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61.
Paul Bardos Brian Bone Miroslav Černík Daniel W. Elliott Sarah Jones Corinne Merly 《补救:环境净化治理成本、技术与工艺杂志》2015,25(2):83-94
Nanoscale zero‐valent iron (nZVI) is the most commonly used nanoremediation material. While there has been a reasonable level of application of nZVI technologies for in situ remediation in the United States, its utilization across Europe has been much more limited. There has been significant uncertainty about the balance between deployment risks and benefits for nanoparticles (NPs), which has affected the regulatory position in several countries. Some member states of the European Union (EU) take a strong precautionary view of the risks from the deployment of NPs into the subsurface, preventing the adoption of the technology. This article provides a risk–benefit assessment for nZVI based on published information and describes the steps that will be taken by a major European research project (NanoRem), as part of its work to provide a basis for better informed decision making in European environmental restoration markets. A key part of this process is dialogue between practitioners and researchers. NanoRem therefore has an active process of communication with different stakeholder networks (regulators, service providers, and site owners). NanoRem hopes to stimulate a consensus on appropriate use of nanoremediation and thereby stimulate effective technology transfer to the European remediation market. ©2015 The Authors 相似文献
62.
Spatial and temporal variation of metal concentrations in adult honeybees (Apis mellifera L.) 总被引:1,自引:0,他引:1
van der Steen JJ de Kraker J Grotenhuis T 《Environmental monitoring and assessment》2012,184(7):4119-4126
Honeybees (Apis mellifera L.) have great potential for detecting and monitoring environmental pollution, given their wide-ranging foraging behaviour. Previous studies have demonstrated that concentrations of metals in adult honeybees were significantly higher at polluted than at control locations. These studies focused at a limited range of heavy metals and highly contrasting locations, and sampling was rarely repeated over a prolonged period. In our study, the potential of honeybees to detect and monitor metal pollution was further explored by measuring the concentration in adult honeybees of a wide range of trace metals, nine of which were not studied before, at three locations in the Netherlands over a 3-month period. The specific objective of the study was to assess the spatial and temporal variation in concentration in adult honeybees of Al, As, Cd, Co, Cr, Cu, Li, Mn, Mo, Ni, Pb, Sb, Se, Sn, Sr, Ti, V and Zn. In the period of July-September 2006, replicated samples were taken at 2-week intervals from commercial-type bee hives. The metal concentration in micrograms per gram honeybee was determined by inductive coupled plasma-atomic emission spectrometry. Significant differences in concentration between sampling dates per location were found for Al, Cd, Co, Cr, Cu, Mn Sr, Ti and V, and significant differences in average concentration between locations were found for Co, Sr and V. The results indicate that honeybees can serve to detect temporal and spatial patterns in environmental metal concentrations, even at relatively low levels of pollution. 相似文献
63.
Elie Gaget Alison Johnston Diego Pavón-Jordán Aleksi S. Lehikoinen Brett K. Sandercock Alaaeldin Soultan Luka Božič Preben Clausen Koen Devos Cristi Domsa Vitor Encarnação Sándor Faragó Niamh Fitzgerald Teresa Frost Clemence Gaudard Lívia Gosztonyi Fredrik Haas Menno Hornman Tom Langendoen Christina Ieronymidou Leho Luigujõe Włodzimierz Meissner Tibor Mikuska Blas Molina Zuzana Musilová Jean-Yves Paquet Nicky Petkov Danae Portolou Jozef Ridzoň Laimonas Sniauksta Antra Stīpniece Norbert Teufelbauer Johannes Wahl Marco Zenatello Jon E. Brommer 《Conservation biology》2022,36(4):e13877
Protected area networks help species respond to climate warming. However, the contribution of a site's environmental and conservation-relevant characteristics to these responses is not well understood. We investigated how composition of nonbreeding waterbird communities (97 species) in the European Union Natura 2000 (N2K) network (3018 sites) changed in response to increases in temperature over 25 years in 26 European countries. We measured community reshuffling based on abundance time series collected under the International Waterbird Census relative to N2K sites’ conservation targets, funding, designation period, and management plan status. Waterbird community composition in sites explicitly designated to protect them and with management plans changed more quickly in response to climate warming than in other N2K sites. Temporal community changes were not affected by the designation period despite greater exposure to temperature increase inside late-designated N2K sites. Sites funded under the LIFE program had lower climate-driven community changes than sites that did not received LIFE funding. Our findings imply that efficient conservation policy that helps waterbird communities respond to climate warming is associated with sites specifically managed for waterbirds. 相似文献
64.
Černoch I Fránek M Diblíková I Hilscherová K Randák T Ocelka T Bláha L 《Journal of environmental monitoring : JEM》2012,14(1):250-257
Sulfonamide antibiotics coming from both human and veterinary medicine are among the most common emerging pollutants in freshwater. The present paper shows the successful application of passive sampling using POCIS in combination with an immunochemical ELISA technique and HPLC/MS/MS analysis to study the distribution of sulfonamides in streams around small towns in the Czech Republic, as well as around a major agglomeration of the city of Brno, including its waste water treatment plant (WWTP). Results indicated the presence of sulfonamides at most studied sites with concentrations ranging from <20 up to 736 ng of sulfamethoxazole equivalents per POCIS. Very high levels were detected in both the influent and effluent of the Brno WWTP with maxima > 8000 ng SMX per POCIS. All samplers collected down-stream of the studied towns and WWTPs clearly showed an increase in sulfonamide drug residues. Higher concentrations were determined in rivers at the city of Brno agglomeration. In agreement with other available studies, these findings indicate low efficiency of conventional WWTPs to eliminate polar pharmaceuticals such as sulfonamides. Good performance and correlation with the LC/MS results, as well as ease of use, indicate good potential for the immunochemical ELISA technique to become the screening tool for sulfonamide determination in surface waters including passive samplers. 相似文献
65.
Edgar Hiller Slavomír Čerňanský Zoltán Krascsenits Ján Milička 《Environmental science and pollution research international》2009,16(5):546-554
Background, aim, and scope Herbicide fate and its transport in soils and sediments greatly depend upon sorption–desorption processes. Quantitative determination
of herbicide sorption–desorption is therefore essential for both the understanding of transport and the sorption equilibrium
in the soil/sediment–water system; and it is also an important parameter for predicting herbicide fate using mathematical
simulation models. The total soil/sediment organic carbon content and its qualitative characteristics are the most important
factors affecting sorption–desorption of herbicides in soil or sediment. Since the acetochlor is one of the most frequently
used herbicides in Slovakia to control annual grasses and certain annual broad-leaved weeds in maize and potatoes, and posses
various negative health effects on human beings, our aim in this study was to investigate acetochlor sorption and desorption
in various soil/sediment samples from Slovakia. The main soil/sediment characteristics governing acetochlor sorption–desorption
were also identified.
Materials and methods The sorption–desorption of acetochlor, using the batch equilibration method, was studied on eight surface soils, one subsurface
soil and five sediments collected from the Laborec River and three water reservoirs. Soils and sediments were characterized
by commonly used methods for their total organic carbon content, distribution of humus components, pH, grain-size distribution,
and smectite content, and for calcium carbonate content. The effect of soil/sediment characteristics on acetochlor sorption–desorption
was examined by simple correlation analysis.
Results Sorption of acetochlor was expressed as the distribution coefficient (K
d). K
d values slightly decreased as the initial acetochlor concentration increased. These values indicated that acetochlor was moderately
sorbed by soils and sediments. Highly significant correlations between the K
d values and the organic carbon content were observed at both initial concentrations. However, sorption of acetochlor was most
closely correlated to the humic acid carbon, and less to the fulvic acid carbon. The total organic carbon content was found
to also significantly influence acetochlor desorption.
Discussion Since the strong linear relationship between the K
d values of acetochlor and the organic carbon content was already released, the corresponding K
oc values were calculated. Considerable variation in the K
oc values suggested that other soil/sediment parameters besides the total soil organic carbon content could be involved in acetochlor
sorption. This was revealed by a significant correlation between the K
oc values and the ratio of humic acid carbon to fulvic acid carbon (CHA/CFA).
Conclusions When comparing acetochlor sorption in a range of soils and sediments, different K
d values which are strongly correlated to the total organic carbon content were found. Concerning the humus fractions, the
humic acid carbon content was strongly correlated to the K
d values, and it is therefore a better predictor of the acetochlor sorption than the total organic carbon content. Variation
in the K
oc values was attributed to the differences in distribution of humus components between soils and sediments. Desorption of acetochlor
was significantly influenced by total organic carbon content, with a greater organic carbon content reducing desorption.
Recommendations and perspectives This study examined the sorption–desorption processes of acetochlor in soils and sediments. The obtained sorption data are
important for qualitative assessment of acetochlor mobility in natural solids, but further studies must be carried out to
understand its environmental fate and transport more thoroughly. Although, the total organic carbon content, the humus fractions
of the organic matter and the CHA/CFA ratio were sufficient predictors of the acetochlor sorption–desorption. Further investigations of the structural and chemical
characteristics of humic substances derived from different origins are necessary to more preciously explain differences in
acetochlor sorption in the soils and sediments observed in this study. 相似文献
66.
67.
Ulrike Kummer Jozef Pacyna Elisabeth Pacyna Rainer Friedrich 《Atmospheric environment (Oxford, England : 1994)》2009,43(3):640-647
An emission inventory was compiled for heavy metal air emissions from road transport in Europe (EU-40). For the database, country-specific data was taken such as the diesel and gasoline fuel consumption per country, the content of Pb in gasoline and diesel fuel and the share of different vehicle types. For tyre and brake wear emissions, average wear rates and heavy metal contents of different materials were used to develop emission factors for tyre and brake wear. It covers exhaust emissions (Pb from gasoline and diesel) as well as non-exhaust emissions (As, Cd, Cr, Ni and Pb from the wear of brake linings and vehicle tyres). The base year is 2000, and two scenarios were developed for 2010, a business as usual (BAU) scenario and a maximum feasible technical reduction (MFTR) scenario. Both result in a remarkable decrease in Pb exhaust emissions and a rising share of non-exhaust emissions. To assess the results, the inventory is (a) compared to an inventory compiled with a top-down approach that covers the same area and years but only emissions from combustion processes and (b) added to an inventory covering all sectors for heavy metal air emissions. 相似文献
68.
František Štork Martin Bačkor Bořivoj Klejdus Josef Hedbavny Jozef Kováčik 《Environmental science and pollution research international》2013,20(8):5502-5511
Effect of nitric oxide donor (sodium nitroprusside, SNP, 500 μM) or hydrogen peroxide scavenger (dithiothreitol, DTT, 500 μM) on cadmium (Cd) or copper (Cu) uptake (150 μM solutions) and toxicity using Scenedesmus quadricauda was studied. Combined treatments (Cd or Cu + DTT or SNP) usually ameliorated metal-induced toxicity at the level of pigments, proteins, and mineral nutrients in comparison with respective metal alone. Viability tests (MTT and TTC) showed the lowest values preferentially in Cu treatments, indicating higher toxicity in comparison with Cd. Cd showed low impact on amino acids while strong Cu-induced depletion was mitigated by DTT and SNP. Amount of ROS and NO showed the most pronounced responses in SNP variants being rather reciprocal than parallel and regulated ascorbate peroxidase activity. Blot gel analyses of hsp70 protein did not reveal extensive changes after given exposure period. Phenols were elevated by DTT alone while all Cu treatments revealed depletion. Total Cu content decreased while total Cd content increased in metal + SNP or metal + DTT. Subsequent experiment using lower Cd, SNP or DTT doses (10 and 100 μM) revealed concentration-dependent impact on Cd uptake. Overall, DTT was found to be more suitable for the amelioration of metal-induced toxicity. 相似文献
69.
Jana Chovancová Beáta Drobná Anna Fabišiková Kamil Čonka Soňa Wimmerová Marian Pavuk 《Environmental monitoring and assessment》2014,186(11):7643-7653
The concentrations of indicator polychlorinated biphenyls (PCBs No. 28, 52, 101, 138, 153 and 180) and organochlorine pesticides (HCB, p,p′-DDE and p,p′-DDT) in 121 blood serum specimens collected from non-occupationally exposed adults living in contaminated and comparison areas were determined using high-resolution gas chromatography/electron capture detection (HRGC/ECD). The sum of the serum concentrations of the three most abundant PCB congeners (No. 138, 153 and 180) found in participants (N?=?81) living in industrial areas near incinerators, metallurgical and chemical plants (Krompachy, Kosice, Nemecka and Sala) was significantly higher (p?0.001) than in participants living in villages and towns without known sources causing persistent organic pollutant (POP) contamination (N?=?40). Similarly, significant differences were observed for p,p′-DDE (p?0.0001) and p,p′-DDT (p?0.002). However, a Mann-Whitney U test between groups showed that the difference for HCB was not statistically significant (p?=?0.089). Age was positively correlated with the sum of PCBs (No. 138, 153 and 180), HCB and the sum of p,p′-DDE and p,p′-DDT (p?0.01 for all). 相似文献
70.