102(2):107-118
The south east basin of France shelters deep CO2 reservoirs often studied with the aim of better constraining geological CO2 storage operations. Here we present new soil gas data, completing an existing dataset (CO2, 222Rn, 4He), together with mineralogical and physical characterisations of soil columns, in an attempt to better understand the spatial distribution of gas concentrations in the soils and to rule on the sealed character of the CO2 reservoir at present time.Anomalous gas concentrations were found but did not appear to be clearly related to geological structures that may drain deep gases up to the surface, implying a dominant influence of near surface processes as indicated by carbon isotope ratios. Coarse grained, quartz-rich soils favoured the existence of high CO2 concentrations. Fine grained clayey soils preferentially favoured the existence of 222Rn but not CO2. Soil formations did not act as barriers preventing gas migrations in soils, either due to water content or due to mineralogical composition. No abundant leakage from the Montmiral reservoir can be highlighted by the measurements, even near the exploitation well. As good correlation between CO2 and 222Rn concentrations still exist, it is suggested that 222Rn migration is also CO2 dependent in non-leaking areas - diffusion dominated systems. 相似文献
84.
Shamia Hoque Bakhtier Farouk Charles N. Haas 《Journal of the Air & Waste Management Association (1995)》2013,63(9):968-982
ABSTRACT Linear, quadratic, and artificial neural network (ANN)-based metamodels were developed for predicting the extent of anthrax spore inactivation by chlorine dioxide in a ventilated three-dimensional space over time from computational fluid dynamics model (CFD) simulation data. Dimensionless groups were developed to define the design space of the problem scenario. The Hammersley sequence sampling (HSS) method was used to determine the sampling points for the numerical experiments within the design space. A CFD model, comprised of multiple submodels, was applied to conduct the numerical experiments. Large eddy simulation (LES) with the Smagorinsky subgrid-scale model was applied to compute the airflow. Anthrax spores were modeled as a dispersed solid phase using the Lagrangian treatment. The disinfectant transport was calculated by solving a mass transport equation. Kinetic decay constants were included for spontaneous decay of the disinfectant and for the reaction of the disinfectant with the surfaces of the three-dimensional space. To enhance the mixing of the disinfectant with the room air, a momentum source was included in the simulation. An inactivation rate equation accounted for the reaction between the spores and the disinfectant. The ANN-based metamodels were most successful in predicting the number of viable bioaerosols remaining in an arbitrary enclosed space. Sensitivity analysis showed that the mass fraction of the disinfectant, inactivation rate constant, and contact time had the most influence on the inactivation of the spores.
IMPLICATIONS This investigation presents a framework for the development of user-friendly models; metamodels for the prediction of the number of viable spores remaining in an indoor room during disinfection from accurate but time-consuming CFD studies. During any decontamination event, to know when to stop pumping in the disinfectant and to know what level of log reduction of the spores have been achieved before even starting decontamination would provide valuable guidance. The neural network based metamodels can be applied to obtain quick and relatively accurate answers. This would be necessary when immediate information is required during emergencies. 相似文献
85.
Rainer Haas 《Environmental Sciences Europe》1998,10(4):198-199
2-Chlorovinylarsine dichloride (Lewisite I) and 2,2′-dichlorodivinylarsine chloride (Lewisite II) react by room temperature rapidly and quantitatively with dithiols in a substitution reaction. The derivatives were identified with mass spectrometry. They can be detected with GC/ECD. This reactions can be used for the gas chromatographic detection of Lewisites in water and soil samples. 相似文献
86.
Elie Gaget Alison Johnston Diego Pavón-Jordán Aleksi S. Lehikoinen Brett K. Sandercock Alaaeldin Soultan Luka Božič Preben Clausen Koen Devos Cristi Domsa Vitor Encarnação Sándor Faragó Niamh Fitzgerald Teresa Frost Clemence Gaudard Lívia Gosztonyi Fredrik Haas Menno Hornman Tom Langendoen Christina Ieronymidou Leho Luigujõe Włodzimierz Meissner Tibor Mikuska Blas Molina Zuzana Musilová Jean-Yves Paquet Nicky Petkov Danae Portolou Jozef Ridzoň Laimonas Sniauksta Antra Stīpniece Norbert Teufelbauer Johannes Wahl Marco Zenatello Jon E. Brommer 《Conservation biology》2022,36(4):e13877
Protected area networks help species respond to climate warming. However, the contribution of a site's environmental and conservation-relevant characteristics to these responses is not well understood. We investigated how composition of nonbreeding waterbird communities (97 species) in the European Union Natura 2000 (N2K) network (3018 sites) changed in response to increases in temperature over 25 years in 26 European countries. We measured community reshuffling based on abundance time series collected under the International Waterbird Census relative to N2K sites’ conservation targets, funding, designation period, and management plan status. Waterbird community composition in sites explicitly designated to protect them and with management plans changed more quickly in response to climate warming than in other N2K sites. Temporal community changes were not affected by the designation period despite greater exposure to temperature increase inside late-designated N2K sites. Sites funded under the LIFE program had lower climate-driven community changes than sites that did not received LIFE funding. Our findings imply that efficient conservation policy that helps waterbird communities respond to climate warming is associated with sites specifically managed for waterbirds. 相似文献
87.
Mit impr?gnierten Filtermaterialien ist es m?glich, die Schwermetalle Blei, Kupfer und Nickel sowie Arsen durch Sorption bzw.
chemische Bindung aus Wasser zu entfernen. Bei 24stündiger Einwirkungszeit wurden Reduktionsraten von 97% bis>99,9% erreicht. 相似文献
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