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681.
Analysis of per- and polyfluorinated alkyl substances in air samples from Northwest Europe 总被引:1,自引:0,他引:1
Barber JL Berger U Chaemfa C Huber S Jahnke A Temme C Jones KC 《Journal of environmental monitoring : JEM》2007,9(6):530-541
Air samples were collected from 4 field sites in Europe: 2 sites from the UK, Hazelrigg (semi-rural) and Manchester (urban); 1 site from Ireland: Mace Head (rural); and 1 site from Norway: Kjeller (rural). Additionally, air samples were taken from indoor locations in Troms?, Norway. Air samples were collected using high-volume air samplers employing sampling modules containing glass-fibre filters (GFFs, particle phase), and glass columns with a polyurethane foam (PUF)-XAD-2-PUF sandwich (gaseous phase). Typical outdoor air volumes required for the determination of per- and polyfluorinated alkyl substances (PFAS) ranged from 500-1800 m3. GFFs and PUF-XAD columns were analysed separately to obtain information on phase partitioning. All air samples were analysed for volatile, neutral PFAS, with selected GFF samples halved for analysis of both neutral and airborne particle-bound ionic PFAS. Volatile PFAS were extracted from air samples by cold-column immersion with ethyl acetate, and were analysed by gas chromatography-mass spectrometry in the positive chemical ionisation mode (GC-PCI-MS). Ionic PFAS were extracted from GFFs by sonication in methanol, and were analysed by liquid chromatography-time-of-flight-mass spectrometry (LC-TOF-MS) using electrospray ionisation in the negative ion mode (ESI-). Perfluorooctanoate (PFOA) was often the predominant analyte found in the particulate phase at concentrations ranging from 1-818 pg m(-3), and 8:2 fluorotelomer alcohol (FTOH) and 6:2 FTOH were the prevailing analytes found in the gas phase, at 5-243 pg m(-3) and 5-189 pg m(-3), respectively. These three PFAS were ubiquitous in air samples. Many other PFAS, both neutral and ionic, were also present, and levels of individual analytes were in the 1-125 pg m(-3) range. Levels of some PFAS exceeded those of traditional persistent organic pollutants (POPs). In this study, the presence of 12:2 FTOH and fluorotelomer olefins (FTolefins), and ionic PFAS other than perfluorooctane sulfonate (PFOS) and PFOA, are reported in air samples for the first time. Concentrations of neutral PFAS were several orders of magnitude higher in indoor air than outdoor air, making homes a likely important diffuse source of PFAS to the atmosphere. Our repeated findings of non-volatile ionic PFAS in air samples raises the possibility that they might directly undergo significant atmospheric transport on particles away from source regions, and more atmospheric measurements of ionic PFAS are strongly recommended. 相似文献
682.
Djati Utomo Handojo Li Xiaodong Ng Eng Tak Jonathan 《Environmental science and pollution research international》2022,29(14):20078-20084
Environmental Science and Pollution Research - 相似文献
683.
Jonathan M. P. Torres Kalina Bermúdez Marmolejo-Rodríguez Ana Judith López Eugenia López 《Environmental science and pollution research international》2022,29(41):61547-61549
Environmental Science and Pollution Research - 相似文献
684.
Heintz William J. Willis Jonathan M. 《Environmental science and pollution research international》2022,29(44):66148-66159
Environmental Science and Pollution Research - Oil spills are a significant stressor to coastal and maritime environments worldwide. The growth responses of Batis maritima and Avicennia germinans... 相似文献
685.
Escobar-Flores Jonathan Gabriel Sandoval Sarahi Gámiz-Romero Eduardo 《Environmental science and pollution research international》2022,29(41):61662-61673
Environmental Science and Pollution Research - In this study, six supervised classification algorithms were compared. The algorithms were based on cluster analysis, distance, deep learning, and... 相似文献
686.
Nick Hahlbeck William R. Tinniswood Matthew R. Sloat Jordan D. Ortega Matthew A. Wyatt Mark E. Hereford Ben S. Ramirez David A. Crook Kara J. Anlauf-Dunn Jonathan B. Armstrong 《Conservation biology》2022,36(3):e13857
A central tenet of landscape ecology is that mobile species depend on complementary habitats, which are insufficient in isolation, but combine to support animals through the full annual cycle. However, incorporating the dynamic needs of mobile species into conservation strategies remains a challenge, particularly in the context of climate adaptation planning. For cold-water fishes, it is widely assumed that maximum temperatures are limiting and that summer data alone can predict refugia and population persistence. We tested these assumptions in populations of redband rainbow trout (Oncorhynchus mykiss newberrii) in an arid basin, where the dominance of hot, hyperproductive water in summer emulates threats of climate change predicted for cold-water fish in other basins. We used telemetry to reveal seasonal patterns of movement and habitat use. Then, we compared contributions of hot and cool water to growth with empirical indicators of diet and condition (gut contents, weight–length ratios, electric phase angle, and stable isotope signatures) and a bioenergetics model. During summer, trout occurred only in cool tributaries or springs (<20 °C) and avoided Upper Klamath Lake (>25 °C). During spring and fall, ≥65% of trout migrated to the lake (5–50 km) to forage. Spring and fall growth (mean [SD] 0.58% per day [0.80%] and 0.34 per day [0.55%], respectively) compensated for a net loss of energy in cool summer refuges (–0.56% per day [0.55%]). In winter, ≥90% of trout returned to tributaries (25–150 km) to spawn. Thus, although perennially cool tributaries supported thermal refuge and spawning, foraging opportunities in the seasonally hot lake ultimately fueled these behaviors. Current approaches to climate adaptation would prioritize the tributaries for conservation but would devalue critical foraging habitat because the lake is unsuitable and unoccupied during summer. Our results empirically demonstrate that warm water can fuel cold-water fisheries and challenge the common practice of identifying refugia based only on summer conditions. 相似文献