全文获取类型
收费全文 | 1325篇 |
免费 | 92篇 |
国内免费 | 470篇 |
专业分类
安全科学 | 100篇 |
废物处理 | 82篇 |
环保管理 | 97篇 |
综合类 | 766篇 |
基础理论 | 191篇 |
环境理论 | 1篇 |
污染及防治 | 495篇 |
评价与监测 | 60篇 |
社会与环境 | 52篇 |
灾害及防治 | 43篇 |
出版年
2024年 | 3篇 |
2023年 | 34篇 |
2022年 | 101篇 |
2021年 | 86篇 |
2020年 | 67篇 |
2019年 | 42篇 |
2018年 | 52篇 |
2017年 | 79篇 |
2016年 | 77篇 |
2015年 | 95篇 |
2014年 | 105篇 |
2013年 | 156篇 |
2012年 | 120篇 |
2011年 | 113篇 |
2010年 | 93篇 |
2009年 | 67篇 |
2008年 | 97篇 |
2007年 | 71篇 |
2006年 | 62篇 |
2005年 | 35篇 |
2004年 | 34篇 |
2003年 | 36篇 |
2002年 | 34篇 |
2001年 | 32篇 |
2000年 | 33篇 |
1999年 | 29篇 |
1998年 | 21篇 |
1997年 | 27篇 |
1996年 | 17篇 |
1995年 | 17篇 |
1994年 | 13篇 |
1993年 | 17篇 |
1992年 | 6篇 |
1991年 | 4篇 |
1990年 | 5篇 |
1989年 | 2篇 |
1987年 | 1篇 |
1986年 | 1篇 |
1985年 | 2篇 |
1973年 | 1篇 |
排序方式: 共有1887条查询结果,搜索用时 15 毫秒
71.
Yuan Zhengqiu Yang Huizhi Xu Pan Li Chengfeng Jian Jian Zeng Jianxian Zeng Lingwei Sui Yuguang Zhou Hu 《Environmental science and pollution research international》2021,28(6):6411-6421
Environmental Science and Pollution Research - In this work, various photocatalysts were synthesized with an impregnation-precipitation process to in situ decorate Ag-based nanoparticles (NPs,... 相似文献
72.
Pb/Zn冶炼废渣中重金属的生物浸出-盐浸处理 总被引:3,自引:0,他引:3
利用中温嗜热菌对某铅锌冶炼废渣进行生物浸出盐浸处理研究,并根据国家固体废物浸出毒性方法(HJ/T299-2007)对盐浸后余渣进行毒性分析。研究结果表明,在pH 1.5、温度65℃、矿浆浓度5%的优化条件下生物浸出3 d后,废渣中Cu、In、Ga和Zn的浸出率分别达到了91.5%、91.8%、84.9%和93.4%;盐浸生物浸出渣,其浸出液中Ag、Pb浓度分别为7.6和247.5 mg/L,可从废渣中有效回收Cu、In、Ga、Zn、Ag和Pb。生物浸出盐浸处理后余渣约为原渣量的70%;毒性分析浸出液中重金属元素Ag、As、Cd、Cu、Pb和Zn浓度分别为2~3.5、2~3、0.3~0.5、30~50、2~4、20~60 mg/L,低于国家危险废物鉴别标准(GB5085.3-2007)。根据试验结果,提出了针对冶炼废渣资源化、减量化、无害化的生物浸出盐浸联用工艺。 相似文献
73.
Dane Westerdahl Xing Wang Xiaochuan Pan K. Max Zhang 《Atmospheric environment (Oxford, England : 1994)》2009,43(3):697-705
In this paper, we report the results and analysis of a recent field campaign in August 2007 investigating the impacts of emissions from transportation on air quality and community concentrations in Beijing, China. We conducted measurements in three different environments, on-road, roadside and ambient. The carbon monoxide, black carbon and ultrafine particle number emission factors for on-road light-duty vehicles are derived to be 95 g kg?1-fuel, 0.3 g kg?1-fuel and 1.8 × 1015 particles kg?1-fuel, respectively. The emission factors for on-road heavy-duty vehicles are 50 g kg?1-fuel, 1.3 g kg?1-fuel and 1.1 × 1016 particles kg?1-fuel, respectively. The carbon monoxide emission factors from this study agree with those derived from remote sensing and on-board vehicle emission testing systems in China. The on-road black carbon and particle number emission factors for Chinese vehicles are reported for the first time in the literature. Strong traffic impacts can be observed from the concentrations measured in these different environments. Most clear is a reflection of diesel truck traffic activity in black carbon concentrations. The comparison of the particle size distributions measured at the three environments suggests that the traffic is a major source of ultrafine particles. A four-day traffic control experiment conducted by the Beijing Government as a pilot to test the effectiveness of proposed controls was found to be effective in reducing extreme concentrations that occurred at both on-road and ambient environments. 相似文献
74.
Liming Zhang Dongsheng Yu Xuezheng Shi David C. Weindorf Limin Zhao Weixin Ding Hongjie Wang Jianjun Pan Changsheng Li 《Atmospheric environment (Oxford, England : 1994)》2009,43(17):2737-2746
Quantifying greenhouse gas (GHG) emissions from wetland ecosystems is a relatively new issue in global climate change studies. China has approximately 22% of the world's rice paddies and 38% of the world's rice production, which are crucial to accurately estimate the global warming potential (GWP) at regional scale. This paper reports an application of a biogeochemical model (DeNitrification and DeComposition or DNDC) for quantifying GWP from rice fields in the Tai-Lake region of China. For this application, DNDC is linked to a 1:50,000 soil database, which was derived from 1107 paddy soil profiles compiled during the Second National Soil Survey of China in the 1980–1990s. The simulated results show that the 2.34 Mha of paddy soil cultivated in rice–wheat rotation in the Tai-Lake region emitted about ?1.48 Tg C, 0.84 Tg N and 5.67 Tg C as CO2, N2O, and CH4 respectively, with a cumulative GWP of 565 Tg CO2 equivalent from 1982 to 2000. As for soil subgroups, the highest GWP (26,900 kg CO2 equivalent ha?1 yr?1) was linked to gleyed paddy soils accounting for about 4.4% of the total area of paddy soils. The lowest GWP (5370 kg CO2 equivalent ha?1 yr?1) was associated with submergenic paddy soils accounting for about 0.32% of the total area of paddy soils. The most common soil in the area was hydromorphic paddy soils, which accounted for about 53% of the total area of paddy soils with a GWP of 12,300 kg CO2 equivalent ha?1 yr?1. On a regional basis, the annual averaged GWP in the polder, Tai-Lake plain, and alluvial plain soil regions was distinctly higher than that in the low mountainous and Hilly soil regions. As for administrative areas, the average annual GWP of counties in Shanghai city was high. Conversely, the average annual GWP of counties in Jiangsu province was low. The high variability in soil properties throughout the Tai-Lake region is important and affects the net greenhouse gas emissions. Therefore, the use of detailed soil data sets with high-resolution digital soil maps is essential to improve the accuracy of GWP estimates with process-based models at regional and national scales. 相似文献
75.
进水水质成分改变引发的污泥粘性膨胀及控制 总被引:2,自引:0,他引:2
在研究强化SBR工艺除污性能时,由于可溶性淀粉投加导致进水水质成分发生改变,污泥沉降性能在短时间内迅速恶化,污泥出现大量的粘液。镜检发现,大量指状菌胶团异常增殖且丝状菌的数量也逐渐减少。实验结果表明,系统膨胀属于污泥粘性膨胀。停止可溶性淀粉和提高主反应池的DO浓度,污泥粘性膨胀并未得到恢复,但污泥粘液逐渐消失。粘液消失后,通过模拟前期进水水质成分和缩短泥龄,污泥粘性膨胀得以控制,污泥沉降性能在短时间内恢复。实验还研究了污泥粘性膨胀对污染物去除性能的影响。 相似文献
76.
77.
78.
以酸性矿山废水生成的铁絮体和秸秆生物炭为原料,采用化学改性和紫外辐射联用技术制备改性生物炭,并通过正交试验确定最佳改性条件,同时利用FTIR、SEM和BET等方法对吸附材料的形貌特征、孔隙结构及其表面化学性质进行表征.结果表明,通过改性使吸附材料比表面积增大,吸附位点增多,在25℃、pH为7时,吸附材料改性后比表面积为295.71 m2·g-1,对Pb(II)的拟合吸附量可达278 mg·g-1.改性材料对Pb(II)的吸附过程符合Langmuir吸附等温线模型和准二级动力学模型,主要为单分子层吸附,受化学吸附控制. 相似文献
79.
矿山开采过程产生的酸性排水及其携带的重金属对生态环境造成了严重的危害,其防控的关键在于控酸,因此矿井水酸化过程的解析可为矿山酸性排水的源头防控提供理论依据。本文以独山半坡锑矿为研究区,采集矿井内部不同区域水体样品32件,通过对水体酸化的矿物端元解析和重金属的共氧化过程、离子水解过程以及不同类型矿井水的混合过程分析,揭示了矿井水的酸化过程。结果表明,矿井内辉锑矿与黄铁矿的氧化使流经的矿井水具有低p H和高硫酸根的特征,与未受矿业活动影响的地下水具有明显差异。在矿井水流动过程中,Sb(Ⅲ)与Fe(Ⅱ)的共氧化过程消耗了氢离子,不同水体混合过程中碳酸氢根对酸的缓冲作用明显,以上过程延缓了矿井水的酸化;由于水体酸化使Al、Mn、Fe等离子溶出,而这些离子可能发生的水解过程加速了矿井水的酸化。 相似文献
80.
抗生素残留物是一种新兴的微污染物,广泛存在于各种环境介质及生物样品中,长期暴露在抗生素环境会对人体健康、生态环境产生一定的潜在威胁。由于农村污水排放量逐渐增大、农村地区对抗生素的不合理使用以及受经济、地理地形的限制大部分农村地区都缺乏完整的污水收集管网和污水治理设施,进而导致抗生素通过多种途径进入农村环境,可能会对农村生态环境产生一定的环境风险。为了解贵州农村污水中抗生素的污染水平及处理后污水对环境的影响,作者采用固相萃取—液相色谱—串联质谱(SPE-LC-MS)联用技术,选取贵州省3处典型农村地区,对农村污水治理设施进出水中典型抗生素(包括6种磺胺类、3种四环素类、1种喹诺酮类抗生素)的浓度水平进行分析。结果表明,3处农村污水治理设施进水和出水中均检出不同程度的抗生素,浓度范围分别在ND~417.57 ng/L和ND~253.68 ng/L,其中土霉素浓度最高,进出水的浓度分别为417.57、253.68 ng/L;其次是氧氟沙星,在进出水中的最高浓度分别为278.75、183.73 ng/L。3处农村污水治理设施对抗生素的去除率在-58.32%~45.52%,对目标抗生素的去除率较... 相似文献