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941.
Zhiling Gao Raymond L. Desjardins Thomas K. Flesch 《Atmospheric environment (Oxford, England : 1994)》2010,44(26):3128-3134
Dispersion techniques are useful for assessing the effectiveness of management practices in mitigating methane (CH4) emissions from animal operations. In this paper, the accuracy of an inverse-dispersion technique was examined for two common situations: 1) emissions from animals in a barn and 2) emissions from animals in a pen. For both situations, the accuracy of emission estimates generally increased with increasing fetch (scaled to barn height, h, or to pen width, Xs) between the source and the concentration measurement. The gas recovery ratio increased from 0.66 at 5 h to 0.93–1.03 at 10 h–25 h for the barn, and decreased from 1.59 at 0 Xs to 0.99 at 5 Xs and from 1.54 at 0 Xs to 1.09 at 5 Xs for the two small pen scenarios, due to the declining sensitivity of the dispersion model to errors in wind complexity and errors in the assumed source configuration. However, the relative uncertainty of the measured concentration increased with fetch due to the decreasing gas concentrations. Hence, improving the accuracy of emission estimates is a compromise between the source configuration sensitivity and the concentration measurement sensitivity. Fetches of about twice the size of the pen and about 10 times the height of the barn are suggested. 相似文献
942.
L.-W. Antony Chen John G. Watson Judith C. Chow David W. DuBois Lisa Herschberger 《Atmospheric environment (Oxford, England : 1994)》2010,44(38):4908-4918
The Minnesota Particulate Matter 2.5 (PM2.5) Source Apportionment Study was undertaken to explore the utility of PM2.5 mass, element, ion, and carbon measurements from long-term speciation networks for pollution source attribution. Ambient monitoring data at eight sites across the state were retrieved from the archives of the Interagency Monitoring of Protected Visual Environments (IMPROVE) and the Speciation Trends Network (STN; part of the Chemical Speciation Network [CSN]) and analyzed by an Effective Variance – Chemical Mass Balance (EV-CMB) receptor model with region-specific geological source profiles developed in this study. PM2.5 was apportioned into contributions of fugitive soil dust, calcium-rich dust, taconite (low grade iron ore) dust, road salt, motor vehicle exhaust, biomass burning, coal-fired utility, and secondary aerosol. Secondary sulfate and nitrate contributed strongly (49–71% of PM2.5) across all sites and was dominant (≥60%) at IMPROVE sites. Vehicle exhausts accounted for 20–70% of the primary PM2.5 contribution, largely exceeding the proportion in the primary PM2.5 emission inventory. The diesel exhaust contribution was separable from the gasoline engine exhaust contribution at the STN sites. Higher detection limits for several marker elements in the STN resulted in non-detectable coal-fired boiler contributions which were detected in the IMPROVE data. Despite the different measured variables, analytical methods, and detection limits, EV-CMB results from a nearby IMPROVE-STN non-urban/urban sites showed similar contributions from regional sources – including fugitive dust and secondary aerosol. Seasonal variations of source contributions were examined and extreme PM2.5 episodes were explained by both local and regional pollution events. 相似文献
943.
L.Q. Xu L.G. Sun H. Yan Y.H. Luo Y.H. Wang 《Journal of environmental radioactivity》2010,101(5):362-368
Several natural and anthropogenic radionuclides (210Pb, 226Ra and 137Cs) in guano-phosphatic coral sediments and pure guano particles collected from Ganquan, Guangjin, Jinqing and Jinyin Islands of the Xisha archipelago, South China Sea, were analyzed. The Constant Initial Concentration (CIC) model and the Constant Rate of Supply (CRS) model were applied for age calculation. The average supply rate of 210Pb was 126 Bq m−2 a−1, very close to the flux of northern hemisphere average (125 Bq m−2 a−1). The activities of anthropogenic radionuclides in the sediments were very low, indicating that human nuclear tests did not notably impact this region. The main source of radionuclides in the sediments was from atmospheric precipitation, and the organic matter derived from plant and produced by nutrient-rich guano could further enhance them. 相似文献
944.
To study the Pu concentration and isotope ratio distributions present in China, the 239+240Pu total activities and 240Pu/239Pu atom ratios in core soil samples from Hubei Province in central China were investigated using Accelerator Mass Spectrometry (AMS). The activities ranged from 0.019 to 0.502 mBq g−1 and the 239+240Pu inventories of 45 and ∼55 Bq m−2 agree well with that expected from global fallout. The 240Pu/239Pu atom ratios in the soil ranged from 0.172 to 0.220. The ratios are similar to typical global fallout values. Hence, any close-in fallout contribution from the Chinese nuclear weapons tests, mainly conducted in the 1970s, must have either been negligible or had a similar 240Pu/239Pu ratio to that of global fallout. The top 10 cm layer of the soil contributes ∼90% of the total inventory and the maximum concentrations appeared in the 2-4 cm or 4-6 cm layers. It is suggested that climatic conditions and organic content are the two main factors that affect the vertical migration of plutonium in soil. 相似文献
945.
946.
Southern Chile encompasses one of the most extensive fjord regions of the world, the Patagonia, currently exposed to natural
and anthropogenic perturbations. These fjord ecosystems provide important services to humans, which have not been adequately
measured and valued. As a consequence, ecosystem services are commonly ignored in public policy design and in the evaluation
of development projects. Here we tackle questions that are highly relevant for the nation’s development, namely (1) understanding
fjord functioning, and (2) developing management strategies based on ecosystem services, in order to secure simultaneous and
adequate use of these ecosystems which area influenced by ecological (e.g., biogeochemical) and productive (e.g., aquaculture,
fisheries) processes. We also seek to strengthen the analysis of fjord ecosystem value from the economical (including coastal
zoning), socio-cultural, institutional, and governmental points of view. In addition, the investigation of current and future
effects of climate change on this large region offers a unique opportunity to understand the social and economic consequences
of a global phenomenon at local to regional scales. Biogeochemical and socio-economic models will be used to simulate future
scenarios under a gamut of management options. 相似文献
947.
Laura B. Brentner Sachiyo T. Mukherji Jerald L. Schnoor 《Environmental pollution (Barking, Essex : 1987)》2010,158(2):470-475
Phosphor imager autoradiography is a technique for rapid, sensitive analysis of the localization of xenobiotics in plant tissues. Use of this technique is relatively new to research in the field of plant science, and the potential for enhancing visualization and understanding of plant uptake and transport of xenobiotics remains largely untapped. Phosphor imager autoradiography is used to investigate the uptake and translocation of the explosives 1,3,5-trinitro-1,3,5-triazine (RDX) and 2,4,6-trinitrotoluene within Populus deltoides × nigra DN34 (poplar) and Panicum vigratum Alamo (switchgrass). In both plant types, TNT and/or TNT-metabolites remain predominantly in root tissues while RDX and/or RDX-metabolites are readily translocated to leaf tissues. Phosphor imager autoradiography is further investigated for use in semi-quantitative analysis of uptake of TNT by switchgrass. 相似文献
948.
Katherine B. Beem Florian M. Schwandner Taehyoung Lee Christian M. Carrico Derek Day Jenny Hand Bret Schichtel Jeffrey L. Collett Jr. 《Environmental pollution (Barking, Essex : 1987)》2010,158(3):862-872
Increases in reactive nitrogen deposition are a growing concern in the U.S. Rocky Mountain west. The Rocky Mountain Airborne Nitrogen and Sulfur (RoMANS) study was designed to improve understanding of the species and pathways that contribute to nitrogen deposition in Rocky Mountain National Park (RMNP). During two 5-week field campaigns in spring and summer of 2006, the largest contributor to reactive nitrogen deposition in RMNP was found to be wet deposition of ammonium (34% spring and summer), followed by wet deposition of nitrate (24% spring, 28% summer). The third and fourth most important reactive nitrogen deposition pathways were found to be wet deposition of organic nitrogen (17%, 12%) and dry deposition of ammonia (14%, 16%), neither of which is routinely measured by air quality/deposition networks operating in the region. Total reactive nitrogen deposition during the spring campaign was determined to be 0.45 kg ha−1 and more than doubled to 0.95 kg ha−1 during the summer campaign. 相似文献
949.
The forest hydrologic budget may be impacted by increasing CO2 and tropospheric O3. Efficient means to quantify such effects are beneficial. We hypothesized that changes in the balance of canopy interception, stem flow, and through-fall in the presence of elevated CO2 and O3 could be discerned using image analysis of leafless branches. We compared annual stem flow to the results of a computerized analysis of all branches from the 2002, 2004, and 2006 annual growth whorls of 97 ten-year-old trees from the Aspen Free-Air CO2 and O3 Enrichment (Aspen FACE) experiment in Rhinelander, WI. We found significant effects of elevated CO2 and O3 on some branch metrics, and that the branch metrics were useful for predicting stem flow from birch, but not aspen. The results of this study should contribute to development of techniques for efficient characterization of effects on the forest hydrologic budget of increasing CO2 and tropospheric O3. 相似文献
950.
Kheirghadam Enayatzamir Hossein A. Alikhani Bagher Yakhchali Fatemeh Tabandeh Susana Rodríguez-Couto 《Environmental science and pollution research international》2010,17(1):145-153