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671.
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The distribution of PCDD/F and a selection of heavy metals in the surrounding area of the Hazardous Waste Incinerator (HWI) at Schwabach has been determined. The PCDD/F concentrations measured in soil, grass and lettuce samples are compared to modeling studies realized by the TÜV Bayern. 相似文献
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S. Hellsten U. Dragosits C. J. Place T. H. Misselbrook Y. S. Tang M. A. Sutton 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):3-13
Most ammonia (NH3) emission inventories have been calculated on an annual basis and do not take into account the seasonal variability of emissions
that occur as a consequence of climate and agricultural practices that change throughout the year. When used as input to atmospheric
transport models to simulate concentration fields, these models therefore fail to capture seasonal variations in ammonia concentration
and dry and wet deposition. In this study, seasonal NH3 emissions from agriculture were modelled on a monthly basis for the year 2000, by incorporating temporal aspects of farming
practice. These monthly emissions were then spatially distributed using the AENEID model (Atmospheric Emissions for National
Environmental Impacts Determination). The monthly model took the temporal variation in the magnitude of the ammonia emissions,
as well as the fine scale (1-km) spatial variation of those temporal changes into account to provide improved outputs at 5-km
resolution. The resulting NH3 emission maps showed a strong seasonal emission pattern, with the highest emissions during springtime (March and April) and
the lowest emissions during summer (May to July). This emission pattern was mainly influenced by whether cattle were outside
grazing or housed and by the application of manures and fertilizers to the land. When the modelled emissions were compared
with measured NH3 concentrations, the comparison suggested that the modelled emission trend corresponds fairly well with the seasonal trend
in the measurements. The remaining discrepancies point to the need to develop functional parametrisations of the interactions
with climatic seasonal variation. 相似文献
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677.
A supercritical fluid extraction (SFE) method was developed for the extraction of polycyclic aromatic hydrocarbons (PAHs) from fresh and fallen pine needles. Toluene-modified CO2 was used as the extracting fluid, and the extracted PAHs were analyzed by GC-MS. Using a two-stage extraction procedure, a static extraction at 180 degrees C and a dynamic extraction at 60 degrees C, and an in-cell silica gel plug plus a post-oven silica gel column, the extraction and fractionation of PAHs can be accomplished in one step. Over a seven month period, a significant variation was observed for PAHs in urban samples, while PAHs in mountain samples were at much lower levels (by a factor of approximately 8) and showed little seasonal change. Although dry fallen needles and fresh needles contained similar amounts of PAHs, in the fallen needles the lower molecular weight PAHs were partially lost while the higher molecular weight PAHs were slightly enriched. Pollution in urban areas was found to be highly localized, and buildings and trees are believed to be important factors in the restriction of atmospheric PAHs. 相似文献
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Rahman MM Rahman MM Koddus A Ahmad GU Voigt G 《Journal of environmental radioactivity》2005,83(2):199-211
Soil-to-plant transfer factors (TF) of radiocaesium (137Cs) were determined under field condition for grassy vegetation grown in Bangladesh at contaminated land in the Atomic Energy Research Establishment (AERE) campus. TF values for rice, grass and grassy/root vegetations grown in the same type of soil were also measured under pot condition. TF values of 137Cs for grassy vegetation (2.4 x 10(-2) -4.2 x 10(-2) with an average of 3.1 x 10(-2) +/-0.005) obtained under field condition were slightly lower than the values for grass and grassy/root vegetations (2.9 x 10(-2) -6.6 x 10(-2) with an average of 4.8 x 10(-2) +/-0.01 for grass and grassy vegetations and 2.3 x 10(-2) -5.6 x 10(-2) with an average of 4.0 x 10(-2) +/-0.009 for root vegetations, respectively) obtained under pot condition. However, TF values (9.0 x 10(-3) -2.6 x 10(-2) with an average of 1.9 x 10(-2) +/-0.004) obtained for rice were about a factor of 4 lower than the values obtained for grass and grassy/root vegetations. When the properties of the AERE soils as input parameters were used in the soil-plant transfer model of Absalom, the estimated TF values (4.5 x 10(-2) -6.7 x 10(-2) with an average of 5.3 x 10(-2) +/-0.006) were consistent with the measured values obtained for grass and grassy vegetations under pot condition, however, the model overestimates the TF values for rice. 相似文献